Related papers: Femtosecond-laser-pulse characterization and optim…
Semiconductor lasers offer native bifunctionality enabling coherent light emission and linear photodetection. They can also operate as sensitive two-photon absorption detectors due to the third-order nonlinearity of the heterostructure…
Numerous techniques have been demonstrated for effective generation of orbital angular momentum-carrying radiation, but intracavity generation of continuously tunable pulses in the femtosecond regime remains challenging. Even if such a…
In this work, we demonstrate a discrete dispersion scan scheme using a low number of flat windows to vary the dispersion of laser pulses in discrete steps. Monte Carlo simulations indicate that the pulse duration can be retrieved accurately…
We report our investigation on ultrashort laser pulse optimization using an AI algorithm in a system consisting of a mode-locked oscillator, a spectral phase shaper, and a highly nonlinear amplifier. We analyzed the performance of the pulse…
A two level model of a single molecule undergoing spectral diffusion dynamics and interacting with a sequence of two short laser pulses is investigated. Analytical solution for the probability of n=0,1,2 photon emission events for the…
Stimulated Raman scattering (SRS) microscopy has emerged as a powerful technique for probing the spatiotemporal dynamics of molecular bonds with exceptional sensitivity, resolution, and speed. However, classically, its performance remains…
Arbitrary manipulation of the temporal and spectral properties of X-ray pulses at free-electron lasers (FELs) would revolutionize many experimental applications. At the Linac Coherent Light Source at Stanford National Accelerator…
Real-time optics and spectroscopy simulations ideally provide results at update rates of 120 Hz or more without any noticeable delay between changing input parameters and the calculated results. Such calculations require models of…
We present a novel, straightforward method for spatiotemporal characterization of ultra-short laser pulses. The method employs far-field interferometry and inverse Fourier transform spectroscopy, built on the theoretical basis derived in…
Femtosecond spectroscopy is an important tool for tracking rapid photoinduced processes in a variety of materials. To spatially map the processes in a sample would substantially expand the capabilities of the method. This is, however,…
Split-pulse x-ray photon correlation spectroscopy has been proposed as one of the unique capabilities made possible with the x-ray free electron lasers. It enables characterization of atomic scale structural dynamics that dictates the…
Adaptive methods of laser irradiation of plasmas are proposed consisting of deterministic, `on-off' amplitude modulations in time, and intermittently changing speckle-patterns. These laser pulses consist of a series of picosecond time-scale…
The non-equilibrium ro-vibrational distribution functions of molecules in a plasma can heavily influence the discharge operation and the plasma-chemistry. A convenient method for measuring the distribution function is by means of coherent…
Accurate spatio-temporal and spatio-spectral metrology is critical to the characterization and use of ultra-short, high-power lasers. The emergence of few cycle pulses, with bandwidths of tens or hundreds of nanometers, poses a significant…
We present the characterization of ultrashort laser pulses by using the plasma-induced frequency resolved optical switching (PI-FROSt) technique, implemented in ambient air. This recently developed method allows for a temporal…
Two atoms in an ultracold gas are correlated at short inter-atomic distances due to threshold effects where the potential energy of their interaction dominates the kinetic energy. The correlations manifest themselves in a distinct nodal…
Coherent anti-Stokes Raman scattering (CARS) spectroscopy with time-delayed ultrashort pulses and a single-pixel photodetector has shown great potential for spectroscopic imaging and transient studies in chemistry and biological research.…
This work investigates the utility of femtosecond pulse shaping in increasing the efficiency of Raman excitation of molecules in the strong-field interaction regime. We study experimentally and theoretically the effect of pulse shaping on…
We demonstrate the use of hybrid rotational femtosecond/picosecond (fs/ps) coherent anti-Stokes Raman spectroscopy (HR-CARS) as a technique for temperature measurements in nitrogen gas at high pressures and temperatures. A broadband pulse…
We suggest pump-probe spectroscopy to study pair correlations that determine the many-body dynamics in weakly interacting, dilute ultracold gases. A suitably chosen, short laser pulse depletes the pair density locally, creating a 'hole' in…