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Related papers: Rotational cooling of trapped polyatomic molecules

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Ultracold molecules, because of their rich internal structures and interactions, have been proposed as a promising platform for quantum science and precision measurement. Direct laser-cooling promises to be a rapid and efficient way to…

Atomic Physics · Physics 2024-06-18 Yukai Lu , Samuel J. Li , Connor M. Holland , Lawrence W. Cheuk

We demonstrate optical cycling and transverse laser cooling of a beam of fermionic 137BaF molecules. Their high masses and nuclear spins make these molecules sensitive probes for parity violation and properties of the weak interaction.…

Atomic Physics · Physics 2025-07-30 Felix Kogel , Tatsam Garg , Marian Rockenhäuser , Tim Langen

Direct laser cooling and trapping of molecules to temperature below Doppler limit and density exceeding $10^8$ are challenging due to the sub-Doppler heating effects of molecular magneto-optical trap (MOT). In our previous paper [1], we…

Atomic Physics · Physics 2023-05-29 S. Xu , R. Li , Y. Zhai , Y. Xia , M. Siercke , S. Ospelkaus

Only bosonic molecular species have been directly laser cooled to date, primarily due to an abundance of bosonic isotopes in nature and to their simpler hyperfine structure. Fermionic molecules provide new opportunities for ultracold…

Atomic Physics · Physics 2024-08-07 Jinyu Dai , Qi Sun , Benjamin C. Riley , Debayan Mitra , Tanya Zelevinsky

We here report on the realization of an electrodynamic trap, capable of trapping neutral atoms and molecules in both low-field and high-field seeking states. Confinement in three dimensions is achieved by switching between two electric…

Atomic Physics · Physics 2009-11-11 Jacqueline van Veldhoven , Hendrick L. Bethlem , Gerard Meijer

Trapping lithium with a big number in a simplified experimental setup has difficulties and challenges today. In this paper, we experimentally demonstrate the enhancement of \textsuperscript{6}Li trapping efficiency in a three-dimensional…

Atomic Physics · Physics 2017-08-16 Kai Li , Dongfang Zhang , Tianyou Gao , Shi-Guo Peng , Kaijun Jiang

We have realized a scheme for continuous loading of a magnetic trap (MT). ^{52}Cr atoms are continuously captured and cooled in a magneto-optical trap (MOT). Optical pumping to a metastable state decouples atoms from the cooling light. Due…

Quantum Physics · Physics 2009-11-06 J. Stuhler , P. O. Schmidt , S. Hensler , J. Werner , J. Mlynek , T. Pfau

We analyze in detail the possibility to use charge-dipole interaction between a single polar molecule or a 1D molecular array and a single Rydberg atom to read out rotational populations. The change in the Rydberg electron energy is…

Quantum Physics · Physics 2016-10-05 Elena Kuznetsova , Seth T. Rittenhouse , H. R. Sadeghpour , Susanne F. Yelin

A radiofrequency quadrupole ion trap system for use with a multi-reflection time-of-flight mass spectrograph (MRTOF) for short-lived nuclei has been developed. The trap system consists of two different parts, an asymmetric taper trap and a…

Instrumentation and Detectors · Physics 2015-06-17 Y. Ito , P. Schury , M. Wada , S. Naimi , C. Smorra , T. Sonoda , H. Mita , A. Takamine , K. Okada , A. Ozawa , H. Wollnik

Improved optical control of molecular quantum states promises new applications including chemistry in the quantum regime, precision tests of fundamental physics, and quantum information processing. While much work has sought to prepare…

We propose to sympathetically slow and cool polar molecules in a cold, low-density beam using laser-cooled Rydberg atoms. The elastic collision cross sections between molecules and Rydberg atoms are large enough to efficiently thermalize…

Kinetic temperature is a fundamental parameter in molecular clouds. Symmetric top molecules, such as NH$_3$ and CH$_3$CCH, are often used as thermometers. However, at high temperatures, NH$_3$(2,2) can be collisionally excited to…

The rotational and hyperfine spectrum of the $X^1\Sigma^+ \rightarrow B^3\Pi_1$ transition in TlF molecules was measured using laser-induced fluorescence from both a thermal and a cryogenic molecular beam. Rotational and hyperfine constants…

We experimentally and theoretically study the continuous accumulation of cold atoms from a magneto-optical trap (MOT) into a finite depth trap, consisting in a magnetic quadrupole trap dressed by a radiofrequency (RF) field. Chromium atoms…

We demonstrate full quantum state control of two species of single atoms using optical tweezers and assemble the atoms into a molecule. Our demonstration includes 3D ground-state cooling of a single atom (Cs) in an optical tweezer,…

We propose a method for laser cooling and trapping a substantial class of polar molecules, and in particular titanium (II) oxide (TiO). This method uses pulsed electric fields to nonadiabatically remix the ground-state magnetic sublevels of…

Atomic Physics · Physics 2008-12-13 Benjamin K. Stuhl , Brian C. Sawyer , Dajun Wang , Jun Ye

Over the past years, radiofrequency ion traps have become an attractive platform for studying chemical reactions as they enable a high degree of control over ion-molecule dynamics. In this review, we summarize techniques for the trapping…

Chemical Physics · Physics 2025-10-13 Prerna Paliwal , Jutta Toscano , Stefan Willitsch

We show that the precise preparation of a quantum superposition between three rotational states of an ultracold dipolar molecule generates controllable interferences in their two-body scattering dynamics and collisional rate coefficients,…

Quantum Gases · Physics 2024-06-21 Thibault Delarue , Goulven Quéméner

In this paper, we use steady-state measurements to obtain evidence of radiation trapping in an optically thick a cloud of cold rubidium atoms. We investigate the fluorescence properties of our sample, pumped on opened transitions. The…

Atomic Physics · Physics 2015-06-11 Quentin Baudouin , Nicolas Mercadier , Robin Kaiser

Thermodynamics is one of the oldest and well-established branches of physics that sets boundaries to what can possibly be achieved in macroscopic systems. While it started as a purely classical theory, it was realized in the early days of…

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