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We study theoretically the effects of f-d magnetic exchange interaction in the R$_2$Ir$_2$O$_7$ pyrochlore iridates. The R$^{3+}$ f-electrons form localized magnetic doublets due to the crystal field environment, while the Ir$^{4+}$ d-…

Strongly Correlated Electrons · Physics 2013-01-07 Gang Chen , Michael Hermele

The pyrochlore materials have long been predicted to harbor a quantum spin liquid, an intrinsic long-range-entangled state supporting fractionalized excitations. Existing pyrochlore experiments, on the other hand, have discovered several…

Strongly Correlated Electrons · Physics 2019-08-19 Chunxiao Liu , Gábor B. Halász , Leon Balents

This report presents azimuthal dependent and polarisation dependent x-ray resonant magnetic scattering at the Ir L3 edge for the bilayered iridate compound, Sr3Ir2O7. Two magnetic wave vectors, k1=(1/2,1/2,0) and k2=(1/2,-1/2,0), result in…

Strongly Correlated Electrons · Physics 2012-08-31 S. Boseggia , R Springell , H C Walker , A T Boothroyd , D Prabhakaran , S P Collins , D F McMorrow

We report inelastic neutron scattering studies of magnetic excitations in antiferromagnetically ordered SrFe$_{2}$As$_{2}$ ($T_{N}=220$ K), the parent compound of the FeAs-based superconductors. At low temperatures (T=7 K), the spectrum of…

The entangled charge and spin dynamics in strongly electron correlated system has been a fruitful playground for exploring new physical phenomena. Here with resonant inelastic X-ray scattering we studied the spin dynamics of SrIrO$_3$, a…

Strongly Correlated Electrons · Physics 2026-04-03 Xiang Li , Xiaoting Li , Jiaqi Lin , Peng Dong , Jun Li , Mary H. Upton , Yifan Jiang , Dawei Shen , Haizhong Guo , Xuerong Liu

We point out the emergence of magnetism from the interplay of electron quasi-itinerancy and quantum order by disorder in pyrochlore iridates. Like other Mott insulating iridates, the Ir$^{4+}$ ion in pyrochlore iridates develops an…

Strongly Correlated Electrons · Physics 2020-12-22 Gang Chen , Xiaoqun Wang

Our single crystal study of the magneto-thermal and transport properties of the pyrochlore iridate Eu2Ir2O7 reveals a continuous phase transition from a paramagnetic metal to an antiferromagnetic insulator for a sample with stoichiometry…

Strongly Correlated Electrons · Physics 2015-06-04 Jun J. Ishikawa , Eoin C. T. O'Farrell , Satoru Nakatsuji

Honeycomb iridates such as $\gamma$-Li$_2$IrO$_3$ are argued to realize Kitaev spin-anisotropic magnetic exchange, along with Heisenberg and possibly other couplings. While systems with pure Kitaev interactions are candidates to realize a…

We investigate the properties of the XY pyrochlore antiferromagnet with local <111> planar anisotropy. We find the ground states and show that the configurational ground state entropy is subextensive. By computing the free energy due to…

Statistical Mechanics · Physics 2014-04-11 Pawel Stasiak , Paul A. McClarty , Michel J. P. Gingras

We present a first-principles investigation of the spin-ice state in Dy$_2$Ti$_2$O$_7$ using a magnetic source-free exchange and correlation functional, implemented in the Castep electronic-structure code. By comparing results from the…

Materials Science · Physics 2023-02-20 Z. Hawkhead , N. Gidopoulos , S. J. Blundell , S. J. Clark , T. Lancaster

We investigated Sr$_3$Ru$_2$O$_7$, a quantum critical metal that shows a metamagnetic quantum phase transition and electronic nematicity, through density functional calculations. These predict a ferromagnetic ground state in contrast to the…

Strongly Correlated Electrons · Physics 2020-07-24 A. Putatunda , G. Qin , W. Ren , D. J. Singh

The layered perovskites $R$Cr(BO$_3$)$_2$ ($R$ = Y and Ho) with magnetic triangular lattices were studied by performing ac/dc susceptibility, specific heat, elastic and inelastic neutron scattering, and dielectric constant measurements. The…

Materials Science · Physics 2017-09-13 R. Sinclair , H. D. Zhou , M. Lee , E. S. Choi , G. Li , T. Hong , S. Calder

The spin-orbit coupled double perovskite iridate Ba$_2$YIrO$_6$ with $d^4$ occupancy of Ir is considered as a candidate material for a non-magnetic $J=0$ ground state. The issue of existence of such a state in Ba$_2$YIrO$_6$ however has…

Strongly Correlated Electrons · Physics 2022-12-21 Hermann Schnait , Daniel Bauernfeind , Tanusri Saha-Dasgupta , Markus Aichhorn

We review recent studies of spin dynamics in rare-earth orthorhombic perovskite oxides of the type $RM$O$_3$, where $R$ is a rare-earth ion and $M$ is a transition-metal ion, using single-crystal inelastic neutron scattering (INS). After a…

Strongly Correlated Electrons · Physics 2021-07-28 A. Podlesnyak , S. Nikitin , G. Ehlers

We report experimental signatures of topological transitions among the Weyl semimetal states of pyrochlore Pr2Ir2O7, where the Kondo coupling between the Ir topological electrons and the spin-ice like orders of Pr moments plays a decisive…

Muon spin rotation technique is used to study magnetic ordering in ultra-pure samples of SrCu$_{1-x}$Ni$_x$O$_2$, an archetypical $S=1/2$ antiferromagnetic Heisenberg chain system with a small amount of $S=1$ defects. The ordered state in…

Strongly Correlated Electrons · Physics 2016-06-23 G. Simutis , M. Thede , R. Saint-Martin , A. Mohan , C. Baines , Z. Guguchia , R. Khasanov , C. Hess , A. Revcolevschi , B. Buchner , A. Zheludev

Motivated by recent experiments exploring the spin-orbit-coupled magnetism in $4d$- and $5d$-band transition metal oxides, we study magnetic interactions in Ir- and Rh-based compounds. In these systems, the comparable strength of spin-orbit…

Strongly Correlated Electrons · Physics 2015-06-17 Natalia B. Perkins , Yuriy Sizyuk , Peter Wölfle

The scenario of a metal-insulator transition driven by the onset of antiferromagnetic order in NaOsO$_3$ calls for a trustworthy derivation of the underlying effective spin Hamiltonian. To determine the latter we rely on {\it ab initio}…

We have investigated the structural, electronic, and magnetic properties of the pyrochlore iridates Eu2Ir2O7 and Pr2Ir2O7 using a combination of resonant elastic x-ray scattering, x-ray powder diffraction, and resonant inelastic x-ray…

We study the high-temperature phase diagram of the chiral magnetic insulator Cu$_2$OSeO$_3$ by measuring the spin-Hall magnetoresistance (SMR) in a thin Pt electrode. We find distinct changes in the phase and amplitude of the SMR signal at…

Mesoscale and Nanoscale Physics · Physics 2021-03-24 A. Aqeel , M. Azhar , N. Vlietstra , A. Pozzi , J. Sahliger , H. Huebl , T. T. M. Palstra , C. H. Back , M. Mostovoy