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We demonstrate subpicosecond-time-scale population transfer between the pair of hyperfine ground states of atomic rubidium using a single laser-pulse. Our scheme utilizes the geometric and dynamic phases induced during Rabi oscillation…

Atomic Physics · Physics 2018-05-23 Yunheung Song , Han-gyeol Lee , Hyosub Kim , Hanlae Jo , Jaewook Ahn

We apply techniques of subriemannian geometry on Lie groups to laser-induced population transfer in a three-level quantum system. The aim is to induce transitions by two laser pulses, of arbitrary shape and frequency, minimizing the pulse…

Optimization and Control · Mathematics 2007-05-23 Ugo Boscain , Thomas Chambrion , Jean-Paul Gauthier

We present our experimental investigation of an optical Raman transition between the magnetic clock states of $^{87}$Rb in an atom chip magnetic trap. The transfer of atomic population is induced by a pair of diode lasers which couple the…

Atomic Physics · Physics 2016-08-03 J B Naber , L Torralbo-Campo , T Hubert , R J C Spreeuw

We improve by a factor of 4-20 the energy accuracy of the strongest soft X-ray transitions of Fe XVII ions by resonantly exciting them in an electron beam ion trap with a monochromatic beam at the P04 beamline of the PETRA III synchrotron…

We report the observation of a novel nonlinear effect in the hard x-ray range. Upon illuminating Fe and Cu metal foils with intense x-ray pulses tuned near their respective K edges, photons at nearly twice the incoming photon energy are…

We design, by invariant-based inverse engineering, driving fields that invert the population of a two-level atom in a given time, robustly with respect to dephasing noise and/or systematic frequency shifts. Without imposing constraints,…

Quantum Physics · Physics 2013-09-10 Xiao-Jing Lu , Xi Chen , A. Ruschhaupt , D. Alonso , S. Guérin , J. G. Muga

Data for inelastic processes due to hydrogen atom collisions with iron are needed for accurate modelling of the iron spectrum in late-type stars. Excitation and charge transfer in low-energy Fe+H collisions is studied theoretically using a…

Solar and Stellar Astrophysics · Physics 2018-05-09 P. S. Barklem

We design, by invariant-based inverse engineering, resonant laser pulses to perform fast population transfers in three-level systems. The efficiency and laser intensities are examined for different protocols. The energy cost to improve the…

Quantum Physics · Physics 2012-11-16 Xi Chen , J. G. Muga

Excitation and charge transfer in low-energy O+H collisions is studied; it is a problem of importance for modelling stellar spectra and obtaining accurate oxygen abundances in late-type stars including the Sun. The collisions have been…

Solar and Stellar Astrophysics · Physics 2018-02-28 P. S. Barklem

An analytic study is presented of the efficient multiphoton excitation and strong harmonic generation in three-level systems specified by a pair of nearly degenerate, strongly dipole-coupled excited states. Such systems are physically…

Quantum Physics · Physics 2015-05-19 Michal Berent , Ryszard Parzyński

The optimal control of population transfer for multi-level systems is investigated from the perspective of quantum geometry. Firstly, the general theoretical framework of optimizing the stimulated Raman adiabatic passage (STIRAP) scheme…

Quantum Physics · Physics 2025-12-24 Guan-Qiang Li , Yu-Qi Zhang , Hao Guo , You-Jiao Dong , Zhi-Yu Lin , Ping Peng

In a recent publication Larson \textit{et al.} reported remarkably clear $d$-$d$ excitations for NiO and CoO measured with x-ray energies well below the transition metal $K$ edge. In this letter we demonstrate that we can obtain an accurate…

Strongly Correlated Electrons · Physics 2008-01-09 M. W. Haverkort , A. Tanaka , L. H. Tjeng , G. A. Sawatzky

Achieving a high population of antihydrogen/hydrogen atoms in the 2S level is essential for spectroscopy measurements testing similarities between matter and antimatter. We propose and examine the efficiency of applying the STIRAP…

Atomic Physics · Physics 2025-09-19 AbdAlGhaffar K. Amer , A. Capra , T. Friesen , M. C. Fujiwara , T. Momose , C. So , F. Robicheaux

We present and implement a new scheme for independent control of both the final and the transient population utilizing the symmetry properties of the system. By proper pulse shaping, utilizing the invariance of the two-photon absorption to…

Atomic Physics · Physics 2009-10-20 Andrey Gandman , Leonid Rybak , Michal Bronstein , Naser Shakour , Zohar Amitay

We report and propose a simple scheme to achieve the ultrafast and selective population transfer in four-level atoms by utilizing a single frequency chirped few-cycle pulse. It is demonstrated that the almost complete population may be…

Quantum Physics · Physics 2015-06-15 Parvendra Kumar , Amarendra K. Sarma

High quality InN nanoparticles are grown using atmospheric chemical vapour deposition technique via a self-seeded catalytic approach in the temperature range of 580 to 650 oC. In this temperature region, nucleation barrier of InN is…

Materials Science · Physics 2016-08-24 Kishore K. Madapu , S. R. Polaki , Sandip Dhara

There has long been interest to control the transfer of population between specified quantum states. Recent work has optimized the control law for closed system population transfer by using a gradient ascent pulse engineer- ing algorithm…

Quantum Physics · Physics 2010-04-28 Wei Cui , Zairong Xi , Yu Pan

The influence of photon-momentum recoil on adiabatic population transfer in an atomic three-level lambda system is studied. It is shown that the Doppler frequency shifts, due to atomic motion can play an important role in adiabatic…

Quantum Physics · Physics 2016-11-03 R. G. Unanyan

We consider the population transfer process in a Lambda-type atomic medium of unequal oscillator strengths by stimulated Raman adiabatic passage via bright-state (b-STIRAP) taking into account propagation effects. Using both analytic and…

Quantum Physics · Physics 2013-06-11 G. G. Grigoryan , C. Leroy , Y. Pashayan-Leroy , L. Chakhmakhchyan , S. Guérin , H. R. Jauslin

We present a theoretical framework to describe state-resolved ionization dynamics of neon atoms driven by ultraintense x-ray free-electron-laser pulses. In general, x-ray multiphoton ionization dynamics of atoms have been described by…

Atomic Physics · Physics 2023-01-10 Laura Budewig , Sang-Kil Son , Robin Santra