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We demonstrate the capability of growing high quality ultrathin films of the topological insulators Bi2Se3 and Bi2Te3 using molecular beam epitaxy. Unlike previous growth techniques, which often pin the Fermi energy in the conduction band…

Materials Science · Physics 2014-01-15 J. J. Lee , F. T. Schmitt , R. G. Moore , I. M. Vishik , Y. Ma , Z. X. Shen

The naturally existing chalcogenide Bi2Se3 is topologically nontrivial due to the band inversion caused by strong spin-orbit coupling inside the bulk of the material. The surface states are spin polarized, protected by the time-inversion…

Materials Science · Physics 2021-11-11 Zhengtianye Wang , Stephanie Law

Bulk Bi2Te3 is known to be a topological insulator. We investigate surface states of Bi2Te3(111) thin films using density-functional theory including spin-orbit coupling. We construct a method to unambiguously identify surface states of…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Kyungwha Park , J. J. Heremans , V. W. Scarola , Djordje Minic

The surface electronic properties of the important topological insulator Bi2Te3 are shown to be robust under an extended surface preparation procedure which includes exposure to atmosphere and subsequent cleaning and recrystallization by an…

Materials Science · Physics 2015-05-27 L. Plucinski , G. Mussler , J. Krumrain , S. Suga , D. Gruetzmacher , C. M. Schneider

We consider in our work high quality single crystal thin films of Bi2Se3, grown by molecular beam epitaxy, both with and without Pb doping. Our ARPES data demonstrate topological surface states with a Fermi level lying inside the bulk band…

Mesoscale and Nanoscale Physics · Physics 2012-01-20 Jian Wang , Ashley M. DaSilva , Cui-Zu Chang , Ke He , J. K. Jain , Nitin Samarth , Xu-Cun Ma , Qi-Kun Xue , Moses H. W. Chan

Ultrathin topological insulator membranes are building blocks of exotic quantum matter. However, traditional epitaxy of these materials does not facilitate stacking in arbitrary orders, while mechanical exfoliation from bulk crystals is…

Bi2Se3 is theoretically predicted1 2and experimentally observed2,3 to be a three dimensional topological insulator. For possible applications, it is important to understand the electronic structure of the planar device. In this work,…

Epitaxial thin films of (Sn$_{x}$Pb$_{1-x}$)$_{1-y}$In$_{y}$Te were successfully grown by molecular-beam-epitaxy (MBE) in a broad range of compositions (0 $\leq$ x $\leq$ 1, 0 $\leq$ y $\leq$ 0.23). We investigated electronic phases of the…

We use real-time reflection high energy electron diffraction intensity oscillation to establish the Te-rich growth dynamics of topological insulator thin films of Bi2Te3 on Si(111) substrate by molecular beam epitaxy. In situ angle resolved…

We have identified epitaxially grown elemental Te as a capping material that is suited to protect the topological surface states of intrinsically insulating Bi$_2$Te$_3$. By using angle-resolved photoemission, we were able to show that the…

Materials Science · Physics 2017-04-04 Katharina Höfer , Christoph Becker , Steffen Wirth , Liu Hao Tjeng

Ternary (Bi1-xSbx)2Te3 films with an Sb content between 0 and 100% were deposited on a Si(111) substrate by means of molecular beam epitaxy. X-ray diffraction measurements confirm single crystal growth in all cases. The Sb content is…

Topological insulators are novel quantum materials with metallic surface transport, but insulating bulk behavior. Often, topological insulators are dominated by bulk contributions due to defect induced bulk carriers, making it difficult to…

A topological insulator (TI), a new quantum state featured with the topologically-protected surface state (TSS) originating from its peculiar topology in band structure, has attracted much interest due to academic and practical importance.…

Materials Science · Physics 2016-12-14 Seong Won Cho , Kwang-Chon Kim , Seong Keun Kim , Byung-ki Cheong , Jin-Sang Kim , Suyoun Lee

SrMoO$_3$ is a promising material for its excellent electrical conductivity, but growing high-quality thin films remains a challenge. Here we synthesized epitaxial films of SrMoO$_3$ using the molecular beam epitaxy (MBE) technique under a…

High quality thin films of the topological insulator (Bi$_{0.4}$Sb$_{0.6}$)$_2$Te$_3$ have been deposited on SrTiO$_3$ (111) by molecular beam epitaxy. Their electronic structure was investigated by in situ angle-resolved photoemission…

Atomically flat thin films of topological insulator Bi2Se3 have been grown on double-layer graphene formed on 6H-SiC(0001) substrate by molecular beam epitaxy. By a combined study of reflection high energy electron diffraction and scanning…

Topological insulators are insulating in the bulk but possess spin-momentum locked metallic surface states protected by time-reversal symmetry. The existence of these surface states has been confirmed by angle-resolved photoemission…

Materials Science · Physics 2012-11-09 Jian Wang , Handong Li , Cui-Zu Chang , Ke He , Joon Sue Lee , Xu-Cun Ma , Nitin Samarth , Qi-Kun Xue , Maohai Xie , M. H. W. Chan

The superconductor Sn$_{1-x}$In$_{x}$Te is derived from the topological crystalline insulator SnTe and is a candidate topological superconductor. So far, high-quality thin films of this material have not been available, even though such…

Materials Science · Physics 2019-10-22 Andrea Bliesener , Junya Feng , A. A. Taskin , Yoichi Ando

Topological insulators(1-8) are a novel form of matter which features metallic surface states with quasirelativistic dispersion similar to graphene(9). Unlike graphene, the locking of spin and momentum and the protection by time-reversal…

Mesoscale and Nanoscale Physics · Physics 2012-07-23 M. R. Scholz , J. Sánchez-Barriga , D. Marchenko , A. Varykhalov , A. Volykhov , L. V. Yashina , O. Rader

High quality thin films of topological insulators (TI) such as Bi2Se3 have been successfully synthesized by molecular beam epitaxy (MBE). Although the surface of MBE films can be protected by capping with inert materials such as amorphous…

Materials Science · Physics 2014-12-10 Jixia Dai , Wenbo Wang , Matthew Brahlek , Nikesh Koirala , Maryam Salehi , Seongshik Oh , Weida Wu
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