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We introduce the rare-earth delafossite compound TlYbSe$_2$ -- extending the search for quantum spin liquids in frustrated triangular lattice magnets. While the DC magnetisation suggests magnetic exchange interactions in the order of…

Strongly Correlated Electrons · Physics 2025-09-16 Bishnu P. Belbase , Arjun Unnikrishnan , Shi Feng , Eun Sang Choi , Johannes Knolle , Arnab Banerjee

Quantum spin liquid (QSL) is a novel state of matter with exotic excitations and was theoretically predicted to be realized most possibly in an S=1/2 kagome antiferromagnet. Experimentally searching for the candidate materials is a big…

Strongly Correlated Electrons · Physics 2014-09-15 Yuesheng Li , Bingying Pan , Shiyan Li , Wei Tong , Langsheng Ling , Zhaorong Yang , Junfeng Wang , Zhongjun Chen , Zhonghua Wu , Qingming Zhang

In this paper, we study the spin excitation properties of the frustrated triangular-lattice antiferromagnet Yb(BaBO$_3$)$_3$ with nuclear magnetic resonance. From the spectral analysis, neither magnetic ordering nor spin freezing is…

Strongly Correlated Electrons · Physics 2020-08-03 K. Y. Zeng , Long Ma , Y. X. Gao , Z. M. Tian , L. S. Ling , Li Pi

$^{1}$H NMR and static susceptibility measurements have been performed in an organic Mott insulator with nearly isotropic triangular lattice, $\kappa$-(BEDT-TTF)$_{2}$Cu$_{2}$(CN)$_{3}$, which is a model system of frustrated quantum spins.…

Strongly Correlated Electrons · Physics 2009-11-10 Y. Shimizu , K. Miyagawa , K. Kanoda , M. Maesato , G. Saito

A three-dimensional system of interacting spins typically develops static long-range order when it is cooled. If the spins are quantum (S = 1/2), however, novel quantum paramagnetic states may appear. The most highly sought state among them…

Strongly Correlated Electrons · Physics 2015-05-13 S. -H. Lee , H. Kikuchi , Y. Qiu , B. Lake , Q. Huang , K. Habicht , K. Kiefer

We study spin liquid in the frustrated diamond lattice antiferromagnet CoAl2O4 by means of single crystal neutron scattering in zero and applied magnetic field. The magnetically ordered phase appearing below TN=8 K remains nonconventional…

Muon spin relaxation experiments have been performed in the pyrochlore iridate Pr_2Ir_2O_7 for temperatures in the range 0.025-250 K. Kubo-Toyabe relaxation functions are observed up to > 200 K, indicating static magnetism over this…

Strongly Correlated Electrons · Physics 2009-11-13 D. E. MacLaughlin , Y. Ohta , Y. Machida , S. Nakatsuji , G. M. Luke , K. Ishida , R. H. Heffner , Lei Shu , O. O. Bernal

Frustration-induced strong quantum fluctuations accompanied by spin-orbit coupling and crystal electric field can give rise to rich and diverse magnetic phenomena associated with unconventional low-energy excitations in rare-earth based…

Strongly Correlated Electrons · Physics 2024-02-13 J. Khatua , S. Bhattacharya , A. M. Strydom , A. Zorko , J. S. Lord , A. Ozarowski , E. Kermarrec , P. Khuntia

Here, we report both ac and dc magnetization, thermodynamic and electric properties of hexagonal Ba$_3$NiIr$_2$O$_9$. The Ni$^{2+}$ (spin-1) forms layered triangular-lattice and interacts antiferromagnetically while Ir$^{5+}$ is believed to…

Strongly Correlated Electrons · Physics 2021-07-14 Shobha Gondh , Manju Mishra Patidar , Kranti Kumar , M. P. Saravanan , V. Ganesan , A. K. Pramanik

