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Fully relativistic first-principles electronic structure calculations based on a noncollinear local spin density approximation (LSDA) are performed for pyrochlore iridates Y$_2$Ir$_2$O$_7$ and Pr$_2$Ir$_2$O$_7$. The all-in, all-out…

Strongly Correlated Electrons · Physics 2015-06-22 Fumiyuki Ishii , Yo Pierre Mizuta , Takehiro Kato , Taisuke Ozaki , Hongming Weng , Shigeki Onoda

The spin-$\frac{1}{2}$ kagome antiferromagnet is considered an ideal host for a quantum spin liquid ground state. We find that when the bonds of the kagome lattice are modulated with a periodic pattern, new quantum ground states emerge.…

Specific heat, elastic neutron scattering, and muon spin rotation ($\mu$SR) experiments have been carried out on a well-characterized sample of "stuffed" (Pr-rich) Pr$_{2+x}$Ir$_{2-x}$O$_{7-\delta}$. Elastic neutron scattering shows the…

We present a first-principles investigation of the spin-ice state in Dy$_2$Ti$_2$O$_7$ using a magnetic source-free exchange and correlation functional, implemented in the Castep electronic-structure code. By comparing results from the…

Materials Science · Physics 2023-02-20 Z. Hawkhead , N. Gidopoulos , S. J. Blundell , S. J. Clark , T. Lancaster

Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…

We study the phase transition in a face-centered-cubic antiferromagnet with Ising spins as a function of the concentration $p$ of ferromagnetic bonds randomly introduced into the system. Such a model describes the spin-glass phase at strong…

Statistical Mechanics · Physics 2014-03-05 V. Thanh Ngo , D. Tien Hoang , Hung T. Diep , I. A. Campbell

Extensive work on single molecule magnets has identified a fundamental mode of relaxation arising from the nuclear-spin assisted quantum tunnelling of nearly independent and quasi-classical magnetic dipoles. Here we show that nuclear-spin…

Strongly Correlated Electrons · Physics 2019-03-28 C. Paulsen , S. R. Giblin , E. Lhotel , D. Prabhakaran , K. Matsuhira , G. Balakrishnan , S. T. Bramwell

Spin ice materials are the model systems that have a zero-point entropy as \textit{T} $\rightarrow$ 0 K, owing to the frozen disordered states. Here, we chemically alter the well-known spin ice Ho$_{2}$Ti$_{2}$O$_{7}$ by replacing Ti sites…

Strongly Correlated Electrons · Physics 2022-04-20 Sheetal , A. Elghandour , R. Klingeler , C. S. Yadav

We have grown single crystals of PrMgAl$_{11}$O$_{19}$, an ideal triangular-lattice antiferromagnet, and performed magnetic susceptibility, specific heat and thermal conductivity measurements at low temperatures. The main results are as…

Strongly Correlated Electrons · Physics 2024-11-25 N. Li , A. Rutherford , Y. Y. Wang , H. Liang , Q. J. Li , Z. J. Zhang , H. Wang , W. Xie , H. D. Zhou , X. F. Sun

We show using quantum free energy calculation that the quantum phase transition between U(1) quantum spin liquid (QSL) and antiferromagnet (AFM) phases in pyrochlore quantum antiferromagnet (QAFM) is a first order rather than second order.…

Strongly Correlated Electrons · Physics 2014-01-09 Imam Makhfudz

Dy$_{2}$Zr$_{2}$O$_{7}$ a disordered pyrochlore system, exhibits the spin ice freezing under the application of magnetic field. Our studies suggest the stabilization of pyrochlore phase in Dy$_{2-x}$La$_{x}$Zr$_{2}$O$_{7}$ with the…

Strongly Correlated Electrons · Physics 2021-10-12 Sheetal , C. S. Yadav

Pyrochlore magnets of the form $R_2B_2$O$_7$, in which rare-earth ions on the $R$-site form a three-dimensional network of corner-sharing tetrahedra, provide a canonical setting for geometrical frustration. Ho-based pyrochlores host a…

Strongly Correlated Electrons · Physics 2026-04-17 A. A. Aczel , B. R. Ortiz , Y. Luo , G. Pokharel , P. M. Sarte , C. dela Cruz , J. Liu , G. Sala , S. D. Wilson , B. A. Frandsen , J. A. M. Paddison

Spin-liquid and spin-glass states represent two distinct phases of disordered quantum spin systems. These states are, in principle, distinguished by quantum-entangled fluctuations and spin freezing, but identifying each state and…

Strongly Correlated Electrons · Physics 2025-12-09 Shusei Wadashima , Yukitoshi Motome

The magnetic behavior of the Ca3Co2O6 spin chain compound is characterized by a large Ising-like character of its ferromagnetic chains, set on triangular lattice, that are antiferromagnetically coupled. At low temperature, T < 7K, the 3D…

Strongly Correlated Electrons · Physics 2007-05-23 A. Maignan , V. Hardy , S. Hebert , M. Drillon , M. R. Lees , O. Petrenko , D. Mc K. Paul , D. Khomskii

We use the projective symmetry group analysis to classify the quantum spin liquids on the $S=1/2$ pyrochlore magnet with a breathing anisotropy. We find 40 $\mathbb{Z}_2$ spin liquids and 16 $U(1)$ spin liquids that respect the $F\bar{4}3m$…

Strongly Correlated Electrons · Physics 2022-11-17 Li Ern Chern , Yong Baek Kim , Claudio Castelnovo

The recent discovery of Spin-ice is a spectacular example of non-coplanar spin arrangements that can arise in the pyrochlore A2B2O7 structure. We present magnetic and thermodynamic studies on the metallic-ferromagnet pyrochlore Sm2Mo2O7.…

Strongly Correlated Electrons · Physics 2009-11-13 Surjeet Singh , R. Suryanarayanan , R. Tackett , G. Lawes , A. K. Sood , P. Berthet , A. Revcolevschi

Inspired by recent experimental studies of local magnetic moments interacting with a metallic quasicrystal, we study the low-temperature fate of spins placed in two-dimensional tilings. In the diluted local moment limit, we calculate the…

Strongly Correlated Electrons · Physics 2024-10-17 Ronaldo N. Araújo , Carlo C. Bellinati , Eric C. Andrade

We have studied the antiferromagnetic Ising model on the icosahedral bcc lattice, as a model system of 1/1 approximant Tsai-type quasicrystals. We addressed thermal equilibrium properties of this system with Markov-chain Monte Carlo…

Strongly Correlated Electrons · Physics 2026-04-03 Oscar Novat , Ludovic D. C. Jaubert , Masafumi Udagawa

A hidden order that emerges in the frustrated pyrochlore Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ with $T_{\text{c}}=0.53$ K is studied using specific heat, magnetization, and neutron scattering experiments on a high-quality single crystal.…

Strongly Correlated Electrons · Physics 2016-06-22 H. Takatsu , S. Onoda , S. Kittaka , A. Kasahara , Y. Kono , T. Sakakibara , Y. Kato , B. Fåk , J. Ollivier , J. W. Lynn , T. Taniguchi , M. Wakita , H. Kadowaki

Magnetic pyrochlore oxides, including the spin ice materials, have proved to be a rich field for the study of geometrical frustration in 3 dimensions. Recently, a new family of magnetic oxides has been synthesised in which the half of the…

Strongly Correlated Electrons · Physics 2015-12-08 Owen Benton , Nic Shannon
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