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We investigate the emergence of quantum spin liquid phases in pyrochlore oxides with non-Kramers ions, in which structural randomness effectively acts as a transverse field, introducing quantum fluctuations on top of the spin ice manifold.…

Strongly Correlated Electrons · Physics 2026-01-09 Marcus V. Marinho , Eric C. Andrade

We present results from muon spin relaxation/rotation, magnetization, neutron scattering and transport measurements on polycrystalline samples of the pyrochlore iridates Y2Ir2O7 (Y-227) and Yb2Ir2O7 (Yb-227). Well-defined spontaneous…

Strongly Correlated Electrons · Physics 2012-08-08 S. M. Disseler , Chetan Dhital , A. Amato , S. R. Giblin , Clarina de la Cruz , Stephen D. Wilson , M. J. Graf

We report that the local Ising anisotropy in pyrochlore oxides - the crucial requirement for realizing the spin-ice state - can be broken by means of high magnetic fields. For the case of the well-established classical spin-ice compound…

Strongly Correlated Electrons · Physics 2019-03-27 L. Opherden , T. Herrmannsdörfer , M. Uhlarz , D. I. Gorbunov , A. Miyata , O. Portugall , I. Ishii , T. Suzuki , H. Kaneko , H. Suzuki , J. Wosnitza

Ice states, in which frustrated interactions lead to a macroscopic ground-state degeneracy, occur in water ice, in problems of frustrated charge order on the pyrochlore lattice, and in the family of rare-earth magnets collectively known as…

Strongly Correlated Electrons · Physics 2015-03-19 Nic Shannon , Olga Sikora , Frank Pollmann , Karlo Penc , Peter Fulde

Frustration in magnetic systems is fertile ground for complex behaviour, including unconventional ground states with emergent symmetries, topological properties, and exotic excitations. A canonical example is the emergence of…

Strongly Correlated Electrons · Physics 2022-03-02 M. J. Pearce , K. Götze , A. Szabó , T. S. Sikkenk , M. R. Lees , A. T. Boothroyd , D. Prabhakaran , C. Castelnovo , P. A. Goddard

The magnetic behavior of polycrystalline samples of Er$_2$Ir$_2$O$_7$ and Tb$_2$Ir$_2$O$_7$ pyrochlores is studied by magnetization measurements and neutron diffraction. Both compounds undergo a magnetic transition at 140 and 130 K…

Strongly Correlated Electrons · Physics 2015-07-30 E. Lefrançois , V. Simonet , R. Ballou , E. Lhotel , A. Hadj-Azzem , S. Kodjikian , P. Lejay , P. Manuel , D. Khalyavin , L. C. Chapon

We report experimental signatures of topological transitions among the Weyl semimetal states of pyrochlore Pr2Ir2O7, where the Kondo coupling between the Ir topological electrons and the spin-ice like orders of Pr moments plays a decisive…

Spin liquids are highly correlated yet disordered states formed by the entanglement of magnetic dipoles$^1$. Theories typically define such states using gauge fields and deconfined quasiparticle excitations that emerge from a simple rule…

Recent experiments on the dipolar-octupolar pyrochlore compound Ce$_2$Zr$_2$O$_7$ indicate that it may realize a three-dimensional quantum spin liquid (QSL). In particular, the analyses of available data suggest that the system is in a…

Strongly Correlated Electrons · Physics 2022-06-30 Félix Desrochers , Li Ern Chern , Yong Baek Kim

Neutron scattering measurements on the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ reveal an unusual crystal field splitting of its lowest $J$=5/2 multiplet, such that its ground state doublet is composed of m$_J$=$\pm$3/2, giving these doublets a…

Multipolar magnetism is an emerging field of quantum materials research. The building blocks of multipolar phenomena are magnetic ions with a non-Kramers doublet, where the orbital and spin degrees of freedom are inextricably intertwined,…

Strongly Correlated Electrons · Physics 2020-07-08 Adarsh S. Patri , Masashi Hosoi , SungBin Lee , Yong Baek Kim

Metal-insulator transitions in pyrochlore iridates (A2Ir2O7) are believed to occur due to subtle interplay of spin-orbit coupling, geometric frustration, and electron interactions. In particular, the nature of magnetic ordering of iridium…

Strongly Correlated Electrons · Physics 2014-07-29 Eric Kin-Ho Lee , Subhro Bhattacharjee , Yong Baek Kim

The competition between fractionalized spin-liquid states and magnetically ordered phases is an important paradigm in frustrated magnetism. Spin-orbit coupled Mott insulators with Ising-like magnetic anisotropies, such as Kitaev materials,…

Strongly Correlated Electrons · Physics 2022-12-08 G. Shankar , Chien-Hung Lin , Joseph Maciejko

Quantum spin liquids (QSLs) represent a novel state where spins are highly entangled but do not order even at zero temperature due to strong quantum fluctuations. Such a state is mostly studied in Heisenberg models defined on geometrically…

The complexity embedded in condensed matter fertilizes the discovery of new states of matter, enriched by ingredients like frustration. Illustrating examples in magnetic systems are Kitaev spin liquids, skyrmions phases, or spin ices. These…

Strongly Correlated Electrons · Physics 2017-02-10 E. Lefrançois , V. Cathelin , E. Lhotel , J. Robert , P. Lejay , C. V. Colin , B. Canals , F. Damay , J. Ollivier , B. Fåk , L. C. Chapon , R. Ballou , V. Simonet

Ho2Ti2O7 and Dy2Ti2O7 spin ices exhibit elementary excitations akin to magnetic monopoles. Here we focus on Tb2Ti2O7 spin liquid, where correlated magnetic moments keep fluctuating down to very low temperatures. Using a monopole picture, we…

Strongly Correlated Electrons · Physics 2015-06-05 A. P. Sazonov , A. Gukasov , I. Mirebeau , P. Bonville

We study an effective spin model derived perturbatively from random transverse-field Ising model on the pyrochlore lattice. The model consists of spin-configurations on the pyrochlore lattice, restricted to the spin-ice subspace, with spins…

Strongly Correlated Electrons · Physics 2020-05-27 Anirudha Menon , Tom Pardini , Rajiv R. P. Singh

We study the ground state and thermodynamic properties of the spin-half XXZ model, with an Ising interaction $J_z$ and a transverse exchange interaction $J_{x}$, on a pyrochlore tube obtained by joining together elementary cubes in a…

Strongly Correlated Electrons · Physics 2022-08-31 Chunhan Feng , Alexander Wietek , E. Miles Stoudenmire , Rajiv R. P. Singh

Physical properties of a pyrohafnate compound Pr2Hf2O7 have been investigated by ac magnetic susceptibility \chi_ ac(T), dc magnetic susceptibility \chi(T), isothermal magnetization M(H) and heat capacity C_p(T) measurements on…

We investigate a variant of spin ice whose degenerate ground states are densely packed monopole configurations. An applied field drives this model through a Z2 confinement transition. This phase change is a variant of the U(1) Kasteleyn…