Related papers: Multiple relaxation times in single-molecule magne…
The integral relaxation time \tau_{int} of thermoactivating noninteracting single-domain ferromagnetic particles is calculated analytically in the geometry with a magnetic field H applied parallel to the easy axis. It is shown that the…
The Mn cluster complexes Mn12(RCOO)16(H2O)4O12 with R=CH3 and 2ClPh (hereafter referred to as Mn12 acetate and Mn12 2-Cl benzoate, respectively) exhibit macroscopic magnetic quantum tunneling. Dynamical magnetic measurements indicate for…
We investigate the magnetization dynamics of a conducting magnetic nanoparticle weakly coupled to source and drain electrodes, under the assumption that all relaxation comes from exchange of electrons with the electrodes. The magnetization…
The magnetic relaxation characteristics are investigated in the two-dimensional ($l^{}_x\times l^{}_y$) assembly of nanoparticles as a function of out-of-plane positional disorder strength $\Delta(\%)$ using numerical simulations. Such…
Well-protected magnetization, tunable quantum states and long coherence time are desired for the use of magnetic molecules in spintronics and quantum information technologies. In this work, endohedral fullerene molecules M@C28 with…
Single-molecule magnets weakly coupled to two ferromagnetic leads act as memory devices in electronic circuits---their response depends on history, not just on the instantaneous applied voltage. We show that magnetic anisotropy introduces a…
The low temperature relaxation of the magnetization in magnetic molecular solids such as Fe$_8$ is studied using Monte Carlo simulations. A set of rate equations is developed to understand the simulations, and the results are compared. The…
Modeling blocking temperature in molecular magnets has been a long standing problem in the field of molecular magnetism. We investigate this problem using a kinetic Monte Carlo (kMC) approach on an assembly of 100,000 short molecular…
Magnetic clusters, i.e., assemblies of a finite number (between two or three and several hundred) of interacting spin centers which are magnetically decoupled from their environment, can be found in many materials ranging from inorganic…
Spin-phonon interaction is known to drive magnetic relaxation in solid-state systems, but little evidence is available on how it affects coherence time. Here we extend fourth-order quantum master equations to account for coherence terms and…
The nonlinear dynamical response of Mn$_{12}$ single-molecule magnets is experimentally found to be very large, quite insensitive to the spin-lattice coupling constant, and displaying peaks reversed with respect to classical…
We study the spin-phonon relaxation rate of both Kramers and non-Kramers molecular magnets in strongly diluted samples at low temperature. Using the "rotational" contribution to the spin-phonon Hamiltonian, universal formulae for the…
The process of magnetic relaxation was studied in bismuth ferrite BiFeO3 multiferroic micro-cubes obtained by means of microwave assisted Pechini process. Two different mechanisms of relaxation were found. The first one is a rapid magnetic…
Can magnetic interactions between single-molecule magnets (SMMs) in a crystal establish long-range magnetic order at low temperatures deep in the quantum regime, where the only electron spin-fluctuations are due to incoherent magnetic…
Multi-spins tunneling cross-relaxations in an ensemble of weakly-coupled Ho$^{3+}$ ions, mediated by weak anisotropic dipolar interactions, can be evidenced by ac-susceptibility measurements in a high temperature regime. Based on a…
Four discrete MnIII/MnII tetra-nuclear complexes with double-cuboidal core were synthesized. dc magnetic measurements show that both Mn2+ - Mn3+ and Mn3+ - Mn3+ magnetic interactions are ferromagnetic in three samples leading to an S = 9…
In a two-qubit system the coupling with an environment affects considerably the entanglement dynamics, and usually leads to the loss of entanglement within a finite time. Since entanglement is a key feature in the application of such…
A phenomenological theory of spin-lattice relaxation of multiple-quantum coherences in systems of two dipolar coupled spins at low temperatures is developed. Intensities of multiple-quantum NMR coherences depending on the spin-lattice…
We have studied the magnetic relaxation properties of the phase-separated manganite compound La0.250Pr0.375Ca0.375MnO3 . A series of polycrystalline samples was prepared with different sintering temperatures, resulting in a continuous…
At temperatures below the magnetic anisotropy energy, monodomain magnetic systems (small particles, nanomagnetic devices, etc.) must relax quantum mechanically. This quantum relaxation must be mediated by the coupling to both nuclear spins…