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Muon spin rotation and relaxation experiments in the pyrochlore iridate Eu2Ir2O7 yield a well-defined muon spin precession frequency below the metal-insulator/antiferromagnetic transition temperature TM = 120 K, indicative of long-range…

Strongly Correlated Electrons · Physics 2015-03-19 Songrui Zhao. J. M. Mackie , D. E. MacLaughlin , O. O. Bernal , J. J. Ishikawa , Y. Ohta , S. Nakatsuji

A comprehensive set of muon spin spectroscopy and neutron scattering measurements supported by ab-initio and model Hamiltonian simulations have been used to investigate the magnetic ground state of Na$_2$PrO$_3$. $\mu$SR reveals N\'eel…

The magnetic structure of honeycomb iridate Na$_2$IrO$_3$ is of paramount importance to its exotic properties. The magnetic order is established experimentally to be zigzag antiferromagnetic. However, the previous assignment of ordered…

Materials Science · Physics 2015-10-20 Kaige Hu , Fa Wang , Ji Feng

The search for new quantum phases, especially in frustrated magnets, is central to modern condensed matter physics. One of the most promising places to look is in rare-earth pyrochlore magnets with highly-anisotropic exchange interactions,…

Strongly Correlated Electrons · Physics 2017-03-29 Han Yan , Owen Benton , Ludovic D. C. Jaubert , Nic Shannon

Reliable and profound studies of actual magnetic domain structure in rare-earth A2Ir2O7 pyrochlore iridates are frequently limited by insufficient sample quality or lack of single crystals. We report the magnetic properties of the…

Magnetism of ruthernium pyrochlore oxides A2Ru2O7 (A = Hg, Cd, Ca), whose electronic properties within a localized ion picture are characterized by non-degenerate t2g orbitals (Ru5+, 4d3) and thereby subject to geometrical frustration, has…

Strongly Correlated Electrons · Physics 2015-03-17 M. Miyazaki , R. Kadono , K. H. Satoh , M. Hiraishi , S. Takeshita , A. Koda , A. Yamamoto , H. Takagi

We present a general framework for deriving effective spin Hamiltonians of correlated magnetic systems based on a combination of relativistic ab initio density functional theory calculations (DFT), exact diagonalization of a generalized…

Strongly Correlated Electrons · Physics 2016-07-13 Kira Riedl , Daniel Guterding , Harald O. Jeschke , Michel J. P. Gingras , Roser Valenti

Using a Dirac-Heisenberg Hamiltonian with biquadratic exchange interactions, we study the effect of iron disproportionation on the magnetic ordering, and describe the first-order magnetic transition occurring in the perovskite…

Strongly Correlated Electrons · Physics 2009-10-30 H. Kachkachi , P. Kornilovitch , Y. Meurdesoif , J. -C. Grenier , F. Zhou

Type-II multiferroics, in which the magnetic order breaks inversion symmetry, are appealing for both fundamental and applied research due their intrinsic coupling between magnetic and electrical orders. Using first-principles calculations…

Materials Science · Physics 2023-11-20 Urmimala Dey , Mark S. Senn , Nicholas C. Bristowe

We present a muon spin relaxation study on the Ising pyrochlore Nd$_2$Zr$_2$O$_7$ which develops an "all-in-all-out" magnetic order below 0.4~K. At 20~mK far below the ordering transition temperature, the zero-field muon spin relaxation…

Materials Science · Physics 2016-09-07 J. Xu , C. Balz , C. Baines , H. Luetkens , B. Lake

The frustrated pyrochlore magnet Yb$_2$Ti$_2$O$_7$ has the remarkable property that it orders magnetically, but has no propagating magnons over wide regions of the Brillouin zone. Here we use inelastic neutron scattering to follow how the…

Strongly Correlated Electrons · Physics 2017-08-08 J. D. Thompson , P. A. McClarty , D. Prabhakaran , I. Cabrera , T. Guidi , R. Coldea

The magnetic behavior of polycrystalline samples of Er$_2$Ir$_2$O$_7$ and Tb$_2$Ir$_2$O$_7$ pyrochlores is studied by magnetization measurements and neutron diffraction. Both compounds undergo a magnetic transition at 140 and 130 K…

