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We explore possible superconducting states in $t_{2g}$ multi-orbital correlated electron systems with strong spin-orbit coupling (SOC). In order to study such systems in a controlled manner, we employ large-scale dynamical mean-field theory…

Strongly Correlated Electrons · Physics 2014-10-24 Zi Yang Meng , Yong Baek Kim , Hae-Young Kee

Protected by the interplay of on-site Coulomb interactions and spin-orbit coupling, Sr$_2$IrO$_4$ at high pressure is a rare example of a Mott insulator with a paramagnetic ground state. Here, using optical Raman scattering, we measure both…

Strongly Correlated Electrons · Physics 2021-11-29 Xiang Li , S. E. Cooper , A. Krishnadas , A. de la Torre , R. S. Perry , F. Baumberger , D. M. Silevitch , D. Hsieh , T. F. Rosenbaum , Yejun Feng

By combining 5d transition-metal oxides showing pronounced spin-orbit interactions and oxide-based heterostructures, we propose rutile-based IrO2/TiO2 superlattices as promising candidates for unconventional electronic properties. By means…

Strongly Correlated Electrons · Physics 2017-02-16 Xing Ming , Kunihiko Yamauchi , Tamio Oguchi , Silvia Picozzi

Spin-orbit coupling of as large as a half eV for electrons in 5$d$ orbitals often gives rise to the formation of spin-orbital entangled objects, characterized by the effective total angular momentum $J_{eff}$. Of particular interest are the…

A burning question in the emerging field of spin-orbit driven insulating iridates, such as Na2IrO3 and Li2IrO3 is whether the observed insulating state should be classified as a Mott-Hubbard insulator derived from a half-filled relativistic…

Strongly Correlated Electrons · Physics 2014-01-31 I. I. Mazin , S. Manni , K. Foyevtsova , Harald O. Jeschke , P. Gegenwart , Roser Valenti

For 4$d^1$ and 5$d^1$ spin-orbit-coupled electron configurations, the notion of nonmagnetic j=3/2 quartet ground state discussed in classical textbooks is at odds with the observed variety of magnetic properties. Here we throw fresh light…

Strongly Correlated Electrons · Physics 2016-12-16 Lei Xu , Nikolay A. Bogdanov , Andrew Princep , Peter Fulde , Jeroen van den Brink , Liviu Hozoi

Complex oxides with $4d$ and $5d$ transition-metal ions recently emerged as a new paradigm in correlated electron physics, due to the interplay between spin-orbit coupling and electron interactions. For $4d$ and $5d$ ions, the spin-orbit…

Strongly Correlated Electrons · Physics 2021-05-19 Tomohiro Takayama , Jiri Chaloupka , Andrew Smerald , Giniyat Khaliullin , Hidenori Takagi

It has recently been proposed that Na4Ir3O8 is a weak Mott insulator at ambient pressure, supporting a three-dimensional spin liquid phase with a spinon Fermi surface. This proposal is consistent with recent experimental findings that the…

Strongly Correlated Electrons · Physics 2013-05-29 Daniel Podolsky , Yong Baek Kim

Motivated by recent experiments exploring the spin-orbit-coupled magnetism in $4d$- and $5d$-band transition metal oxides, we study magnetic interactions in Ir- and Rh-based compounds. In these systems, the comparable strength of spin-orbit…

Strongly Correlated Electrons · Physics 2015-06-17 Natalia B. Perkins , Yuriy Sizyuk , Peter Wölfle

Through a neutron scattering, charge transport, and magnetization study, the correlated ground state in the bilayer iridium oxide Sr$_3$Ir$_2$O$_7$ is explored. Our combined results resolve scattering consistent with a high temperature…

Novel phases of two dimensional electron systems resulting from new surface or interface modified electronic structures have generated significant interest in material science. We utilize photoemission spectroscopy to show that the…

Sr2IrO4 is an archetypal spin-orbit-coupled Mott insulator with an antiferromagnetic state below 240 K. Here we report results of our study on single crystals of Sr2Ir1-xFexO4 (0<x<0.32) and Sr2Ir1-xCoxO4 (0<x<0.22). Fe doping retains the…

Strongly Correlated Electrons · Physics 2020-12-21 Bing Hu , Hengdi Zhao , Yu Zhang , Pedro Schlottmann , Feng Ye , Gang Cao

Here, we report an investigation of structural, magnetic and electronic properties in Y-doped layered iridate (Sr$_{1-x}$Y$_x$)$_2$IrO$_4$ ($x$ $\leq$ 0.1). The parent Sr$_2$IrO$_4$ is a well-studied spin-orbit coupling (SOC) induced…

Strongly Correlated Electrons · Physics 2021-03-17 Imtiaz Noor Bhatti , A. K. Pramanik

We have systematically investigated substrate-strain effects on the electronic structures of two representative Sr-iridates, a correlated-insulator Sr$_2$IrO$_4$ and a metal SrIrO$_3$. Optical conductivities obtained by the \emph{ab initio}…

Materials Science · Physics 2016-06-07 Bongjae Kim , Beom Hyun Kim , Kyoo Kim , B. I. Min

Sr$_2$IrO$_4$ is an extensively studied spin-orbit coupling induced insulator with antiferromagnetic ground state. The delicate balance between competing energy scales plays crucial role for its low temperature phase, and the route of…

Strongly Correlated Electrons · Physics 2017-10-31 Imtiaz Noor Bhatti , R. S. Dhaka , A. K. Pramanik

In the light of recent interesting experimental work on MgV$_2$O$_4$ we employ the density functional theory to investigate the crucial role played by different interaction parameters in deciding its electronic and magnetic properties. The…

Strongly Correlated Electrons · Physics 2011-09-15 Sudhir K. Pandey

Using ab initio calculations, we have investigated an insulating tetragonally distorted perovskite BaCrO$_3$ with a formal $3d^2$ configuration, the volume of which is apparently substantially enhanced by a strain due to SrTiO$_3$…

Strongly Correlated Electrons · Physics 2014-11-24 Hyo-Sun Jin , Kyo-Hoon Ahn , Myung-Chul Jung , K. -W. Lee

We report the in-plane and out-of-plane heat conductivity of the antiferromagnetic spin-orbit induced Mott insulator Sr$_2$IrO$_4$ with $J_\mathrm{eff} = 1/2$. Our data reveal clear-cut evidence for magnetic heat transport within the…

Strongly Correlated Electrons · Physics 2016-08-23 Frank Steckel , Akiyo Matsumoto , Tomohiro Takayama , Hidenori Tagaki , Bernd Büchner , Christian Hess

Spin-orbit (SO) Mott insulators are regarded as a new paradigm of magnetic materials, whose properties are largely influenced by SO coupling and featured by highly anisotropic bond-dependent exchange interactions between the spin-orbital…

Strongly Correlated Electrons · Physics 2018-11-14 S. A. Nikolaev , I. V. Solovyev , A. N. Ignatenko , V. Yu. Irkhin , S. V. Streltsov

Spin-orbit coupling (SOC) is a fundamental interaction in solids which can induce a broad spectrum of unusual physical properties from topologically non-trivial insulating states to unconventional pairing in superconductors. In iron-based…

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