Related papers: Rotational cooling of trapped polyatomic molecules
We demonstrate the measurement and manipulation of the temperature of cold CO molecules in a microchip environment. Through the use of time-resolved spatial imaging, we are able to observe the phase-space distribution of the molecules, and…
We demonstrate laser cooling and magneto-optical trapping of europium. The atoms are optically pumped to a metastable state and then loaded from an atomic-beam source via conventional Zeeman slowing and magneto-optical trapping techniques…
Ground state cooling and coherent manipulation of ions in an rf-(Paul) trap is the prerequisite for quantum information experiments with trapped ions. With resolved sideband cooling on the optical S1/2 - D5/2 quadrupole transition we have…
Sideband cooling is a popular method for cooling atoms to the ground state of an optical trap. Applying the same method to molecules requires a number of challenges to be overcome. Strong tensor Stark shifts in molecules cause the optical…
We demonstrate cryogenic buffer-gas cooling of gas-phase methyltrioxorhenium (MTO). This molecule is closely related to chiral organometallic molecules where the parity-violating energy differences between enantiomers may be measurable. The…
We investigate rotational state changes in a single collision of diatomic molecular ions, polar or apolar, with an atomic ion. Rotational state changes may occur since the angular degree of freedom of the molecular ions interacts with the…
We report on a scheme to cool and compress trapped clouds of highly magnetic 52Cr atoms. This scheme combines sequences of gray molasses, which freeze the velocity distribution, and free evolutions in the (close to) harmonic trap, which…
Cooling a range of molecules to ultracold temperatures (<1 mK) is a difficult but important challenge in molecular physics and chemistry. Collective cavity cooling of molecules is a promising method that does not rely on molecular energy…
We propose a novel computational strategy to study the glass transition of molecular fluids. Our approach combines the construction of simple yet realistic models with the development of Monte Carlo algorithms to accelerate equilibration…
Laser cooling of translational motion of small molecules is performed by addressing transitions that ensure spontaneous emission cannot cause net rotational excitation. This will not be possible once the rotational splitting becomes…
We demonstrate optical cycling and sub-Doppler laser cooling of a cryogenic buffer-gas beam of calcium monohydride (CaH) molecules. We measure vibrational branching ratios for laser cooling transitions for both excited electronic states A…
Laser cooling and magneto-optical trapping of molecules typically involves multiple transitions driven by several laser frequencies. We analyze how magneto-optical trapping forces depend on the angular momenta, $F_l$ and $F_u$, and the…
We report magneto-optical trapping (MOT) of a polyatomic molecule, calcium monohydroxide (CaOH). The MOT contains $2.0(5)\times 10^4$ CaOH molecules at a peak density of $3.0(8)\times10^{6}$ cm$^{-3}$. CaOH molecules are further sub-Doppler…
We show, both experimentally and theoretically, that sympathetic cooling of $^{87}$Rb atoms in the $|F=2,m_F=2>$ state by evaporatively cooled atoms in the $|F=1,m_F=-1>$ state can be precisely controlled to produce dual or single…
We report radiation pressure slowing of YbF molecules to low velocity. In YbF, laser slowing is hindered by leaks out of the optical cycle attributed to low-lying metastable electronic states arising from inner-shell excitation. We bring…
Sympathetic laser cooling is a key concept in precision spectroscopy and quantum state control of charged particles. Significant challenges arise in the metrologically relevant case where the effective interaction between the particles is…
Over the past decade, tremendous progress has been made to extend the tools of laser cooling and trapping to molecules. Those same tools have recently been applied to polyatomic molecules (molecules containing three or more atoms). In this…
We present a method which delivers a continuous, high-density beam of slow and internally cold polar molecules. In our source, warm molecules are first cooled by collisions with a cryogenic helium buffer gas. Cold molecules are then…
Selection of "magic" trapping conditions with ultracold atoms or molecules, where pairs of internal states experience identical trapping potentials, brings substantial benefits to precision measurements and quantum computing schemes.…
The collective Raman cooling of trapped one- and two-component Fermi gases is considered. We obtain the quantum master equation that describes the laser cooling in the festina lente regime, for which the heating due to photon reabsorption…