Related papers: Time-resolved four-wave-mixing spectroscopy for in…
Four-wave mixing (FWM) is an efficient source of light waves emitted at various frequencies, usually associated with third-order optical nonlinearities. Whereas attention has mostly been paid in the past to the generation of Stokes (e.g.,…
Infrared optical measurement has a wide range of applications in industry and science, but infrared light detectors suffer from high costs and inferior performance than visible light detectors. Four-wave mixing (FWM) process allows…
Correlation-function expressions are derived for the coherent nonlinear response of molecules to three resonant ultrafast pulses in the x-ray regime. The ability to create two-core-hole states with controlled attosecond timing in…
We resolve the real-time electric field of a femtosecond third-order nonlinear optical signal in the molecular frame. The electric field emitted by the induced third-order polarization from impulsively pre-aligned gas-phase molecules at…
Semiconductor quantum dot molecules are considered as promising candidates for quantum technological applications due to their wide tunability of optical properties and coverage of different energy scales associated with charge and spin…
We present an efficient scheme for the generation and control of a degenerate four-wave mixing (FWM) signal in a N-type inhomogeneously broadened 85Rb atomic system. We observe the propagation dynamics of the generated FWM signal along with…
We report here experimental results of perturbative nonlinear optical wave-mixing processes in the extreme ultraviolet region by using two-color and three-color laser fields. Besides the usual odd-harmonic spectrum of high harmonic…
Infrared-infrared double resonance measurements of the $\nu_3$ absorption band of $SF_6$ using a $CO_2$ TEA laser radiation have been carried out. The results obtained in the present and in some earlier works are discussed taking into…
The use of few-femtosecond, extreme ultraviolet (XUV) pulses, produced by high-order harmonic generation, in combination with few-femtosecond infrared (IR) pulses in pump-probe experiments has great potential to disclose ultrafast dynamics…
Attosecond noncollinear four wave mixing spectroscopy with one attosecond extreme ultraviolet (XUV) pulse and two few-cycle near-infrared (NIR) pulses was used to measure the autoionization decay lifetimes of inner valence electronic…
Excited-state vibrational dynamics in molecules can be studied by an electronically off-resonant Raman process induced by a probe pulse with variable delay with respect to an actinic pulse. We establish the connection between several…
We theoretically investigate a N-type 87Rb atomic system for efficient generation and control of a non-degenerate Four wave mixing (FWM) signal in pulsed regime. The susceptibility of the atomic medium is customized as a gain profile by a…
This tutorial provides a joint theoretical and experimental overview of heterodyne wave mixing spectroscopy, focusing mainly on four-wave mixing (FWM). This powerful and versatile time-resolved nonlinear optical spectroscopy technique…
We employ two-dimensional (2D) coherent, nonlinear spectroscopy to investigate couplings within individual InAs quantum dots (QD) and QD molecules. Swapping pulse ordering in a two-beam sequence permits to distinguish between rephasing and…
Combined spectrally and time resolved measurements provide information not otherwise available if performed in either domain alone. We demonstrate a new approach to Four Wave Mixing spectroscopy, where spectral selectivity is achieved by…
We describe a setup to study ultrafast dynamics in gas-phase molecules using time-resolved photoelectron and photoion spectroscopy. The vacuum ultraviolet (VUV) probe pulses are generated via strong field high-order harmonic generation from…
Coherent light pulses of few to hundreds of femtoseconds (fs) duration have prolifically served the field of ultrafast phenomena. While fs pulses address mainly dynamics of nuclear motion in molecules or lattices in the gas, liquid or…
The development of schemes for coherent nonlinear time-domain spectroscopy in the extreme-ultraviolet regime (XUV) has so far been impeded by experimental difficulties that arise at these short wavelengths. In this work we present a novel…
Measuring an electric field waveform beyond radio frequencies is often accomplished via a second-order nonlinear interaction with a laser pulse shorter than half of the field's oscillation period. However, synthesizing such a gate pulse is…
Coherent extreme ultraviolet (XUV) radiation produced by table-top high-harmonic generation (HHG) sources provides a wealth of possibilities in research areas ranging from attosecond physics to high resolution coherent imaging. However, it…