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Continuous quantum phase transitions involving all-in-all-out (AIAO) antiferromagnetic order in strongly spin-orbit-coupled 5d compounds could give rise to various exotic electronic phases and strongly-coupled quantum critical phenomena.…

Strongly Correlated Electrons · Physics 2020-07-01 Yishu Wang , T. F. Rosenbaum , D. Prabhakaran , A. T. Boothroyd , Yejun Feng

Metal-insulator transitions in pyrochlore iridates (A2Ir2O7) are believed to occur due to subtle interplay of spin-orbit coupling, geometric frustration, and electron interactions. In particular, the nature of magnetic ordering of iridium…

Strongly Correlated Electrons · Physics 2014-07-29 Eric Kin-Ho Lee , Subhro Bhattacharjee , Yong Baek Kim

The magnetic properties of the pyrochlore iridate material Eu$_2$Ir$_2$O$_7$ (5$d^5$) have been studied based on the first principle calculations, where the crystal field splitting $\Delta$, spin-orbit coupling (SOC) $\lambda$ and Coulomb…

Strongly Correlated Electrons · Physics 2017-11-08 Yilin Wang , Hongming Weng , Liang Fu , Xi Dai

Rare-earth pyrochlore iridates host two interlocking magnetic sublattices of corner-sharing tetrahedra and can harbour a unique combination of frustrated moments, exotic excitations and highly correlated electrons. They are also the first…

In the pyrochlore iridates, \textit{R}$_{2}$Ir$_{2}$O$_{7}$ (\textit{R} = Lanthanide, Y), determination of the magnetic structure of the iridium moments remains an outstanding problem despite the role this is expected to play in the…

Strongly Correlated Electrons · Physics 2014-06-23 Steven M. Disseler

We report a combined muon spin relaxation/rotation, bulk magnetization, neutron scattering, and transport study of the electronic properties of the pyrochlore iridate Nd2Ir2O7. We observe the onset of strongly hysteretic behavior in the…

We investigate novel topological magnon band crossings of pyrochlore antiferromagnets with all-in-all-out (AIAO) magnetic order. By general symmetry analysis and spin-wave theory, we show that pyrochlore materials with AIAO orders can host…

Strongly Correlated Electrons · Physics 2018-04-03 Shao-Kai Jian , Wenxing Nie

Pyrochlore iridates A2Ir2O7 (A = rare earth elements, Y or Bi) hold great promise for realizing novel electronic and magnetic states owing to the interplay of spin-orbit coupling, electron correlation and geometrical frustration. A…

Strongly Correlated Electrons · Physics 2017-10-04 W. C. Yang , W. K. Zhu , H. D. Zhou , L. Ling , E. S. Choi , M. Lee , Y. Losovyj , Chi-Ken Lu , S. X. Zhang

The pyrochlore material Nd$_2$Zr$_2$O$_7$ with an "all-in-all-out" (AIAO) magnetic order shows novel quantum moment fragmentation with gapped flat dynamical spin ice modes. The parameterized spin Hamiltonian with a dominant frustrated…

Materials Science · Physics 2020-03-11 J. Xu , Owen Benton , A. T. M. N. Islam , T. Guidi , G. Ehlers , B. Lake

The interplay of spin-orbit interactions and electronic correlations dominates the physical properties of pyrochlore iridates, R2Ir2O7 (R = Y, rare earth element), which are typically magnetic insulators. We report an…

Strongly Correlated Electrons · Physics 2015-06-03 T. F. Qi , O. B. Korneta , Xiangang Wan , L. E. DeLong , P. Schlottmann , G. Cao

Semimetallic osmium pyrochlore oxide Cd2Os2O7 undergoes a magnetic transition to an all-in-all-out (AIAO)-type order at 227 K, followed by a crossover to an AIAO insulator at around 210 K. Here, we studied the isostructural and…

Strongly Correlated Electrons · Physics 2022-02-09 Kota Kataoka , Daigorou Hirai , Akihiro Koda , Ryosuke Kadono , Takashi Honda , Zenji Hiroi

Pyrochlore oxides possessing "all-in-all-out" spin ordering have attracted burgeoning interest as a rich ground of emergent states. This ordering has two distinct types of magnetic domains (all-in-all-out or all-out-all-in) with broken…

Materials Science · Physics 2016-03-09 T. C. Fujita , M. Uchida , Y. Kozuka , W. Sano , A. Tsukazaki , T. Arima , M. Kawasaki

We report the observation of magnetic domains in the exotic, antiferromagnetically ordered all-in-all-out state of Nd$_2$Zr$_2$O$_7$, induced by spin canting. The all-in-all-out state can be realized by Ising-like spins on a pyrochlore…

Strongly Correlated Electrons · Physics 2017-05-16 L. Opherden , J. Hornung , T. Herrmannsdörfer , J. Xu , A. T. M. N. Islam , B. Lake , J. Wosnitza

We present results from muon spin relaxation/rotation, magnetization, neutron scattering and transport measurements on polycrystalline samples of the pyrochlore iridates Y2Ir2O7 (Y-227) and Yb2Ir2O7 (Yb-227). Well-defined spontaneous…

Strongly Correlated Electrons · Physics 2012-08-08 S. M. Disseler , Chetan Dhital , A. Amato , S. R. Giblin , Clarina de la Cruz , Stephen D. Wilson , M. J. Graf

A2Ir2O7 iridates were proven to crystallise in the geometrically frustrated pyrochlore structure, which remains stable upon rare-earth cation substitution, temperature variation, and external pressure application. However, the change of…

Strongly Correlated Electrons · Physics 2024-08-05 Daniel Staško , Petr Proschek , Jiří Prchal , Milan Klicpera

Owing to comparably strong spin-orbit coupling and Hubbard interaction, iridium based 227 pyrochlore oxides harbor a rich confluence of competing magnetic orders and emergent multipolar Weyl quasiparticles. Here we show that this family of…

Strongly Correlated Electrons · Physics 2021-06-30 Konstantinos Ladovrechis , Tobias Meng , Bitan Roy

Strong electronic interactions and spin orbit coupling can be conducive for realizing novel broken symmetry phases supporting quasiparticles with nontrivial band topology. 227 pyrochlore iridates provide a suitable material platform for…

Strongly Correlated Electrons · Physics 2017-02-22 Pallab Goswami , Bitan Roy , Sankar Das Sarma

Magnetic-rare-earth pyrochlore iridates exhibit a rich variety of unconventional phases, driven by the complex interactions within and between the rare-earth and the iridium sublattices. In this study, we investigate the peculiar magnetic…

Strongly Correlated Electrons · Physics 2026-01-05 Y. Alexanian , E. Lhotel , J. Robert , S. Petit , E. Lefrançois , P. Lejay , A. Hadj-Azzem , F. Damay , J. Ollivier , B. Fåk , R. Ballou , S. De Brion , V. Simonet

Electrons in the pyrochore iridates experience a large interaction energy in addition to a strong spin-orbit interaction. Both features make the iridates promising for realizing novel states such as the Topological Mott Insulator. The…

Strongly Correlated Electrons · Physics 2017-09-21 Tian Liang , Timothy H. Hsieh , Jun J. Ishikawa , Satoru Nakatsuji , Liang Fu , N. P. Ong

We investigated the electronic and magnetic properties of the pyrochlore oxide Cd$_2$Os$_2$O$_7$ using the density-functional theory plus on-site repulsion ($U$) method, and depict the ground-state phase diagram with respect to $U$. We…

Strongly Correlated Electrons · Physics 2012-06-15 Hiroshi Shinaoka , Takashi Miyake , Shoji Ishibashi
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