Strongly Correlated Electrons · Physics 2015-07-30 E. Lefrançois , V. Simonet , R. Ballou , E. Lhotel , A. Hadj-Azzem , S. Kodjikian , P. Lejay , P. Manuel , D. Khalyavin , L. C. Chapon

Fully relativistic first-principles electronic structure calculations based on a noncollinear local spin density approximation (LSDA) are performed for pyrochlore iridates Y$_2$Ir$_2$O$_7$ and Pr$_2$Ir$_2$O$_7$. The all-in, all-out…

Strongly Correlated Electrons · Physics 2015-06-22 Fumiyuki Ishii , Yo Pierre Mizuta , Takehiro Kato , Taisuke Ozaki , Hongming Weng , Shigeki Onoda

Muon-spin relaxation results on the pyrochlore iridate Nd$_2$Ir$_2$O$_7$ are reported. Spontaneous coherent muon-spin precession below the metal-insulator transition (MIT) temperature of about 33 K is observed, indicating the appearance of…

Strongly Correlated Electrons · Physics 2013-09-03 Hanjie Guo , Kazuyuki Matsuhira , Ikuto Kawasaki , Makoto Wakeshima , Yukio Hinatsu , Isao Watanabe , Zhu-an Xu

The recent discovery of Spin-ice is a spectacular example of non-coplanar spin arrangements that can arise in the pyrochlore A2B2O7 structure. We present magnetic and thermodynamic studies on the metallic-ferromagnet pyrochlore Sm2Mo2O7.…

Strongly Correlated Electrons · Physics 2009-11-13 Surjeet Singh , R. Suryanarayanan , R. Tackett , G. Lawes , A. K. Sood , P. Berthet , A. Revcolevschi

Neutron inelastic scattering has been used to probe the spin dynamics of the quantum (S=1/2) ferromagnet on the pyrochlore lattice Lu2V2O7. Well-defined spin waves are observed at all energies and wavevectors, allowing us to determine the…

Strongly Correlated Electrons · Physics 2015-06-19 M. Mena , R. S. Perry , T. G. Perring , M. D. Le , S. Guerrero , M. Storni , D. T. Adroja , Ch. Ruegg , D. F. McMorrow

Building a full understanding of the complex magnetism in the rare-earth pyrochlore iridates, A2Ir2O7, is an ongoing issue in condensed matter physics. The possibility of two interpenetrating and interacting frustrated magnetic pyrochlore…

Strongly Correlated Electrons · Physics 2021-01-01 Ross H. Colman , Kristina Vlaskova , Adam Berlie , Milan Klicpera

This article reports a detailed x-ray resonant scattering study of the bilayer iridate compound, Sr3Ir2O7, at the Ir L2 and L3 edges. Resonant scattering at the Ir L3 edge has been used to determine that Sr3Ir2O7 is a long-range ordered…

Strongly Correlated Electrons · Physics 2012-08-31 S. Boseggia , R. Springell , H. C. Walker , A. T. Boothroyd , D. Prabhakaran , D. Wermeille , L. Bouchenoire , S. P. Collins , D. F. McMorrow

The single ion physics of Ho$_2$Ti$_2$O$_7$ is well-understood to produce strong Ising anisotropy, which is an essential ingredient to its low-temperature spin ice state. We present inelastic neutron scattering measurements on…

Strongly Correlated Electrons · Physics 2018-07-25 J. Gaudet , A. M. Hallas , C. R. C. Buhariwalla , G. Sala , M. B. Stone , M. Tachibana , K. Baroudi , R. J. Cava , B. D. Gaulin

Materials that realize Kitaev spin models with bond-dependent anisotropic interactions have long been searched for, as the resulting frustration effects are predicted to stabilize novel forms of magnetic order or quantum spin liquids. Here…

Strongly Correlated Electrons · Physics 2014-11-11 A. Biffin , R. D. Johnson , I. Kimchi , R. Morris , A. Bombardi , J. G. Analytis , A. Vishwanath , R. Coldea