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We report the results of magnetic susceptibility $\chi$ and $^1$H nuclear magnetic resonance (NMR) measurements on a three-dimensional hyper-honeycomb lattice compound [(C$_2$H$_5$)$_3$NH]$_2$Cu$_2$(C$_2$O$_4$)$_3$ (CCCO). The average value…

Strongly Correlated Electrons · Physics 2022-03-29 Q. -P. Ding , C. Dissanayake , Santanu Pakhira , W. J. Newsome , F. Uribe-Romo , D. C. Johnston , Y. Nakajima , Y. Furukawa

We report the discovery of a novel gapless quantum spin liquid in the S=1 honeycomb system Cu$_3$LiRu$_2$O$_6$ with Ru$^{4+}$ ($4d^4$) where moments remain dynamic down to 50 mK. Heat capacity measurements show no sign of magnetic ordering…

Quantum spin liquids are exotic states of matter which form when strongly frustrated magnetic interactions induce a highly entangled quantum paramagnet far below the energy scale of the magnetic interactions. Three-dimensional cases are…

A layered triangular lattice with spin-1/2 ions is an ideal platform to explore highly entangled exotic states like quantum spin liquid (QSL). Here, we report a systematic in-field neutron scattering study on a perfect two-dimensional…

Strongly Correlated Electrons · Physics 2024-07-18 Tao Xie , Jie Xing , S. E. Nikitin , S. Nishimoto , M. Brando , P. Khanenko , J. Sichelschmidt , L. D. Sanjeewa , Athena S. Sefat , A. Podlesnyak

$^{31}$P nuclear magnetic resonance (NMR) measurements have been carried out to investigate the magnetic properties and spin dynamics of Fe$^{3+}$ ($S$ = 5/2) spins in the two-dimensional triangular lattice (TL) compound…

Strongly Correlated Electrons · Physics 2022-11-23 Devi V. Ambika , Qing-Ping Ding , Sebin J. Sebastian , Ramesh Nath , Yuji Furukawa

Quantum spin liquids (QSL) are novel phases of matter which remain quantum disordered even at the lowest temperature. They are characterized by emergent gauge fields and fractionalized quasiparticles. Here we show that the sub-Kelvin…

Quantum spin liquid (QSL) represents a new class of condensed matter states characterized by the long-range many-body entanglement of topological orders. The most prominent feature of the elusive QSL state is the existence of fractionalized…

The most fascinating feature of certain two-dimensional (2D) gapless quantum spin liquid (QSL) is that their spinon excitations behave like the fermionic carriers of a paramagnetic metal. The spinon Fermi surface is then expected to produce…

Strongly Correlated Electrons · Physics 2020-09-17 N. Li , Q. Huang , X. Y. Yue , W. J. Chu , Q. Chen , E. S. Choi , X. Zhao , H. D. Zhou , X. F. Sun

The Kitaev model on a honeycomb lattice predicts a paradigmatic quantum spin liquid (QSL) exhibiting Majorana Fermion excitations. The insight that Kitaev physics might be realized in practice has stimulated investigations of candidate…

We present a combination of thermodynamic and dynamic experimental signatures of a disorder driven dynamic cooperative paramagnet in a 50% site diluted triangular lattice spin-1/2 system, Y$_2$CuTiO$_6$. Magnetic ordering and spin freezing…

The nature of the magnetic ground state of highly frustrated systems remained puzzling to this day. Here, we have performed multifrequency electron spin resonance (ESR) measurements on a putative quantum spin liquid compound…

Inelastic neutron scattering studies in single crystals of TbInO3 and TbIn0.95Mn0.05O3 with nearly-triangular antiferromagnetic lattice are reported. At low energies, a broad and apparently gapless continuum of magnetic excitations, located…

Strongly Correlated Electrons · Physics 2019-07-10 M. G. Kim , B. Winn , S. Chi , A. T. Savici , J. A. Rodriguez-Rivera , W. C. Chen , X. Xu , Y. Li , J. W. Kim , S. -W. Cheong , V. Kiryukhin

Magnetism of Cu$_2$(OH)$_3$Br single crystals based on a triangular lattice is studied by means of magnetic susceptibility, pulsed-field magnetization, and specific heat measurements. There are two inequivalent Cu$^{2+}$ sites in an…

Strongly Correlated Electrons · Physics 2019-09-04 Z Y Zhao , H L Che , R Chen , J F Wang , X F Sun , Z Z He

We have studied the low temperature a.c. magnetic susceptibility of the diluted spin ice compound Dy(2-x)MxTi2O7, where the magnetic Dy ions on the frustrated pyrochlore lattice have been replaced with non-magnetic ions, M = Y or Lu. We…

Materials Science · Physics 2007-05-23 J. Snyder , B. G. Ueland , Ari Mizel , J. S. Slusky , H. Karunadasa , R. J. Cava , P. Schiffer

A comprehensive $^{31}$P nuclear magnetic resonance (NMR) study, combined with thermodynamic measurements and first-principle band-structure calculations, has been conducted to explore the ground state of the $S = 5/2$ double trillium…

Strongly Correlated Electrons · Physics 2025-12-08 Sebin J. Sebastian , Q. -P. Ding , A. A. Tsirlin , R. Nath , Y. Furukawa

We report magnetic susceptibility, specific heat and muon spin relaxation (muSR) experiments on the triangular antiferromagnet La2Ca2MnO7 which develops a genuine two-dimensional, three-sublattice \sqrt{3} \times \sqrt{3} magnetic order…

Strongly Correlated Electrons · Physics 2015-07-08 P. Dalmas de Réotier , C. Marin , A. Yaouanc , T. Douce , A. Sikora , A. Amato , C. Baines

The subtle interplay between competing degrees of freedom, crystal electric fields, and spin correlations can lead to exotic quantum states in 4f ion-based frustrated triangular lattice antiferromagnets. We present the crystal structure,…

Strongly Correlated Electrons · Physics 2026-03-17 M. Barik , J. Khatua , Suyoung Kim , Eundeok Mun , Suheon Lee , Bassam Hitti , Gerald D. Morris , Kwang-Yong Choi , P. Khuntia

Quantum spin liquids are highly entangled ground states of quantum systems with emergent gauge structure, fractionalized spinon excitations, and other unusual properties. While these features clearly distinguish quantum spin liquids from…

Strongly Correlated Electrons · Physics 2013-06-18 Lucile Savary , Leon Balents

The static and dynamic local spin susceptibility of the organic Mott insulator $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$, a model material of the spin- 1/2 triangular lattice, is studied by $^{13}$C NMR spectroscopy from room temperature down to 20…

Strongly Correlated Electrons · Physics 2007-05-23 Yasuhiro Shimizu , Kazuya Miyagawa , Kazushi Kanoda , Maesato Mitsuhiko , Gunzi Saito

Quantum spin liquids (QSLs) represent an exotic quantum many-body state characterized by the suppression of long-range magnetic order due to strong quantum fluctuations. The kagome spin-1/2 antiferromagnet (AFM) is a prime candidate for…

Strongly Correlated Electrons · Physics 2024-07-24 S. Suetsugu , T. Asaba , S. Ikemori , Y. Sekino , Y. Kasahara , K. Totsuka , B. Li , Y. Zhao , Y. Li , Y. Kohama , Y. Matsuda
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