Related papers: Time-resolved four-wave-mixing spectroscopy for in…
We describe an experiment to measure the emitted real-time electric field from an ultrafast third-order nonlinear optical interaction in molecules, using a phase-tracked spectral interferometry scheme. By combining a software lock-in…
We demonstrate time-resolved nonlinear extreme-ultraviolet absorption spectroscopy on multiply charged ions, here applied to the doubly charged neon ion, driven by a phase-locked sequence of two intense free-electron laser pulses.…
New experimental techniques based on non-linear ultrafast spectroscopies have been developed over the last few years, and have been demonstrated to provide powerful probes of quantum dynamics in different types of molecular aggregates,…
Here we show indirect precise angular control using a four-wave mixing (FWM) process. This was performed with a superposition of light with orbital angular momentum (OAM) in an M-Type configuration of a hot 85Rb atomic ensemble. A…
We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…
Quantum systems composed of solid-state electronic spins can be sensitive detectors of narrowband magnetic fields. A prominent example is the nitrogen-vacancy (NV) center in diamond, which has been employed for magnetic spectroscopy with…
Nonlinear spectroscopy in the extreme ultraviolet (EUV) and soft x-ray spectral range offers the opportunity for element selective probing of ultrafast dynamics using core-valence transitions (Mukamel et al., Acc. Chem. Res. 42, 553…
We observed electromagnetically-induced-transparency-based four-wave mixing (FWM) in the pulsed regime at low light levels. The FWM conversion efficiency of 3.8(9)% was observed in a four-level system of cold 87Rb atoms using a driving…
Three-color coherent anti-Stokes Raman scattering represents non-degenerate four wave mixing process that includes both a non-resonant and resonant processes, the contributions of which depend on how the molecular vibrational modes are…
Understanding the interaction of charge carriers with lattice vibrations in the quasi-equilibrium regime is crucial for semiconductor functionality. However, the structural signatures of these interactions are often too subtle for…
Exploring intermixing and interplay between different frequency-mixing processes has always been one of the interesting subjects at the interface of nonlinear optics with quantum optics. Here we investigate coherent competition and control…
A combined approach that uses the vibrational self-consistent field (VSCF) and vibrational configuration interaction (VCI) method together with the semiclassical instanton theory was developed to study vibrational tunneling spectra of…
Core excitons in solids have garnered increasing interest, yet their behavior and decay mechanisms are not fully understood. Here, we use attosecond extreme ultraviolet (XUV) transient absorption spectroscopy, performed with a broadband…
The Pixel-Imaging Mass Spectrometry (PImMS) camera allows for 3D charged particle imaging measurements, in which the particle time-of-flight is recorded along with $(x,y)$ position. Coupling the PImMS camera to an ultrafast pump-probe…
Frequency-modulation (FM) spectroscopy has been extended to the vacuum-ultraviolet (VUV) range of the electromagnetic spectrum. Coherent VUV laser radiation is produced by resonance-enhanced sum-frequency mixing…
We measure the time-energy correlation of broadband, spontaneously generated four wave mixing (FWM), and demonstrate novel time-frequency coupling effects; specifically, we observe a power-dependent splitting of the correlation in both…
The four-wave mixing produced with two ultrashort phase-locked w-3w laser pulses propagating coherently in a two-level system in the infrared spectral region is shown to depend on the pulses relative phase. The Maxwell-Bloch equations are…
In the last few decades the development of ultrafast lasers has revolutionized our ability to gain insight into light-matter interactions. The appearance of few-cycle light sources available from the visible to the mid-infrared spectral…
Matter-wave interferometry with molecules is intriguing both because it demonstrates a fundamental quantum phenomenon and because it opens avenues to quantum-enhanced measurements in physical chemistry. One great challenge in such…
We observe and control a molecular vibrational wave packet in an electronically excited state of the neutral hydrogen molecule. In an extreme-ultraviolet (XUV) transient-absorption experiment we launch a vibrational wave packet in the $D…