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A new mechanism for reactivity of multiply twinned gold nanoparticles resulting from their inherently strained structure provides a further explanation of the surprising catalytic activity of small gold nanoparticles. Atomic defect…

Chemical Physics · Physics 2017-07-26 Michael Walsh , Kenta Yoshida , Akihide Kuwabara , Mungo Pay , Pratibha Gai , Edward Boyes

Chemically synthesized single-crystalline gold microplates have been attracting increasing interests because of their potential as high-quality gold films for nanotechnology. We present the growth of tens of nanometer thick and tens of…

Materials Science · Physics 2016-12-28 Xiaofei Wu , René Kullock , Enno Krauss , Bert Hecht

In this work, we combine electron microscopy measurements of the surface compositions in Cu-Au nanoparticles and atomistic simulations to investigate the effect of gold segregation. While this mechanism has been extensively investigated…

We use molecular dynamics simulations to study the melting of gold icosahedral clusters of a few thousand atoms. We pay particular attention to the behavior of surface atoms, and to the equilibrium shape of the cluster. We find that…

Materials Science · Physics 2009-11-10 Yanting Wang , S. Teitel , Christoph Dellago

Bio-conjugated nanomaterials play a promising role in the development of novel supramolecular structures, molecular machines, and biosensing devices. In this study, lipid-conjugated gold nanoparticles were synthesized and allowed to form a…

Materials Science · Physics 2012-07-24 Subhasish Chatterjee , Markrete Krikorian , Harry D. Gafney , Bonnie Gersten

We present a study showing cooperative behavior of light emitting quantum dots at room temperature, with large increases in radiative decay rates and efficiencies, in the presence of small gold nanoparticles (1.5 - 4 nm radii) in low…

Mesoscale and Nanoscale Physics · Physics 2015-12-24 George J. Vathakkattil , M. Praveena , J. K. Basu , Murugesan Venkatapathi

Crystals in nature often demonstrate curved morphologies rather than classical faceted surfaces. Inspired by biogenic curved single crystals, we demonstrate that gold single crystals exhibiting curved surfaces can be grown with no need of…

Gold nanoparticles are unique electrocatalysts for oxygen reduction, carbon dioxide reduction, and alcohol oxidation. Electrocatalytic processes are influenced by the interaction with the solvent, yet the direct investigation of the…

Colloidal crystals formed by size-asymmetric binary particles co-assemble into a wide variety of colloidal compounds with lattices akin to ionic crystals. Recently, a transition from a compound phase with a sublattice of small particles to…

Soft Condensed Matter · Physics 2023-09-12 Ali Ehlen , Hector Lopez-Rios , Monica Olvera de la Cruz

Understanding and mastering the mechanical properties of metallic nanoparticles is crucial for their use in a wide range of applications. In this context, we use atomic-scale (Molecular Dynamics) and continuous (Finite Elements)…

Materials Science · Physics 2023-03-14 Matteo Erbi , Hakim Amara , Riccardo Gatti

Bulk gold is a good metal, i.e., conductor of electricity and heat, due to its delocalized electron density that can respond to extremely small external perturbations such as electric field or temperature gradient. In energy space, the…

Atomic and Molecular Clusters · Physics 2018-09-13 Sami Malola , Sami Kaappa , Hannu Hakkinen

The coalescence between growing droplets is important for the surface coverage and spatial arrangements of droplets on surfaces. In this work, total internal reflection fluorescence (TIRF) microscopy is utilized to in-situ investigate the…

Soft Condensed Matter · Physics 2018-04-06 Brendan Dyett , Hao Hao , Detlef Lohse , Xuehua Zhang

Aiming at spherical and monodisperse silver nanoparticles with diameters up to 100 nm, the potential of heterogeneous nucleation of silver particles was explored. Gold seed particles, mainly produced with a spark discharge generator, were…

Materials Science · Physics 2014-06-25 Simon Zihlmann , Felix Lüönd , Johanna K. Spiegel

Single crystals in nature often demonstrate fascinating intricate porous morphologies rather than classical faceted surfaces. We attempt to grow such crystals, drawing inspiration from biogenic porous single crystals. Here we show that…

The thermodynamics and kinetics of crystallization of nanoparticles, as opposed to bulk phases, may be influenced by surface and size effects. We investigate the importance of such factors in the crystallization process of gold, silver, and…

Statistical Mechanics · Physics 2024-07-09 Arthur France-Lanord , Sarath Menon , Julien Lam

Understanding the physical and chemical mechanisms occurring during the forming process and operation of an organic resistive memory device is a major issue for better performances. Various mechanisms were suggested in vertically stacked…

The combination of nanodiamonds with plasmonic metal particles is being explored for synergic effects that can enhance biosensing and antibacterial treatments, energy harvesting, photocatalysis, and quantum centres. Here we systematically…

In this work, the structural and magnetic properties of the gold-coated FePt nanoparticles synthesized from high-temperature solution phase are presented. The amount of gold was optimized to obtain most of the FePt particles coated. The…

Materials Science · Physics 2009-11-26 P. de la Presa , M. Multigner , M. P. Morales , T. Rueda , E. Fernandez-Pinel , A. Hernando

Our understanding of the growth of crystals is dominated by the classical description according to which individual atoms or molecules, driven by supersaturation, add to crystal facets. As a result, the growth of hard matter is still mostly…

Chemical Physics · Physics 2020-05-26 Bin Yuan , Ludovico Cademartiri

Monodispersed spherical cadmium sulfide particles were used as a model system in order to explain the size selection in the formation of colloids by aggregation of nanosize subunits. Several procedures of mixing the reactants were employed…

Materials Science · Physics 2010-10-12 Sergiy Libert , Vyacheslav Gorshkov , Vladimir Privman , Dan Goia , Egon Matijevic