In magnetically ordered insulators, elementary quasiparticles manifest as spin waves - collective motions of localized magnetic moments propagating through the lattice - observed via inelastic neutron scattering. In effective spin-1/2…

The quantum spin liquid (QSL) is an exotic phase of magnetic materials where the spins continue to fluctuate without any symmetry breaking down to zero temperature. Among the handful reports of QSL with spin $S\ge$1, examples with magnetic…

Neutron scattering experiments on a polycrystalline sample of the frustrated pyrochlore magnet Tb2Ti2O7, which does not show any magnetic order down to 50 mK, have revealed that it shows condensation behavior below 0.4 K from a thermally…

Disordered Systems and Neural Networks · Physics 2011-12-13 Hiroshi Takatsu , Hiroaki Kadowaki , Taku J. Sato , Jeffrey W. Lynn , Yoshikazu Tabata , Teruo Yamazaki , Kazuyuki Matsuhira

Mott insulators with localized magnetic moments will exhibit a quantum spin liquid (QSL) state when the quantum fluctuations are strong enough to suppress the ordering of the spins. Such an entangled state will give rise to collective…

Strongly Correlated Electrons · Physics 2025-04-17 Haiyang Chen , Fo-Hong Wang , Qiang Gao , Xue-Jian Gao , Zhenhua Chen , Yaobo Huang , Kam Tuen Law , Xiao Yan Xu , Peng Chen

The structure and magnetic properties of rare-earth ions Tm$^{3+}$ kagom\'{e} lattice Tm$_3$Sb$_3$Mg$_2$O$_{14}$ are studied by X-ray diffraction, magnetic susceptibility and muon spin relaxation ($\mu$SR) experiments. The existence of a…

Strongly Correlated Electrons · Physics 2023-10-02 Yanxing Yang , Kaiwen Chen , Zhaofeng Ding , Adrian D. Hillier , Lei Shu

The electron spin resonance (ESR) spectroscopy was employed to investigate the spin dynamics in triangular lattice antiferromagnets CuCr$_{1-x}$Mg$_{x}$O$_2$ with $x =$ 0 and 0.02. All spectra can be well fitted by a single Lorentzian…

Strongly Correlated Electrons · Physics 2012-07-16 Renwen Li , Zhe Qu , Wei Tong , Yuheng Zhang

Experimental quest for the hypothetical "quantum spin liquid" state has recently met a few promising candidate materials including organic salts \kappa-(ET)2Cu2(CN)3 and EtMe3Sb[Pd(dmit)2]2, S=1/2 triangular-lattice Heisenberg…

Strongly Correlated Electrons · Physics 2015-06-17 Ken Watanabe , Hikaru Kawamura , Hiroki Nakano , Toru Sakai

Spin liquids are highly correlated yet disordered states formed by the entanglement of magnetic dipoles$^1$. Theories typically define such states using gauge fields and deconfined quasiparticle excitations that emerge from a simple rule…

Quantum spin liquids are long-range entangled states of matter with emergent gauge fields and fractionalized excitations. While candidate materials, such as the Kitaev honeycomb ruthenate $\alpha$-RuCl$_3$, show magnetic order at low…

Strongly Correlated Electrons · Physics 2019-07-16 I. Rousochatzakis , S. Kourtis , J. Knolle , R. Moessner , N. B. Perkins

We present the temperature dependence of the uniform susceptibility of spin-half quantum antiferromagnets on spatially anisotropic triangular-lattices, using high temperature series expansions. We consider a model with two exchange…

Strongly Correlated Electrons · Physics 2009-11-10 Weihong Zheng , Rajiv R. P. Singh , Ross H. McKenzie , Radu Coldea

One main theme in current condensed matter physics is the search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature without static order. However, there is no…

Strongly Correlated Electrons · Physics 2023-01-10 Chengpeng Tu , Dongzhe Dai , Xu Zhang , Chengcheng Zhao , Xiaobo Jin , Bin Gao , Tong Chen , Pengcheng Dai , Shiyan Li