Related papers: Femtosecond-laser-pulse characterization and optim…
We present a method for a complete characterization of a femtosecond ultraviolet pulse when a fundamental near-infrared beam is also available. Our approach relies on generation of second harmonic from the pre-characterized fundamental,…
We propose a novel femtosecond stimulated Raman spectroscopy (FSRS) technique that combines entangled photons with interference detection to select matter pathways and enhance the resolution. Following photo excitation by an actinic pump,…
We show how to emulate a conventional pump-probe scheme using a single frequency-chirped ultrashort UV pulse to obtain a time-resolved image of molecular ultrafast dynamics. The chirp introduces a spectral phase in time that encodes the…
Coherent anti-Stokes Raman Spectroscopy (CARS) is a laser-based measurement technique widely applied across many science and engineering disciplines to perform non-intrusive gas diagnostics. CARS is often used to study combustion, where the…
We present super-resolved coherent anti-Stokes Raman scattering (CARS) microscopy by implementing phase-resolved image scanning microscopy (ISM), achieving up to two-fold resolution increase as compared with a conventional CARS microscope.…
Synchronising ultra-short (~fs) and focussed laser pulses is a particularly difficult task, as this timescale lies orders of magnitude below the typical range of fast electronic devices. Here we present an optical technique that allows for…
Arbitrary Detuning ASynchronous OPtical Sampling (ADA-SOPS) is an emerging technique for extending standard pump--probe experiments performed with two femtosecond lasers to multitimescale experiments, which are of great interest for the…
We present a simple scheme to determine the diffusion properties of a thin slab of strongly scattering material by measuring the speckle contrast resulting from the transmission of a femtosecond pulse with controlled bandwidth. In contrast…
The effect of the pulse-shape on pump-probe spectroscopies is examined for the simplest model of noninteracting fermions on an infinite-dimensional hypercubic lattice. The probe-modified density of states follows the time evolution of the…
We present a pump-probe technique for monitoring ultrafast polarizability changes. In particular, we use it to measure the plasma density created at the temporal focus of a self-compressing higher-order pump soliton in gas-filled…
Ultra-high intensity femtosecond lasers at focus are now routinely used for relativistic motion of charged particles with peak intensities over 10^18W/cm^2. Such high-field experiments are very sensitive to the value of the peak intensity.…
We present a microresonator-based system capable of simultaneously producing time-advanced and time-delayed pulses. The effect is based on the combination of a sharp spectral feature with two orthogonally-polarized propagating waveguide…
In Impulsive Stimulated Raman Scattering vibrational oscillations, coherently stimulated by a femtosecond Raman pulse, are real time monitored and read out as intensity modulations in the transmission of a temporally delayed probe pulse.…
The interaction between ultrashort light pulses and non-absorbing materials is dominated by Impulsive Stimulated Raman Scattering (ISRS). The description of ISRS in the context of pump\&probe experiments is based on effective classical…
Temporal pulse characterization methods can often not be applied to UV pulses due to the lack of suitable nonlinear crystals and very low pulse energies. Here, a method is introduced for the characterization of two unknown and independent…
The origin of the coherences in two-dimensional spectroscopy of photosynthetic complexes remains disputed. Recently it has been shown that in the ultrashort-pulse limit, oscillations in a frequency-integrated pump-probe signal correspond…
We describe PSR J1926-0652, a pulsar recently discovered with the Five-hundred-meter Aperture Spherical radio Telescope (FAST). Using sensitive single-pulse detections from FAST and long-term timing observations from the Parkes 64-m radio…
We propose and demonstrate a versatile technique to measure the lifetime of the one-phonon Fock state using two-color pump-probe Raman scattering and spectrally-resolved, time-correlated photon counting. Following pulsed laser excitation,…
"Single-shot" ultrafast spectroscopy based on the frequency encoding of transient absorbance kinetics using chirped probe pulses is analyzed theoretically. FDSS has an advantage over pump-probe spectroscopy in a situation where the "noise"…
We describe novel optical switching schemes operating at femtosecond time scales by employing free carrier (FC) excitation. Such unprecedented switching times are made possible by spatially patterning the density of the excited FCs. In the…