English

Quantum spin liquid in frustrated one dimensional LiCuSbO4

Strongly Correlated Electrons 2012-05-04 v4

Abstract

A quantum magnet, LiCuSbO4, with chains of edge-sharing S = 1/2 CuO6 octahedra is reported. While the Curie-Weiss constant is ferromagnetic, \theta = 30 K, no phase transition or spin freezing occurs down to 100 mK. Specific heat indicates a distinct high field phase near the 12 T saturation field. Neutron scattering shows incommensurate spin correlations with q = 0.47\pm0.01{\pi}/a and places an upper limit of 70 \mueV on a potential spin gap. Exact diagonalization of easy plane S = 1/2 chains with competing ferro- and antiferromagnetic interactions (J1 = - 75 K, J2 = 34 K) accounts for the T > 2 K data.

Keywords

Cite

@article{arxiv.1109.4061,
  title  = {Quantum spin liquid in frustrated one dimensional LiCuSbO4},
  author = {S. E. Dutton and M. Kumar and M. Mourigal and Z. G. Soos and J. -J. Wen and C. L. Broholm and N. H. Andersen and Q. Huang and M. Zbiri and R. Toft-Petersen and R. J. Cava},
  journal= {arXiv preprint arXiv:1109.4061},
  year   = {2012}
}

Comments

14 pages, 4 figures

R2 v1 2026-06-21T19:07:12.558Z