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We evaluate the nonlinear coefficient of graphene-on-silicon waveguides through the coincidence measurement of photon-pairs generated via spontaneous four-wave mixing. We observed the temporal correlation of the photon-pairs from the…

Although massless Dirac fermions in graphene constitute a centrosymmetric medium for in-plane excitations, their second-order nonlinear optical response is nonzero if the effects of spatial dispersion are taken into account. Here we present…

Mesoscale and Nanoscale Physics · Physics 2016-12-07 Yongrui Wang , Mikhail Tokman , Alexey Belyanin

The nonlinear magneto-optic responses are investigated for gapped graphene and doped graphene in a perpendicular magnetic field. The electronic states are described by Landau levels, and the electron dynamics in an optical field is obtained…

Materials Science · Physics 2018-03-21 J. L. Cheng , C. Guo

Saturable absorption is a non-perturbative nonlinear optical phenomenon that plays a pivotal role in the generation of ultrafast light pulses. Here we show that this effect emerges in graphene at unprecedentedly low light intensities, thus…

Mesoscale and Nanoscale Physics · Physics 2017-03-15 A. Marini , J. D. Cox , F. J. Garcia de Abajo

We analyze nonlinear optics schemes for generating pairs of quantum entangled plasmons in the terahertz-infrared range in graphene. We predict that high plasmonic field concentration and strong optical nonlinearity of monolayer graphene…

Mesoscale and Nanoscale Physics · Physics 2022-06-17 Zhiyuan Sun , D. N. Basov , M. M. Fogler

Graphene has recently been shown to possess giant nonlinearity; however, the utility of this nonlinearity is limited due to high losses and small interaction volume. We show that by performing waveguide engineering to graphene's…

Mesoscale and Nanoscale Physics · Physics 2014-11-19 Kelvin J. A. Ooi , Lay Kee Ang , Dawn T. H. Tan

We present here a general formulation for the interband dynamical optical conductivity in the nonlinear regime of graphene in the presence of a quantum bath comprising phonons and electrons. Our main focus is the relaxation behavior of the…

Mesoscale and Nanoscale Physics · Physics 2023-07-10 Bristi Ghosh , Sushanta Dattagupta , Malay Bandyopadhyay

Graphene's exceptional nonlinear optical properties combined with resonant photonic structures offer a promising pathway for efficient nonlinear applications at terahertz (THz) frequencies. In this work, we propose and demonstrate a…

Graphene is a promising material for nonlinear THz applications owing to its high third-order susceptibility and tunable optical properties. Its strong nonlinear response, driven by free-carrier thermodynamics, facilitates efficient…

To add the detailed information to the existed knowledge of nonlinear optics field, the nonlinear optical processes of the second and third order have been discussed in their respective susceptibility tensors in the presence of degenerate…

Optics · Physics 2018-01-29 A Srinivasa Rao

Due to its linear dispersion, monolayer graphene is expected to generate a third harmonic response at terahertz frequencies. There have been a variety of different models of this effect and recently it has been experimentally observed.…

Mesoscale and Nanoscale Physics · Physics 2022-04-06 Parvin Navaeipour , Marc M. Dignam

We investigate high-order harmonic generation (HHG) in graphene with a quantum master equation approach. The simulations reproduce the observed enhancement in HHG in graphene under elliptically polarized light [N. Yoshikawa et al, Science…

Materials Science · Physics 2021-02-03 Shunsuke A. Sato , Hideki Hirori , Yasuyuki Sanari , Yoshihiko Kanemitsu , Angel Rubio

We have implemented a generic method, based on the 2n+1 theorem within density functional perturbation theory, to calculate the anharmonic scattering coefficients among three phonons with arbitrary wavevectors. The method is used to study…

Materials Science · Physics 2014-06-24 Lorenzo Paulatto , Francesco Mauri , Michele Lazzeri

This paper is devoted to development of perturbation theory for studying the properties of graphene sheet of finite size, at nonzero temperature and chemical potential. The perturbation theory is based on the tight-binding Hamiltonian and…

Strongly Correlated Electrons · Physics 2015-12-16 N. Yu. Astrakhantsev , V. V. Braguta , M. I. Katsnelson

Nonlinear metasurfaces offer new paradigm for boosting optical effect beyond limitations of conventional materials. In this work, we present an alternative way to produce pronounced third-harmonic generation (THG) based on nonlinear field…

We present a practical scheme to separate the contributions of the electric quadrupole-like and the magnetic dipole-like effects to the forbidden second order optical nonlinear response of graphene, and give analytic expressions for the…

Materials Science · Physics 2017-03-08 J. L. Cheng , N. Vermeulen , J. E. Sipe

High input intensities are usually required to efficiently excite optical nonlinear effects in ultrathin structures. This problem is particularly critical at terahertz (THz) frequencies because high input power THz sources are not…

Optics · Physics 2019-02-27 Tianjing Guo , Boyuan Jin , Christos Argyropoulos

The existence of large nonlinear optical coefficients is one of the preconditions for using nonlinear optical materials in nonlinear optical devices. For a crystal, such large coefficients can be achieved by matching photon energies with…

Materials Science · Physics 2018-12-27 J. L. Cheng , J. E. Sipe , S. W. Wu , Chunlei Guo

We theoretically investigate the effects of Coulomb interaction, at the level of unscreened Hartree-Fock approximation, on third harmonic generation of undoped graphene in an equation of motion framework. The unperturbed electronic states…

Mesoscale and Nanoscale Physics · Physics 2020-01-01 J. L. Cheng , J. E. Sipe , Chunlei Guo

Graphene is known to possess strong optical nonlinearity. Its nonlinear response can be further enhanced by graphene plasmons. Here, we report a novel nonlinear electro-absorption effect observed in nanostructured graphene due to excitation…

Mesoscale and Nanoscale Physics · Physics 2018-02-14 D. Kundys , B. Van Duppen , O. P. Marshall , F. Rodriguez , I. Torre , A. Tomadin , M. Polini , A. N. Grigorenko