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Time-resolved inelastic neutron scattering measurements on an array of single-crystals of the single-molecule magnet Mn12ac are presented. The data facilitate a spectroscopic investigation of the slow relaxation of the magnetization in this…

Other Condensed Matter · Physics 2009-11-11 O. Waldmann , G. Carver , C. Dobe , D. Biner , A. Sieber , H. U. Güdel , H. Mutka , J. Ollivier , N. E. Chakov

Current-induced magnetic switching of a single magnetic molecule attached to two ferromagnetic contacts is considered theoretically, with the main emphasis put on the role of intrinsic spin relaxation processes. It is shown that…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Maciej Misiorny , Józef Barnaś

Exponential and power law temperature dependences are widely used to fit experimental data of magnetic relaxation time in single molecular magnets. We derived a theory to show how these rules arise from the underling relaxation mechanisms…

Mesoscale and Nanoscale Physics · Physics 2020-09-16 Lei Gu , Ruqian Wu

Magnetic hysteresis has become a crucial aspect for characterizing single-molecule magnets, but the comprehension of the coercivity mechanism is still a challenge. By using analytical derivation and quantum dynamical simulations, we reveal…

Materials Science · Physics 2023-09-08 Lei Gu , Qiancheng Luo , Guoping Zhao , Yan-Zhen Zheng , Ruqian Wu

New Mn12 single-molecule magnets (SMM's) with the composition [Mn12O12(O2CR)16(H2O)4] were prepared and structurally characterized. Complexes of this type can exhibit two out-of-phase ac magnetic susceptibility signals, one in the 4-7 K…

Superparamagnetic colloids present interesting assembly dynamics and propulsion in time-varying magnetic fields due to their magnetic relaxation. However, little is known about the mechanisms governing this magnetic relaxation, which is…

A single-molecule magnet placed in a magnetic field perpendicular to its anisotropy axis can be truncated to an effective two-level system, with easily tunable energy splitting. The quantum coherence of the molecular spin is largely…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 A. Morello , A. Millán , L. J. de Jongh

The study of how spin interacts with lattice vibrations and relaxes to equilibrium provides unique insights on its chemical environment and the relation between electronic structure and molecular composition. Despite its importance for…

Materials Science · Physics 2022-08-23 Sourav Mondal , Alessandro Lunghi

We numerically study the relaxation of correlation functions in weakly perturbed integrable XXZ chain. The decay of the spin-current and the energy-current correlations at zero magnetization are well described by single, but quite distinct,…

Strongly Correlated Electrons · Physics 2022-08-08 M. Mierzejewski , J. Pawłowski , P. Prelovšek , J. Herbrych

We study the magnetization reversal and electromagnetic radiation due to collective Landau-Zener relaxation in a crystal of molecular magnets. Analytical and numerical solutions for the time dependence of the relaxation process are…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Collin L. Joseph , Carlos Calero , Eugene M. Chudnovsky

The effect of long range dipole-dipole interactions on the thermal fluctuations of the magnetization of an assembly of single-domain ferromagnetic particles is considered. If orientational correlations between the particles are neglected,…

Statistical Mechanics · Physics 2019-02-05 Pierre-Michel Déjardin

We derive a simple system of equations to describe the magnetization relaxation of a molecular spin in weak interaction with a thermal bath for the whole temperature domain. Using this for the intermediate temperature domain where the…

Materials Science · Physics 2022-12-27 Le Tuan Anh Ho , Liviu Ungur , Liviu F. Chibotaru

The Glauber dynamics is studied in a single-chain magnet. As predicted, a single relaxation mode of the magnetization is found. Above 2.7 K, the thermally activated relaxation time is mainly governed by the effect of magnetic correlations…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 C. Coulon , R. Clerac , L. Lecren , W. Wernsdorfer , H. Miyasaka

The magnetization relaxation of Mn12 single-molecule magnets (SMMs) does not follow a simple Arrhenius law, even for data collected at low frequencies (5-1500 Hz) due to contributions from relaxation pathways via excited states with larger…

Mesoscale and Nanoscale Physics · Physics 2009-06-05 Christos Lampropoulos , Stephen O. Hill , George Christou

We consider the single particle relaxation rate of 2D electrons subject to a random magnetic field. The density of states (DOS) oscillations in a uniform magnetic field (in addition to a random one) are studied. We define a gauge invariant…

Condensed Matter · Physics 2007-05-23 E. Altshuler , A. G. Aronov , A. D. Mirlin , P. Woelfle

We calculate the magnetisation relaxation in the short-time regime for an ensemble of nanomagnets in the presence of a low-frequency external AC biasing field, at temperatures lower than the magnetic anisotropy energy of the individual…

Condensed Matter · Physics 2007-05-23 G. Rose , P. C. E. Stamp

We use millimeter wave radiation to manipulate the populations of the energy levels of a single crystal molecular magnet Fe8. When a continuous wave radiation is in resonance with the transitions from the ground state to the first excited…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 M. Bal , Jonathan R. Friedman , Y. Suzuki , K. Mertes , E. M. Rumberger , D. N. Hendrickson , Y. Myasoedov , H. Shtrikman , N. Avraham , E. Zeldov

For the first time, magnetization of high-Tc samples with different crystalline structure and its isothermal relaxation is studied at very weak constant fields (H <= 0.1 Oe) for temperatures close to the critical ones. Essential influence…

Superconductivity · Physics 2009-11-11 V. P. Timofeev , A. N. Omelyanchouk

We study the slow phase of thermally activated magnetic relaxation in finite two-dimensional ensembles of dipolar interacting ferromagnetic nanoparticles whose easy axes of magnetization are perpendicular to the distribution plane. We…

Condensed Matter · Physics 2009-11-10 S. I. Denisov , T. V. Lyutyy , K. N. Trohidou

We report the experimental observation of dielectric relaxation by quantum critical magnons. Complex capacitance measurements reveal a dissipative feature with a temperature-dependent amplitude due to low-energy lattice excitations and an…

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