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We report proximate quantum spin liquid behavior in K$_2$Co$_2$(SO$_4$)$_3$ with the magnetic Co$^{2+}$ ions embedded on a highly frustrated three-dimensional double trillium lattice. Single-crystal and high-resolution synchrotron powder…

Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…

We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Strongly Correlated Electrons · Physics 2007-05-23 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Yoshida , Y. Takano , A. Suslov , Y. Qiu , J. -H. Chung , D. G. Nocera , Y. S. Lee

Currently under active study in condensed matter physics, both theoretically and experimentally, are quantum spin liquid (QSL) states, in which no long-range magnetic ordering appears at low temperatures due to strong quantum fluctuations…

Strongly Correlated Electrons · Physics 2019-07-04 Ruidan Zhong , Shu Guo , Guangyong Xu , Zhijun Xu , Robert J. Cava

In the quest for materials with unconventional quantum phases, the organic triangular-lattice antiferromagnet $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$ has been extensively discussed as a quantum spin liquid (QSL) candidate. Recently, an intriguing…

Strongly Correlated Electrons · Physics 2019-06-13 Kira Riedl , Roser Valenti , Stephen M. Winter

Cs2CuCl4 is known to possess a quantum spin liquid phase with antiferromagnetic interaction below 2.8 K. We report the observation of a new metastable magnetic phase of the triangular frustrated quantum spin system Cs2CuCl4 induced by the…

Strongly Correlated Electrons · Physics 2017-12-18 Hyeong-Jin Kim , C. R. S. Haines , C. Liu , Sae Hwan Chun , Kee Hoon Kim , H. T. Yi , Sang-Wook Cheong , Siddharth S. Saxena

A quantum spin liquid (QSL) is an exotic state in which electron spins are highly entangled, yet keep fluctuating even at zero temperature. Experimental realization of model QSLs has been challenging due to imperfections, such as antisite…

Strongly Correlated Electrons · Physics 2022-10-25 Huanpeng Bu , Malik Ashtar , Toni Shiroka , Helen C. Walker , Zhendong Fu , Jinkui Zhao , Jason S. Gardner , Gang Chen , Zhaoming Tian , Hanjie Guo

Quantum spin liquid (QSL) is a novel state of matter which refuses the conventional spin freezing even at 0 K. Experimentally searching for the structurally perfect candidates is a big challenge in condensed matter physics. Here we report…

Quantum materials exhibiting magnetic frustration are connected to diverse phenomena including high-Tc superconductivity, topological order and quantum spin liquids (QSLs). A QSL is a quantum phase (QP) related to a quantum-entangled…

Strongly Correlated Electrons · Physics 2021-08-03 Samuel Mañas-Valero , Benjamin Huddart , Tom Lancaster , Eugenio Coronado , Francis Pratt

A quantum magnet, LiCuSbO4, with chains of edge-sharing S = 1/2 CuO6 octahedra is reported. While the Curie-Weiss constant is ferromagnetic, \theta = 30 K, no phase transition or spin freezing occurs down to 100 mK. Specific heat indicates…

Strongly Correlated Electrons · Physics 2012-05-04 S. E. Dutton , M. Kumar , M. Mourigal , Z. G. Soos , J. -J. Wen , C. L. Broholm , N. H. Andersen , Q. Huang , M. Zbiri , R. Toft-Petersen , R. J. Cava

Quantum spin liquid represents an intriguing state where electron spins are highly entangled yet spin fluctuation persists even at 0 K. Recently, the hexaaluminates \textit{R}MgAl$_{11}$O$_{19}$ (\textit{R} = rare earth) have been proposed…

Strongly Correlated Electrons · Physics 2025-04-01 Yantao Cao , Akihiro Koda , M. D. Le , V. Pomjakushin , Benqiong Liu , Zhendong Fu , Zhiwei Li , Jinkui Zhao , Zhaoming Tian , Hanjie Guo

The emergence of a quantum spin liquid (QSL), a state of matter that can result when electron spins are highly correlated but do not become ordered, has been the subject of a considerable body of research in condensed matter physics. Spin…

A quantum spin liquid (QSL) is an exotic state of matter characterized by quantum entanglement and the absence of any broken symmetry. A long-standing open problem, which is a key for fundamental understanding the mysterious QSL states, is…

A quantum spin liquid (QSL) is an exotic state of matter in which electrons' spins are quantum entangled over long distances, but do not show symmetry-breaking magnetic order in the zero-temperature limit. The observation of QSL states is a…

Strongly Correlated Electrons · Physics 2017-03-08 J. A. M. Paddison , M. Daum , Z. L. Dun , G. Ehlers , Y. Liu , M. B. Stone , H. D. Zhou , M. Mourigal

PbCuTe2O6 is a rare example of a spin liquid candidate featuring a three dimensional magnetic lattice. Strong geometric frustration arises from the dominant antiferromagnetic interaction which generates a hyperkagome network of Cu2+ ions…

Strongly Correlated Electrons · Physics 2016-03-14 P. Khuntia , F. Bert , P. Mendels , B. Koteswararao , A. V. Mahajan , M. Baenitz , F. C. Chou , C. Baines , A. Amato , Y. Furukawa

We report discovery of a new iridate family K$_x$Ir$_y$O$_2$ with depleted triangular lattice planes made up of edge sharing IrO$_6$ octahedra separated by K planes. Such a material interpolates between the triangular and honeycomb lattices…

Strongly Correlated Electrons · Physics 2019-08-23 Kavita Mehlawat , Yogesh Singh

Antiferromagnetically coupled S=1/2 spins on an isotropic triangular lattice is the paradigm of frustrated quantum magnetism, but structurally ideal realizations are rare. Here we investigate NaYbO$_2$, which hosts an ideal triangular…

We report a comprehensive investigation of the magnetism of the $S$ = 3/2 triangular-lattice antiferromagnet, $\alpha$-CrOOH(D) (delafossites green-grey powder). The nearly Heisenberg antiferromagnetic Hamiltonian ($J_1$ $\sim$ 23.5 K) with…

Strongly Correlated Electrons · Physics 2021-05-04 Jiabin Liu , Benqiong Liu , Long Yuan , Boqiang Li , Lei Xie , Xiping Chen , Hongxia Zhang , Daye Xu , Wei Tong , Jinchen Wang , Yuesheng Li

Competing magnetic interactions, frustration driven quantum fluctuations, and spin correlations offer an ideal route for the experimental realization of emergent quantum phenomena and exotic quasi particle excitations in 3D frustrated…

Strongly Correlated Electrons · Physics 2024-07-09 J. Khatua , Suheon Lee , Gyungbin Ban , Marc Uhlarz , Kwang-Yong Choi , P. Khuntia

On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases…