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The linear energy dispersion of graphene electrons leads to a strongly nonlinear electromagnetic response of this material. We develop a general quantum theory of the third-order nonlinear local dynamic conductivity of graphene…

Mesoscale and Nanoscale Physics · Physics 2016-02-04 S. A. Mikhailov

Third harmonic generation of terahertz radiation is expected to occur in monolayer graphene due to the nonlinear relationship between the crystal momentum and the current density. In this work, we calculate the terahertz nonlinear response…

Applied Physics · Physics 2018-06-22 Parvin Navaeipour , Marc M. Dignam

Optical harmonic generation occurs when high intensity light ($>10^{10}$W/m$^{2}$) interacts with a nonlinear material. Electrical control of the nonlinear optical response enables applications such as gate-tunable switches and frequency…

Nonlinear-optical refraction is typically described by means of perturbation theory near the material's equilibrium state. Graphene, however, can easily move far away from its equilibrium state upon optical pumping, yielding strong…

Optics · Physics 2020-02-14 David Castello-Lurbe , Hugo Thienpont , Nathalie Vermeulen

We present a finite-temperature diagrammatic perturbation theory of third harmonic generation (THG) in doped graphene. We carry out calculations of the third-order conductivity in the scalar potential gauge, highlighting a subtle…

Mesoscale and Nanoscale Physics · Physics 2016-05-04 Habib Rostami , Marco Polini

A quantum theory of the third-harmonic generation in graphene is presented. An analytical formula for the nonlinear conductivity tensor $\sigma^{(3)}_{\alpha\beta\gamma\delta}(\omega,\omega,\omega)$ is derived. Resonant maxima of the third…

Mesoscale and Nanoscale Physics · Physics 2015-06-02 S. A. Mikhailov

We present a nonperturbative quasi-classical theory of graphene photoconductivity. We consider the influence of low-frequency (microwave, terahertz, mid-infrared) radiation on the static conductivity of a uniform graphene layer and…

Mesoscale and Nanoscale Physics · Physics 2021-06-09 S. A. Mikhailov

A non-perturbative model for graphene optical nonlinearity is developed for the study of ultrafast pulse propagation along a monolayer, as in the case of graphene-comprising nanophotonic integrated waveguides. This graphene `hot electron'…

Optics · Physics 2022-03-18 Alexandros Pitilakis , Emmanouil E. Kriezis

We develop a microscopic large-$N$ theory of electron-electron interaction corrections to multi-legged Feynman diagrams describing second- and third-order nonlinear response functions. Our theory, which reduces to the well-known random…

Materials Science · Physics 2017-01-25 Habib Rostami , Mikhail I. Katsnelson , Marco Polini

Graphene as a zero-bandgap two-dimensional semiconductor with a linear electron band dispersion near the Dirac points has the potential to exhibit very interesting nonlinear optical properties. In particular, third harmonic generation of…

Applied Physics · Physics 2018-01-31 Parvin Navaeipour , Ibraheem Al-Naib , Marc M. Dignam

We observe optical third harmonic generation from graphene and few-layer graphite flakes produced by exfoliation. The emission scales with the cube of the intensity of the incident near-infrared femtosecond pulses and has a wavelength that…

Mesoscale and Nanoscale Physics · Physics 2013-03-20 Nardeep Kumar , Jatinder Kumar , Chris Gerstenkorn , Rui Wang , Hsin-Ying Chiu , Arthur L. Smirl , Hui Zhao

We consider the linear and nonlinear response of a weighted graphene sheet under the normal incidence of a plane electromagnetic wave in the form of a quasi-monochromatic pulse of long duration with a sharp edge and harmonic filling. The…

Mesoscale and Nanoscale Physics · Physics 2025-02-28 Michael V. Davidovich

We investigate the effect of phenomenological relaxation parameters on the third order optical nonlinearity of doped graphene by perturbatively solving the semiconductor Bloch equation around the Dirac points. An analytic expression for the…

Materials Science · Physics 2015-12-24 J. L. Cheng , N. Vermeulen , J. E. Sipe

The linear electronic dispersion relation of graphene endows the atomically thin carbon layer with a large intrinsic optical nonlinearity, with regard to both parametric and photothermal processes. While plasmons in graphene nanostructures…

Mesoscale and Nanoscale Physics · Physics 2026-02-05 Line Jelver , Joel D. Cox

We use a quantum-dynamical model to investigate the optical response of graphene under low excitation power. Ultrafast carrier relaxation processes, which play an important role for understanding the optical response of graphene, are…

Mesoscale and Nanoscale Physics · Physics 2011-06-27 Zheshen Zhang , Paul L. Voss

With the help of numerical simulations in microscopic nonlinear quantum theory of coherent electromagnetic radiation interaction with a gapped bilayer graphene, we find out the optimal values of pump wave intensity, graphene temperature,…

Optics · Physics 2020-01-08 A. K. Avetissian , A. G. Ghazaryan , Kh. V. Sedrakian

The nonlinear responses of different materials provide useful mechanisms for optical switching, low noise amplification, and harmonic frequency generation. However, the nonlinear processes usually have an extremely weak nature and require…

Optics · Physics 2017-08-24 Boyuan Jin , Tianjing Guo , Christos Argyropoulos

Intense efforts have been made in recent years to realize nonlinear optical interactions at the single-photon level. Much of this work has focused on achieving strong third-order nonlinearities, such as by using single atoms or other…

Mesoscale and Nanoscale Physics · Physics 2015-08-25 Marco T. Manzoni , Iván Silveiro , F. Javier García de Abajo , Darrick E. Chang

Using perturbation expansion of Maxwell equations, the amplitude equation is derived for nonlinear TM and TE surface plasmon waves supported by graphene. The equation describes interplay between in-plane beam diffraction and nonlinerity due…

Optics · Physics 2013-01-29 A. V. Gorbach

In this work, we present numerical results for the second and third order conductivities of the plain graphene and gapped graphene monolayers associated with the second and third harmonic generation, the optical rectification and the…

Mesoscale and Nanoscale Physics · Physics 2020-02-05 G. B. Ventura , D. J. Passos , J. M. Viana Parente Lopes , J. M. B. Lopes dos Santos
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