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Spin-orbit coupling (SOC) plays a crucial role in magnetic and electronic properties of 5$d$ iridates. In this paper we have experimentally investigated the structural and physical properties of a series of Ir-based double perovskite…

Strongly Correlated Electrons · Physics 2019-10-02 Abhisek Bandyopadhyay , I. Carlomagno , L. Simonelli , M. Moretti Sala , A. Efimenko , C. Meneghini , Sugata Ray

Rare-earth pyrochlores are known to exhibit exotic magnetic phenomena. We report a study of crystal growth and characterizations of a new rare-earth compound Er$_2$AlSbO$_7$, in which Al$^{3+}$ and Sb$^{5+}$ ions share the same positions…

The insulating iron compounds Eu$_2$SrFe$_2$O$_6$ and Sr$_3$Fe$_2$O$_4$Cl$_2$ have high-temperature antiferromagnetic (AF) order despite their different layered structures. Here we carry out density functional calculations and Monte Carlo…

Strongly Correlated Electrons · Physics 2022-08-18 Di Lu , Ke Yang , Lu Liu , Guangyu Wang , Hua Wu

It turns out that the ground states of some systems are symmetry-broken states in which some property is not symmetrically distributed. In the case of strongly correlated electron systems, that were studied by the DFT+U method, researchers…

Materials Science · Physics 2024-04-29 Mahmoud Payami

Elastic and inelastic neutron scattering were used to study the ordered phase of the quasi-one-dimensional spin-1/2 antiferromagnet ${\rm BaCu_{2}Si_{2}O_{7}}$. The previously proposed model for the low-temperature magnetic structure was…

Strongly Correlated Electrons · Physics 2016-08-15 M. Kenzelmann , A. Zheludev , S. Raymond , E. Ressouche , T. Masuda , P. Böni , K. Kakurai , I. Tsukada , K. Uchinokura , R. Coldea

We theoretically study the magnetic properties of pyrochlore iridate bilayer and trilayer thin films grown along the $[111]$ direction using a strong coupling approach. We find the ground state magnetic configurations on a mean field level…

Strongly Correlated Electrons · Physics 2018-09-19 Pontus Laurell , Gregory A. Fiete

The recent discoveries of proximate quantum spin-liquid compounds and their potential application in quantum computing informs the search for new candidate materials for quantum spin-ice and spin-liquid physics. While the majority of such…

Strongly Correlated Electrons · Physics 2019-01-16 K. M. Taddei , L. Sanjeewa , J. W. Kolis , A. S. Sefat , C. de la Cruz , D. M. Pajerowski

Weyl semimetals are three dimensional analogs of graphene where the energy of the excitations are a linear function of their momentum. Pyrochlore Iridates $(A_{2}Ir_{2}O_{7})$ with A =yttrium or lanthanide element) are conjectured to be…

Strongly Correlated Electrons · Physics 2015-05-30 Vivek Aji

We formulate a superexchange theory of insulating double-perovskite compounds such as Sr$_2$FeWO$_6$. An effective spin-orbital Hamiltonian is derived in the strong coupling limit of Hubbard model for d-electrons on Fe and W ions. The…

Strongly Correlated Electrons · Physics 2009-11-10 S. Di Matteo , G. Jackeli , N. B. Perkins

The electronic and magnetic properties of monoclinic double perovskite Sr$_2$CeIrO$_6$ were examined based on both experiments and first-principles density functional theory calculations. From the calculations we conclude that…

Materials Science · Physics 2016-07-13 Sudipta Kanungo , Kailash Mogare , Binghai Yan , Claudia Felser , Martin Jansen

Geometrically frustrated magnetic systems, such as those based on the Shastry-Sutherland lattice (SSL), offer a rich playground for exploring unconventional magnetic states. The delicate balance between competing interactions in these…

We document the coexistence of ferro- and anti-ferromagnetism in pyrochlore $\rm Yb_2Ti_2O_7$ using three neutron scattering techniques on stoichiometric crystals: elastic neutron scattering shows a canted ferromagnetic ground state,…

Strongly Correlated Electrons · Physics 2020-10-27 A. Scheie , J. Kindervater , S. Zhang , H. J. Changlani , G. Sala , G. Ehlers , A. Heinemann , G. S. Tucker , S. M. Koohpayeh , C. Broholm

We have studied the magnetic excitations of electron-doped Sr$_{2-x}$La$_x$IrO$_4$ ($0 \leq x \leq 0.10$) using resonant inelastic x-ray scattering (RIXS) at the Ir L$_3$-edge. The long range magnetic order is rapidly lost with increasing…

The novel electronic state of the canted antiferromagnetic (AFM) insulator, strontium iridate (Sr2IrO4) has been well described by the spin-orbit-entangled isospin Jeff = 1/2, but the role of isospin in transport phenomena remains poorly…

Strongly Correlated Electrons · Physics 2019-05-03 Nara Lee , Eunjung Ko , Hwan Young Choi , Yun Jeong Hong , Muhammad Nauman , Woun Kang , Hyoung Joon Choi , Young Jai Choi , Younjung Jo

We investigated the piezomagnetic effect in pyrochlore-type oxides Y$_2$Ir$_2$O$_7$ and Cd$_2$Os$_2$O$_7$, which show a non-coplanar magnetic structure called the all-in/all-out antiferromagnetic order at low temperatures. The…

Strongly Correlated Electrons · Physics 2025-05-19 Hiroki Nanjo , Yoshinori Imai , Takuya Aoyama , Junichi Yamaura , Kenya Ohgushi

We study the stability of the antiferromagnetic all-in--all-out state observed in dipolar-octupolar pyrochlores that have neodymium as the magnetic species. Different types of disorder are considered, either affecting the immediate…

Electronic and magnetic properties of molybdenum pyrochlores A2Mo2O7 are studied by the fully relativistic density-functional theory plus on-site repulsion (U) method, with focusing on the spin-glass insulating material Y2Mo2O7. We find…

Strongly Correlated Electrons · Physics 2013-11-27 Hiroshi Shinaoka , Yukitoshi Motome , Takashi Miyake , Shoji Ishibashi

We report detailed measurements of the low temperature magnetic phase diagram of Er$_2$Ti$_2$O$_7$. Heat capacity and time-of-flight neutron scattering studies of single crystals, subject to magnetic fields applied along the…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , J. P. Clancy , A. Bourque , M. A. White , M. Ramazanoglu , J. S. Gardner , Y. Qiu , J. R. D. Copley , H. A. Dabkowska , B. D. Gaulin

We study the band structure topology and engineering from the interplay between local moments and itinerant electrons in the context of pyrochlore iridates. For the metallic iridate Pr$_2$Ir$_2$O$_7$, the Ir $5d$ conduction electrons…

Strongly Correlated Electrons · Physics 2018-12-12 Xu Ping Yao , Gang Chen

We have experimentally identified a new magnetic ground state for the kagome lattice, in the perfectly hexagonal Fe2+ (3d6, S = 2) compound Fe4Si2Sn7O16. Representational symmetry analysis of neutron diffraction data shows that below T_N =…

Strongly Correlated Electrons · Physics 2017-11-22 C. D. Ling , M. C. Allison , S. Schmid , M. Adveev , J. S. Gardner , C. -W. Wang , D. H. Ryan , M. Zbiri , T. Soehnel