Related papers: Time-resolved four-wave-mixing spectroscopy for in…
We report an experiment to measure the femtosecond electric field of the signal emitted from an optical third-order nonlinear interaction in carbon dioxide molecules. Using degenerate four-wave mixing with femtosecond near infrared laser…
We demonstrate quantum interference of three photons that are distinguishable in time, by resolving them in the conjugate parameter, frequency. We show that the multiphoton interference pattern in our setup can be manipulated by tuning the…
It is very important to measure the plasma performances of fusion reactors such as fuel ion density, plasma temperature, fusion power, fast neutron energy, and neutron flux. Various diagnostic systems are needed to measure fast neutron…
We demonstrate rapid imaging based on four-wave mixing (FWM) by assessing the quality of advanced materials through measurement of their nonlinear response, exciton dephasing, and exciton lifetimes. We use a WSe$_2$ monolayer grown by…
We present an experimental and theoretical study of the interplay between ultrafast electron dynamics and librational dynamics in liquid nitrobenzene. A femtosecond ultraviolet pulse and two femtosecond near infrared pulses interact with…
A detailed understanding of the population and coherence dynamics in optically driven individual emitters in solids and their signatures in ultrafast nonlinear-optical signals is of prime importance for their applications in future quantum…
We demonstrate the double electromagnetically induced transparency (double-EIT) and double four-wave mixing (double-FWM) based on a new scheme of non-degenerate four-wave mixing (FWM) involving five levels of a cold 85Rb atomic ensemble, in…
Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…
Interferometry is a fundamental technique in physics, enabling precise measurements through the interference of waves. High-harmonic generation (HHG) in solids has emerged as a powerful method for probing ultrafast electronic dynamics…
Resonance states of axion-like particles were searched for via four-wave mixing by focusing two-color pulsed lasers into a quasi-vacuum. A quasi-parallel collision system that allows probing of the sub-eV mass range was realized by focusing…
We study the nonlinear optical response of argon to a four-wave-mixing pulse sequence consisting of an extreme ultraviolet pulse, an overlapping collinear IR and an non-collinear delayed IR pulses. Absorption of an extreme ultraviolet and…
Recent theoretical studies in quantum spectroscopy have emphasized the potential of non-classical correlations in entangled photon pairs for selectively targeting specific nonlinear optical processes in nonlinear optical responses. However,…
A step towards a successful implementation of timeresolved digital in-line holography with extreme ultraviolet radiation is presented. Ultrashort XUV pulses are produced as high-order harmonics of a femtosecond laser and a Schwarzschild…
We present an experimental and theoretical study of photon pairs generated by spontaneous four wave mixing (SFWM), based on birefringent phasematching, in a fiber which supports more than one transverse mode. We present SFWM spectra,…
We analyze the photoelectron angular distribution in two-pathway interference between non\-resonant one-photon and resonant two-photon ionization of neon. We consider a bichromatic femtosecond XUV pulse whose fundamental frequency is tuned…
The possibility of using time-resolved vibronic spectroscopy for spectral analysis of mixtures of chemical compounds with similar optical properties, when traditional methods are inefficient, is demonstrated by using the method of computer…
The early stage density oscillations of the electronic charge in molecules irradiated by an attosecond XUV pulse takes place on femto- or subfemtosecond timescales. This ultrafast charge migration process is a central topic in attoscience…
Dual-comb spectroscopy can provide broad spectral bandwidth and high spectral resolution in a short acquisition time, enabling time-resolved measurements. Specifically, spectroscopy in the mid-infrared wavelength range is of particular…
Franson interference can be used to test the nonlocal features of energy-time entanglement and has become a standard in quantum physics. However, most of the previous Franson interference experiments were demonstrated in the time domain,…
The utility of resonant scattering spectroscopies for identifying electronic symmetries and density distributions changes dramatically as a function of photon energy. In the hard X-ray regime, strong core hole monopole potentials tend to…