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We used single-crystal x-ray and neutron diffraction to investigate the crystal and magnetic structures of trigonal lattice iridate Ca2Sr2IrO6. The crystal structure is determined to be $R\bar3$ with two distinct Ir sites. The system…

Strongly Correlated Electrons · Physics 2018-06-14 Jieming Sheng , Feng Ye , Christina Hoffmann , Valentino R. Cooper , Satoshi Okamoto , Jasminka Terzic , Hao Zheng , Hengdi Zhao , G. Cao

The magnetic ground state of double perovskite Sr2DyRuO6 has been investigated using muon spin rotation and relaxation (muSR), neutron powder diffraction (NPD) and inelastic neutron scattering (INS), in addition to heat capacity and…

Strongly Correlated Electrons · Physics 2020-03-19 D. T. Adroja , Shivani Sharma , C. Ritter , A. D. Hillier , C. V. Tomy , R. Singh , R. I. Smith , M. Koza , A. Sundaresan , S. Langridge

The ground-state properties of the spin-1/2 antiferromagnetic Heisenberg model with spatially anisotropic couplings on a square lattice are investigated by a spin-rotation-invariant Green's-function approach and by Lanczos diagonalizations…

Strongly Correlated Electrons · Physics 2007-05-23 D. Ihle , C. Schindelin , A. Weisse , H. Fehske

For iridates with large spatially extended 5d orbitals, it may be anticipated that distant neighbor interactions would play a crucial role in their ground state properties. From this perspective, we investigate the magnetic structure of…

Materials Science · Physics 2019-09-04 Vijeta Singh , J. J. Pulikkotil

The magnetic structure and electronic groundstate of the layered perovskite Ba2IrO4 have been investigated using x-ray resonant magnetic scattering (XRMS). Our results are compared with those for Sr2IrO4, for which we provide supplementary…

Strongly Correlated Electrons · Physics 2013-03-19 S. Boseggia , R. Springell , H. C. Walker , Ch. Rüegg , H. Okabe , M. Isobe , R. S. Perry , S. P. Collins , D. F. McMorrow

A spin-orbital superexchange Hamiltonian in a Mott insulator with $t_{2g}$ orbital degeneracy is investigated. More specifically, we focus on a spin ferromagnetic state of the model and study a collective behavior of orbital angular…

Strongly Correlated Electrons · Physics 2009-11-11 G. Khaliullin , S. Okamoto

Sr2IrO4 is one of the prime candidates for realizing exotic quantum spin orders owing to the subtle combination of spin-orbit coupling and electron correlation. Sensitive local magnetization measurement can serve as a powerful tool to study…

Materials Science · Physics 2025-03-26 Hyeokjun Heo , Jeongha An , Junyoung Kwon , Kwangrae Kim , Youngoh Son , B. J. Kim , Joonho Jang

Spin-crossover compounds, which are characterized by magnetic ions showing low-spin and high-spin states at thermally accessible energies, are ubiquitous in nature. We here focus on the effect of an exchange interaction on the collective…

Statistical Mechanics · Physics 2009-11-13 Carsten Timm , Charles J. Pye

The frustrated pyrochlore antiferromagnet Gd$_{2}$Ti$_{2}$O$_{7}$ has an unusual partially-ordered magnetic structure at the lowest measurable temperatures. This structure is currently believed to involve four magnetic propagation vectors…

The ordered tetragonal intermetallic Cr$_2$Al forms the same structure type as Mn$_2$Au, and the latter has been heavily investigated for its potential in antiferromagnetic spintronics due to its degenerate in-plane N\'{e}el vector. We…

Materials Science · Physics 2022-01-20 Chengxi Zhao , Kisung Kang , Joerg C. Neuefeind , Andre Schleife , Daniel P. Shoemaker

The multiferroic ferrimagnet Cu$_2$OSeO$_3$ with a chiral crystal structure attracted a lot of recent attention due to the emergence of magnetic skyrmion order in this material. Here, the topological properties of its magnon excitations are…

The antiferromagnetic structure of Sr3Ir2O7, the bilayer analogue of a spin-orbital Mott insulator Sr2IrO4, was revealed by resonant magnetic x-ray diffraction. Contrasting intensities of the magnetic diffraction at the Ir LIII and LII…

Strongly Correlated Electrons · Physics 2015-06-05 Shigeki Fujiyama , K. Ohashi , H. Ohsumi , K. Sugimoto , T. Takayama , T. Komesu , M. Takata , T. Arima , H. Takagi

We investigate magnetic excitations in the frustrated zigzag spin-1/2 chain compound $\beta$-TeVO$_4$ by inelastic neutron scattering. In the magnetically ordered ground state, the excitation spectrum exhibits coexisting magnon dispersion,…

Strongly Correlated Electrons · Physics 2018-09-10 M. Pregelj , O. Zaharko , U. Stuhr , A. Zorko , H. Berger , A. Prokofiev , D. Arčon

Pyrochlore iridates have attracted growing attention because of a theoretical prediction of a possible topological semimetal phase originating from all-in-all-out spin ordering. Related to the topological band structure, recent findings of…

Materials Science · Physics 2016-01-14 T. C. Fujita , M. Uchida , Y. Kozuka , S. Ogawa , A. Tsukazaki , T. Arima , M. Kawasaki

A new iridium containing layered cuprate material, IrSr_2Sm_{1.15}Ce_{0.85}Cu_{2.175}O_{10, has been synthesized by conventional ambient-pressure solid-state techniques. The material's structure has been fully characterized by Rietveld…

Materials Science · Physics 2012-09-22 R. H. Colman , A. C. Mclaughlin

The frustrated magnet Bi2Fe4O9 has been reported to exhibit complex spin dynamics coexisting with conventional spin wave excitations. The magnetic Fe3+ (S = 5/2) ions are arranged into a distorted two-dimensional Cairo pentagonal lattice…

Resonant x-ray diffraction experiments were performed for the metallic iridium oxide IrO$_{2}$. We observed anisotropic tensor of susceptibility (ATS) scattering, the spectrum of which shows a sharp contrast between the $L_{3}$ and $L_{2}$…

Strongly Correlated Electrons · Physics 2015-06-12 Yasuyuki Hirata , Kenya Ohgushi , Jun-ichi Yamaura , Hiroyuki Ohsumi , Soshi Takeshita , Masaki Takata , Takahisa Arima

The quantum spin liquid states as a natural ground state of the Kitaev model has led to a quest for new materials candidates hosting Kitaev physics. Yet, there are very few material candidates in this category. Using a combination of $ab$…

Strongly Correlated Electrons · Physics 2023-03-29 Shishir Kumar Pandey , Qiangqiang Gu , Yihao Lin , Rajarshi Tiwari , Ji Feng

The electronic and magnetic properties of spin-1/2 pyrochlores R2V2O7 were investigated on the basis of density-functional calculations. Contrary to the common belief, the spin-1/2 V4+ ions are found to have a substantial easy-axis…

Strongly Correlated Electrons · Physics 2015-05-20 H. J. Xiang , E. J. Kan , M. -H. Whangbo , C. Lee , Su-Huai Wei , X. G. Gong

By many-body quantum-chemical calculations, we investigate the role of two structural effects - local ligand distortions and the anisotropic Cd-ion coordination - on the magnetic state of Cd2Os2O7, a spin S=3/2 pyrochlore. We find that…

Strongly Correlated Electrons · Physics 2013-03-28 Nikolay A. Bogdanov , Rémi Maurice , Ioannis Rousochatzakis , Jeroen van den Brink , Liviu Hozoi
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