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Related papers: Rotational cooling of trapped polyatomic molecules

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We report optical trapping of laser-cooled molecules at sufficient density to observe molecule-molecule collisions for the first time in a bulk gas. SrF molecules from a red-detuned magneto-optical trap (MOT) are compressed and cooled in a…

Atomic Physics · Physics 2024-05-09 Varun Jorapur , Thomas K. Langin , Qian Wang , Geoffrey Zheng , David DeMille

We present a study of Sisyphus cooling of molecules: the scattering of a single-photon remove a substantial amount of the molecular kinetic energy and an optical pumping step allow to repeat the process. A review of the produced cold…

Chemical Physics · Physics 2014-04-11 Daniel Comparat

Ultracold atoms at temperatures close to the recoil limit have been achieved by extending Doppler cooling to forbidden transitions. A cloud of ^40Ca atoms has been cooled and trapped to a temperature as low as 6 \mu K by operating a…

Atomic Physics · Physics 2015-11-30 T. Binnewies , G. Wilpers , U. Sterr , F. Riehle , J. Helmcke , T. E. Mehlstäubler , E. M. Rasel , W. Ertmer

We propose an optical pumping scheme to prepare trapped $\mathrm{AlH}^+$ molecules in a pure state, the stretched hyperfine state $\lvert F=\frac{7}{2},\, m_F=\frac{7}{2}\rangle$ of the rovibronic ground manifold $\lvert…

Atomic and Molecular Clusters · Physics 2020-12-02 Panpan Huang , Schuyler Kain , Antonio de Oliveira-Filho , Brian C. Odom

We report on a cycling scheme for Doppler cooling of trapped OH$^+$ ions using transitions between the electronic ground state $X^3\Sigma^-$ and the first excited triplet state $A^3\Pi$. We have identified relevant transitions for photon…

Atomic Physics · Physics 2023-11-20 Niccolò Bigagli , Daniel W. Savin , Sebastian Will

Cryogenic 22-pole ion traps have found many applications in ion-molecule reaction kinetics and in high resolution molecular spectroscopy. For most of these applications it is important to know the translational and internal temperatures of…

Atomic Physics · Physics 2017-02-07 E. S. Endres , G. Egger , S. Lee , O. Lakhmanskaya , M. Simpson , R. Wester

A single neutral atom is trapped in a three-dimensional optical lattice at the center of a high-finesse optical resonator. Using fluorescence imaging and a shiftable standing-wave trap, the atom is deterministically loaded into the maximum…

Atomic Physics · Physics 2013-06-14 Andreas Reiserer , Christian Nölleke , Stephan Ritter , Gerhard Rempe

We present a cold atomic beam source based on a two-dimensional (2D)+ magneto-optical trap (MOT), capable of generating a continuous cold beam of 87Rb atoms with a flux up to 4.3*10^9 atoms/s, a mean velocity of 10.96(2.20) m/s, and a…

Atomic Physics · Physics 2023-12-20 Shengzhe Wang , Zhixin Meng , and Peiqiang Yan , Yuanxing Liu , Yanying Feng

Motivated by the observations of high Faraday rotation measures measured in cooling flow clusters we propose a model relevant to plasmas with comparable thermal and magnetic pressures. Magnetic field reconnection may play a major role in…

Astrophysics · Physics 2009-10-28 Colin Norman , Avery Meiksin

Producing large samples of slow molecules from thermal-velocity ensembles is a formidable challenge. Here we employ a centrifugal force to produce a continuous molecular beam with a high flux at near-zero velocities. We demonstrate…

Chemical Physics · Physics 2018-12-04 S. Chervenkov , X. Wu , J. Bayerl , A. Rohlfes , T. Gantner , M. Zeppenfeld , G. Rempe

We demonstrate sub-Doppler laser cooling and magneto-optical trapping of the rare earth element Holmium. Atoms are loaded from an atomic beam source and captured in six-beam $\sigma_+ - \sigma_-$ molasses using a strong $J=15/2…

Atomic Physics · Physics 2016-07-26 J. Miao , J. Hostetter , G. Stratis , M. Saffman

We investigated the optical cycling effect of the $\mathrm{X}^2\Sigma(v=0,\ N=1^-) - \mathrm{A}^2\Pi_{1/2}(v'=0,\ J'=1/2^+)$ band of MgF molecules, specifically the $\mathrm{P_1/Q_{12}(1)}$ transition, which serves as the main transition in…

Atomic and Molecular Clusters · Physics 2025-07-08 Kikyeong Kwon , Seunghwan Roh , Youngju Cho , Yongwoong Lee , Eunmi Chae

By introducing methyl fluoride (CH$_3$F) as a new gain medium for a quantum cascade laser-pumped molecular laser (QPML), we demonstrate continuous-wave lasing from more than 120 discrete transitions spanning the frequency range 0.25 to 1.3…

We determine trapping conditions for ultracold polar molecules, where pairs of internal states experience identical trapping potentials. Such conditions could ensure that detrimental effects of inevitable inhomogeneities across an ultracold…

Atomic Physics · Physics 2015-06-12 Alexander Petrov , Constantinos Makrides , Svetlana Kotochigova

Cold supersonic beams of molecules can be slowed down using a switched sequence of electrostatic field gradients. The energy to be removed is proportional to the mass of the molecules. Here we report deceleration of YbF, which is 7 times…

We report the full control over the internal states of ultracold $^{23}$Na$^{87}$Rb molecules, including vibrational, rotational and hyperfine degrees of freedom. Starting from a sample of weakly bound Feshbach molecules, we realize the…

Quantum Gases · Physics 2018-03-07 Mingyang Guo , Xin Ye , Junyu He , Goulven Quéméner , Dajun Wang

The methods producing cold molecules from cold atoms tend to leave molecular ensembles with substantial residual internal energy. For instance, Cs2 molecules initially formed via photoassociation of cold Cs atoms are in several vibrational…

The efficiency of cavity sideband cooling of trapped molecules is theoretically investigated for the case where the IR transition between two rovibrational states is used as a cycling transition. The molecules are assumed to be trapped…

Quantum Physics · Physics 2011-11-30 Markus Kowalewski , Giovanna Morigi , Pepijn W. H. Pinkse , Regina de Vivie-Riedle

Control over the quantum states of individual molecules is crucial in the quest to harness their rich internal structure and dipolar interactions for applications in quantum science. In this paper, we develop a toolbox of techniques for the…

Atomic Physics · Physics 2024-08-28 Daniel K. Ruttley , Alexander Guttridge , Tom R. Hepworth , Simon L. Cornish

Laser cooling of large, complex molecules is a long-standing goal, instrumental for enabling new quantum technology and precision measurements. A primary consideration for the feasibility of laser cooling, which determines the efficiency…

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