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The pyrochlore spin ice compounds Dy2Ti2O7 and Ho2Ti2O7 are well described by classical Ising models down to very low temperatures. Given the empirical success of this description, the question of the importance of quantum effects in these…

Strongly Correlated Electrons · Physics 2015-10-28 Jeffrey G. Rau , Michel J. P. Gingras

Beyond the conventional electron pairing mediated by phonons, high-temperature superconductivity in cuprates is believed to stem from quantum spin liquid (QSL). The unconventional superconductivity by doping a spin liquid/Mott insulator, is…

Using density functional theory and LDA+U method, we investigate magnetic and electronic structure of Y$_{2}$Ir$_{2}$O$_{7}$ and rare-earth based pyrochlore iridates. Our study reveals that the ground state is a non-collinear magnetic…

Materials Science · Physics 2010-03-18 Xiangang Wan , Jinming Dong , Sergey Y. Savrasov

We propose the idea of a spin-lattice liquid, in which spin and lattice degrees of freedom are strongly coupled and remain disordered and fluctuating down to low temperatures. We show that such a state arises naturally from a microscopic…

Strongly Correlated Electrons · Physics 2019-06-12 Andrew Smerald , George Jackeli

In the pyrochlore compounds, Tb$_2$Ti$_2$O$_7$ and Tb$_2$Sn$_2$O$_7$, only the Tb$^{3+}$ ions are magnetic. They exhibit quite abnormal -- and, in view of their chemical similarity, strikingly different -- magnetic behaviour, as probed by…

Strongly Correlated Electrons · Physics 2009-11-11 I. Mirebeau , A. Apetrei , I. N. Goncharenko , R. Moessner

Geometrical frustration among interacting spins combined with strong quantum fluctuations destabilize long-range magnetic order in favour of more exotic states such as spin liquids. By following this guiding principle, a number of spin…

Among the frustrated magnetic materials, spin-ice stands out as a particularly interesting system. Residual entropy, freezing and glassiness, Kasteleyn transitions and fractionalisation of excitations in three dimensions all stem from a…

Iridate oxides on a honeycomb lattice are considered promising candidates for realization of quantum spin liquid states. We investigate the magnetic couplings in a structural model for a honeycomb iridate K$_2$IrO$_3$, with $C_3$ point…

Strongly Correlated Electrons · Physics 2019-10-23 Ravi Yadav , Satoshi Nishimoto , Manuel Richter , Jeroen van den Brink , Rajyavardhan Ray

Tl$_{2}$Mn$_{2}$O$_{7}$ pyrochlores present colossal magnetoresistance (CMR) around the long range ferromagnetic ordering temperature (T$_{C}$). The character of this magnetic phase transition has been determined to be first order, by…

Materials Science · Physics 2009-11-07 P. Velasco , J. Mira , F. Guinea , J. Rivas , M. J. Martinez-Lope , J. A. Alonso , J. L. Martinez

Pyrochlore oxides with chemical formula of A2B2O7 exhibit a diverse range of electronic properties as a representative family of quantum materials. These properties mostly stem from strong electron correlations at the transition metal B…

Strongly Correlated Electrons · Physics 2025-04-25 Yoshinori Tokura , Yukitoshi Motome , Kentaro Ueda

We present a muon spin relaxation study on the Ising pyrochlore Nd$_2$Zr$_2$O$_7$ which develops an "all-in-all-out" magnetic order below 0.4~K. At 20~mK far below the ordering transition temperature, the zero-field muon spin relaxation…

Materials Science · Physics 2016-09-07 J. Xu , C. Balz , C. Baines , H. Luetkens , B. Lake

$\rm{Sr_2CuTe_{0.5}W_{0.5}O_6}$ is a square-lattice magnet with super-exchange between S=1/2 $\rm{Cu^{2+}}$ spins mediated by randomly distributed Te and W ions. Here, using sub-K temperature and 20 $\rm{\mu}$eV energy resolution neutron…

We study classical spin ice under uniaxial strain along the $[111]$ crystallographic axis. Remarkably, such strain preserves the extensive ice degeneracy and the corresponding classical Coulomb phase. The emergent monopole excitations…

Strongly Correlated Electrons · Physics 2024-11-22 Zhongling Lu , Robin Schäfer , Jonathan N. Hallén , Chris R. Laumann

The fundamental principles of electrodynamics allow an electron carrying both electric monopole (charge) and magnetic dipole (spin) but prohibit its magnetic counterpart. Recently it was predicted that the magnetic "monopoles" carrying…

Strongly Correlated Electrons · Physics 2020-03-04 Feng Jin , Changle Liu , Anmin Zhang , Xiaoqun Wang , Gang Chen , Xuefeng Sun , Qingming Zhang

In a recent letter [Phys. Rev. Lett. {\bf 82}, 1012 (1999)] it was found that the Tb$^{3+}$ magnetic moments in the Tb$_2$Ti$_2$O$_7$ pyrochlore lattice of corner-sharing tetrahedra remain in a {\it collective paramagnetic} state down to…

Disordered Systems and Neural Networks · Physics 2009-10-31 M. J. P. Gingras , B. C. den Hertog , M. Faucher , J. S. Gardner , L. J. Chang , B. D. Gaulin , N. P. Raju , J. E. Greedan

We present a model which accounts for the high field magnetisation at very low temperature in two pyrochlore frustrated systems, Er2Ti2O7 and Tb2Ti2O7. The two compounds present very different ground states: Er2Ti2O7, which has a planar…

Strongly Correlated Electrons · Physics 2015-06-15 Pierre Bonville , Sylvain Petit , Isabelle Mirebeau , Julien Robert , Elsa Lhotel , Carley Paulsen

The spin ice materials Ho$_{2}$Ti$_{2}$O$_{7}$ and Dy$_{2}$Ti$_{2}$O$_{7}$ are by now perhaps the best-studied classical frustrated magnets. A crucial step towards the understanding of their low temperature behaviour -- both regarding their…

Strongly Correlated Electrons · Physics 2019-08-14 Bruno Tomasello , Claudio Castelnovo , Roderich Moessner , Jorge Quintanilla

Quantum spin liquids (QSLs) represent a novel state of matter in which quantum fluctuations prevent conventional magnetic order from being established, and the spins remain disordered even at zero temperature. There have been many…

Strongly Correlated Electrons · Physics 2018-10-11 Zhen Ma , Kejing Ran , Jinghui Wang , Song Bao , Zhengwei Cai , Shichao Li , Jinsheng Wen

One main theme in current condensed matter physics is the search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature without static order. However, there is no…

Strongly Correlated Electrons · Physics 2023-01-10 Chengpeng Tu , Dongzhe Dai , Xu Zhang , Chengcheng Zhao , Xiaobo Jin , Bin Gao , Tong Chen , Pengcheng Dai , Shiyan Li

Spin correlations of the frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been investigated by using inelastic neutron scattering on single crystalline samples ($x=-0.007, 0.000,$ and $0.003$), which have the putative…

Strongly Correlated Electrons · Physics 2019-01-08 Hiroaki Kadowaki , Mika Wakita , Björn Fåk , Jacques Ollivier , Seiko Ohira-Kawamura , Kenji Nakajima , Jeffrey W. Lynn