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A quantum spin liquid is a novel state of matter characterized by quantum entanglement and the absence of any broken symmetry. In condensed matter, the frustrated rare-earth pyrochlore magnets Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$,…

Strongly Correlated Electrons · Physics 2017-04-05 E. Kermarrec , J. Gaudet , K. Fritsch , R. Khasanov , Z. Guguchia , C. Ritter , K. A. Ross , H. A. Dabkowska , B. D. Gaulin

Quantum spin liquids (QSLs) are exotic phases of matter exhibiting long-range entanglement and supporting emergent gauge fields. A vigorous search for experimental realizations of these states has identified several materials with…

Strongly Correlated Electrons · Physics 2018-07-24 Owen Benton

We study the U(1) quantum spin liquid on the pyrochlore spin ice systems. For the non-Kramers doublets such as Pr$^{3+}$ and Tb$^{3+}$, we point out that the inelastic neutron scattering not only detects the low-energy gauge photon, but…

Strongly Correlated Electrons · Physics 2017-11-22 Gang Chen

The pyrochlore materials have long been predicted to harbor a quantum spin liquid, an intrinsic long-range-entangled state supporting fractionalized excitations. Existing pyrochlore experiments, on the other hand, have discovered several…

Strongly Correlated Electrons · Physics 2019-08-19 Chunxiao Liu , Gábor B. Halász , Leon Balents

Pyrochlore materials are characterized by their hallmark network of corner-sharing rare-earth tetrahedra, which can produce a wide array of complex magnetic ground states. Ferromagnetic Ising pyrochlores often obey the "two-in-two-out" spin…

In this paper, we examine the magnetoelectric response of Ising pyrochlores, focusing on both the ordered antiferromagnetic state and the frustrated ferromagnetic case known as "spin-ice". We employ a model which accounts for magnetoelastic…

Strongly Correlated Electrons · Physics 2023-11-28 Tomas Vignau Costa , Santiago Grigera , Rodolfo Borzi

The search for quantum spin liquids (QSL) -- topological magnets with fractionalized excitations -- has been a central theme in condensed matter and materials physics. While theories are no longer in short supply, tracking down materials…

Strongly Correlated Electrons · Physics 2022-05-11 Anish Bhardwaj , Shu Zhang , Han Yan , Roderich Moessner , Andriy H. Nevidomskyy , Hitesh J. Changlani

Frustration in magnetic interactions can give rise to disordered ground states with subtle and beautiful properties. The spin ices Ho2Ti2O7 and Dy2Ti2O7 exemplify this phenomenon, displaying a classical spin liquid state, with…

Strongly Correlated Electrons · Physics 2017-12-11 Mathieu Taillefumier , Owen Benton , Han Yan , L. D. C. Jaubert , Nic Shannon

Actively shought since the turn of the century, two-dimensional quantum spin liquids (QSLs) are exotic phases of matter where magnetic moments remain disordered even at extremely low temperatures. Despite ongoing searches, QSLs remain…

Strongly Correlated Electrons · Physics 2015-07-22 Juan Carrasquilla , Zhihao Hao , Roger G. Melko

Quantum spin ice, modeled for magnetic rare-earth pyrochlores, has attracted great interest for hosting a U(1) quantum spin liquid, which involves spin-ice monopoles as gapped deconfined spinons, as well as gapless excitations analogous to…

Strongly Correlated Electrons · Physics 2017-12-06 Troels Arnfred Bojesen , Shigeki Onoda

Numerous experiments on pyrochlore oxides Pr$_2$(Zr, Sn, Hf, Ir)$_2$O$_7$ with non-Kramers Pr$^{3+}$ ions suggest that they support a quantum spin liquid (QSL) ground state, but the precise nature of the QSL remains unclear. Quantum spin…

Strongly Correlated Electrons · Physics 2025-12-15 Tony An , Félix Desrochers , Yong Baek Kim

An important and continuing theme of modern solid state physics is the realization of exotic excitations in materials (e.g. quasiparticles) that have no analogy (or have not yet been observed) in the actual physical vacuum of free space.…

Strongly Correlated Electrons · Physics 2016-05-04 LiDong Pan , N. J. Laurita , Kate A. Ross , Edwin Kermarrec , Bruce D. Gaulin , N. P. Armitage

At zero temperature, the classical antiferromagnetic Ising model on the pyrochlore lattice is a spin disorder phase of the critical spin correlation. It is a deconfined phase in that the binding energy of the monopole-anti-monopole pair is…

Strongly Correlated Electrons · Physics 2010-08-30 Chyh-Hong Chern , Chen-Nan Liao , Yang-Zhi Chou

We point out the experimental relevance and the detection scheme of symmetry enriched U(1) quantum spin liquids (QSLs) outside the perturbative spin-ice regime. Recent experiments on Ce-based pyrochlore QSL materials suggest that the…

Strongly Correlated Electrons · Physics 2020-03-25 Xu-Ping Yao , Yao Dong Li , Gang Chen

We report low-temperature thermal conductivity $\kappa$ of pyrochlore Yb$_2$Ti$_2$O$_7$, which contains frustrated spin-ice correlations with significant quantum fluctuations. In the disordered spin-liquid regime, $\kappa(H)$ exhibits a…

Strongly Correlated Electrons · Physics 2016-03-24 Y. Tokiwa , T. Yamashita , M. Udagawa , S. Kittaka , T. Sakakibara , D. Terazawa , Y. Shimoyama , T. Terashima , Y. Yasui , T. Shibauchi , Y. Matsuda

Magnetic pyrochlores with non-Kramers rare-earth ions provide a platform for exploring emergent gauge physics and quantum spin-ice behavior, yet the influence of structural disorder on their ground states remains insufficiently understood.…

We report the low temperature magnetic properties of Ce$_2$Sn$_2$O$_7$, a rare-earth pyrochlore. Our susceptibility and magnetization measurements show that due to the thermal isolation of a Kramers doublet ground state, Ce$_2$Sn$_2$O$_7$…

Strongly Correlated Electrons · Physics 2016-08-15 Romain Sibille , Elsa Lhotel , Vladimir Pomjakushin , Chris Baines , Tom Fennell , Michel Kenzelmann

Pyrochlore magnets are candidates for spin-ice behavior. We present theoretical simulations of relevance for the pyrochlore family R2Ti2O7 (R= rare earth) supported by magnetothermal measurements on selected systems. By considering long…

Statistical Mechanics · Physics 2009-10-31 R. Siddharthan , B. S. Shastry , A. P. Ramirez , A. Hayashi , R. J. Cava , S. Rosenkranz

Muon spin rotation and relaxation experiments in the pyrochlore iridate Eu2Ir2O7 yield a well-defined muon spin precession frequency below the metal-insulator/antiferromagnetic transition temperature TM = 120 K, indicative of long-range…

Strongly Correlated Electrons · Physics 2015-03-19 Songrui Zhao. J. M. Mackie , D. E. MacLaughlin , O. O. Bernal , J. J. Ishikawa , Y. Ohta , S. Nakatsuji

Ising models on a pyrochlore oxide lattice are usually associated with spin ice materials and "magnetic monopoles". Ever more often effects connecting magnetic and elastic degrees of freedom are reported on these and other related…

Strongly Correlated Electrons · Physics 2020-12-01 D. Slobinsky , L. Pili , G. Baglietto , S. A. Grigera , R. A. Borzi
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