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We show that an array of polar molecules interacting with Rydberg atoms is a promising hybrid system for scalable quantum computation. Quantum information is stored in long-lived hyperfine or rotational states of molecules which interact…

Quantum Physics · Physics 2022-06-07 Chi Zhang , M. R. Tarbutt

We propose a novel type of Rydberg dimer, consisting of a Rydberg-state atom bound to a distant positive ion. The molecule is formed through long-range electric-multipole interaction between the Rydberg atom and the point-like ion. We…

Atomic Physics · Physics 2021-05-14 A. Duspayev , X. Han , M. A. Viray , L. Ma , J. Zhao , G. Raithel

A Rydberg and a ground-state atom can form ultralong range diatomic molecules provided the interaction between the ground-state atom and the Rydberg electron is attractive [C. H. Greene, et al., Phys. Rev. Lett. 85, 2458 (2000)]. A…

Atomic Physics · Physics 2008-07-15 Ivan C. H. Liu , Jovica Stanojevic , Jan M. Rost

We analyze in detail the possibility to use charge-dipole interaction between a single polar molecule or a 1D molecular array and a single Rydberg atom to read out rotational populations. The change in the Rydberg electron energy is…

Quantum Physics · Physics 2016-10-05 Elena Kuznetsova , Seth T. Rittenhouse , H. R. Sadeghpour , Susanne F. Yelin

Divalent atoms have emerged as powerful alternatives to alkalis in ultracold atom platforms, offering unique advantages arising from their two-electron structure. Among these species, ytterbium (Yb) is especially promising, yet its anionic…

Rydberg atoms with dipole-dipole interactions provide intriguing platforms to explore exotic quantum many-body physics. Here we propose a novel scheme with laser-assisted dipole-dipole interactions to realize synthetic magnetic field for…

Mesoscale and Nanoscale Physics · Physics 2022-08-09 Tian-Hua Yang , Bao-Zong Wang , Xin-Chi Zhou , Xiong-Jun Liu

Non-radiative energy transfer between a Rydberg atom and a polar molecule can be controlled by a DC electric field. Here we show how to exploit this control for state-resolved, non-destructive detection and spectroscopy of the molecules…

Atomic Physics · Physics 2023-11-28 Sabrina Patsch , Martin Zeppenfeld , Christiane P. Koch

We demonstrate Rydberg blockade due to the charge-dipole interaction between a single Rb atom and a single RbCs molecule confined in optical tweezers. The molecule is formed by magnetoassociation of a Rb+Cs atom pair and subsequently…

Cold Rydberg atoms exposed to strong magnetic fields possess unique properties which open the pathway for an intriguing many-body dynamics taking place in Rydberg gases consisting of either matter or anti-matter systems. We review both the…

Atomic Physics · Physics 2015-05-14 T. Pohl , H. R. Sadeghpour , P. Schmelcher

Rydberg molecules, often exemplified by long-range "trilobite" molecules, are a subject of much recent interest at high principal quantum number $n$. States that use the same bonding mechanism can exist at much lower $n$ and less-extreme…

Atomic Physics · Physics 2017-05-01 R. A. Carollo , J. L. Carini , E. E. Eyler , P. L. Gould , W. C. Stwalley

Quantum information processing with neutral atoms relies on Rydberg excitation for entanglement generation. While the use of heavy divalent or open-shell elements, such as strontium or ytterbium, has benefits due to their optically active…

We propose a new kind of qubits composed of electric dipolar molecules. The electric dipolar molecules in an external uniform electric field will take simple harmonic oscillations, whose quantum states belonging to the two lowest energy…

Quantum Physics · Physics 2024-02-13 Yong-Yi Huang

We consider dynamics of a Rydberg impurity in a cloud of ultracold bosonic atoms in which the Rydberg electron can undergo spin-changing collisions with surrounding atoms. This system realizes a new type of the quantum impurity problem that…

Quantum Gases · Physics 2019-11-04 Yuto Ashida , Tao Shi , Richard Schmidt , H. R. Sadeghpour , J. Ignacio Cirac , Eugene Demler

Applicability of Rydberg atoms to quantum computers is examined from experimental point of view. In many theoretical proposals appeared recently, excitation of atoms into highly excited Rydberg states was considered as a way to achieve…

Quantum Physics · Physics 2007-05-23 Igor I. Ryabtsev , Denis B. Tretyakov , Ilya I. Beterov

Versatile controllability of interactions in ultracold atomic and molecular gases has now reached an unprecedented era where quantum correlations and unconventional many-body phases can be studied with no corresponding analogs in solid…

Quantum Gases · Physics 2015-05-18 Xiaopeng Li , S. Das Sarma

We propose a novel experimental method to extend the investigation of ion-atom collisions from the so far studied cold, essentially classical regime to the ultracold, quantum regime. Key aspect of this method is the use of Rydberg molecules…

Atomic Physics · Physics 2018-04-18 T. Schmid , C. Veit , N. Zuber , R. Löw , T. Pfau , M. Tarana , M. Tomza

The interaction between a Rydberg electron and a neutral atom situated inside its extended orbit is described via contact interactions for each atom-electron scattering channel. In ultracold environments, these interactions lead to…

Atomic Physics · Physics 2017-05-10 Matthew T Eiles , Chris H Greene

Quantum entanglement is crucial for simulating and understanding exotic physics of strongly correlated many-body systems, such as high--temperature superconductors, or fractional quantum Hall states. The entanglement of non-identical…

Quantum Physics · Physics 2017-10-25 Y. Zeng , P. Xu , X. D. He , Y. Y. Liu , M. Liu , J. Wang , D. J. Papoular , G. V. Shlyapnikov , M. S. Zhan

We observe a series of conical intersections in the potential energy curves governing both the collision between a Rydberg atom and a ground-state atom and the structure of Rydberg molecules. By employing the electronic energy of the…

Atomic Physics · Physics 2021-07-14 Frederic Hummel , Matthew T. Eiles , Peter Schmelcher

Rydberg atoms represent a platform underpinning many recent developments in quantum computation, simulation, sensing, and metrology. They further facilitate optical nonlinearity at the single-photon level when coupled to photons propagating…

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