Related papers: Continuous probe of cold complex molecules with in…
We demonstrate the advantages of THz frequency combs for high-resolution spectroscopy. This benefits from wide spectral coverage and the exact knowledge of the frequency position of each comb component. Heterodyne detection combined with a…
Spectral shaping is critical to many fields of science. In astronomy for example, the detection of exoplanets via the Doppler effect hinges on the ability to calibrate a high resolution spectrograph. Laser frequency combs can be used for…
Mid infrared (MIR) photonics is a key region for molecular physics [1]. High-resolution spectroscopy in the 1--10 {\mu}m region, though, has never been fully tackled for the lack of widely-tunable and practical light sources. Indeed, all…
Frequency domain spectroscopy allows an experimenter to establish optical properties of solids in a wide frequency band including the technically challenging 10 THz region, and in other bands enables metrological comparison between…
Chemical imaging provides information about the distribution of chemicals within a target. When combined with structural information about the target, in situ chemical imaging opens the door to applications ranging from tissue…
Raman scattering spectroscopy is widely used as an analytical technique in various fields, but its measurement process tends to be slow due to the low scattering cross-section. In the last decade, various broadband coherent Raman scattering…
We introduce an absorption imaging technique for ultracold gases that suppresses interference fringes and coherence-induced artifacts by reducing the transverse spatial coherence of the imaging light. The method preserves the narrow…
A multiscale QM/classical approach is presented, that is able to model the optical properties of complex nanostructures composed of a molecular system adsorbed on metal nanoparticles. The latter are described by a combined…
Mid-infrared photothermal microscopy is a new chemical imaging technology in which a visible beam senses the photothermal effect induced by a pulsed infrared laser. This technology provides infrared spectroscopic information at sub-micron…
While Rydberg atoms have shown tremendous potential to serve as accurate and sensitive detectors of microwaves and millimeter waves, their response is generally limited to a single narrow frequency band around a chosen microwave transition.…
We demonstrate the use of dual-comb spectroscopy for isotope ratio measurements. We show that the analysis spectral range of a free-running near-infrared dual-comb spectrometer can be extended to the mid-infrared by difference frequency…
Electro-optic frequency combs were employed to rapidly interrogate an optomechanical sensor, demonstrating spectral resolution substantially exceeding that possible with a mode-locked frequency comb. Frequency combs were generated using an…
We present integrated optical spectrophotometry for a sample of 417 nearby galaxies. Our observations consist of spatially integrated, S/N=10-100 spectroscopy between 3600 and 6900 Angstroms at ~8 Angstroms FWHM resolution. In addition, we…
Dual-comb interferometry is a measurement technique that uses two laser frequency combs to retrieve complex spectra in a line-by-line basis. This technique can be implemented with electro-optic frequency combs, offering intrinsic mutual…
We radically simplify coherently averaged dual-comb spectroscopy by introducing a real-time self-correction system: a radio frequency system-on-chip computes each incoming dual-comb interferogram's phase, frequency, and arrival time;…
A high-resolution broad-spectral-bandwidth spectrometer on a chip would create new opportunities for gas-phase molecular fingerprinting, especially in environmental sensing. A resolution high enough to observe transitions at atmospheric…
High-speed measurement confronts the extreme speed limit when the signal becomes comparable to the noise level. In the context of broadband mid-infrared spectroscopy, state-of-the-art ultrafast Fourier-transform infrared spectrometers, in…
Improving spectral acquisition rate of broadband mid-infrared spectroscopy promises further advancements of molecular science and technology. Unlike the pump-probe spectroscopy that requires repeated measurements with different pump-probe…
Femtosecond coherent multidimensional spectroscopy is demonstrated for an ultracold gas. For this, a setup for phase modulation spectroscopy is used to probe the $3^2\mathrm{S}_{1/2} - 2^2\mathrm{P}_{1/2, 3/2}$ transition in an 800…
The abundances of ices in planetary environments have historically been obtained through measurements of near-infrared absorption features (lambda = 1.0-2.5 microns), and near-IR transmission measurements of materials present in the…