Related papers: Time-resolved four-wave-mixing spectroscopy for in…
Four-wave mixing (FWM) in gas-filled hollow-core capillaries, a nonlinear optical process that mixes signal and pump photon frequencies to generate idler frequency photons, offers a method for precise spectral phase transfer from signal to…
Nonlinear wave mixing in the X-ray range can provide valuable insights into the structural and electron dynamics of atomic and molecular systems on ultrafast time scales, with state- and site-selectivity and atomic resolution. This…
We report here a detailed study of the four-wave mixing process in the extreme ultraviolet (XUV) region around 30 nm by using two collinear incommensurate frequency laser pulses. The experimental results reveal evidence of the coherent…
The extension of nonlinear spectroscopic techniques into the x-ray domain is in its infancy but holds the promise to provide unique insight into the dynamics of charges in photoexcited processes, which are of fundamental as well as applied…
Extreme-ultraviolet (XUV) sources including high-harmonic generation, free-electron lasers, soft x-ray lasers and laser-driven plasmas are widely used for applications ranging from femtochemistry and attosecond science to coherent…
Strong ultrashort laser pulses give rise to prompt molecular alignment followed by full, half and quarter quantum revivals of the rotational wave packets. In Four Wave Mixing (FWM) experiments, we make use of the long succession of…
All-optical logic-gate-based switching is a prerequisite for photonic computing. This article introduces a logic-gate protocol for noncollinear four-wave mixing (FWM) of one attosecond extreme ultraviolet (XUV) with two few-femtosecond near…
We experimentally demonstrate wide-band (>100 THz) frequency down-conversion of near-infrared (NIR) femtosecond-scale pulses from an Er:fiber laser to the mid-infrared (MIR) using four-wave-mixing (FWM) in photonic-chip silicon-nitride…
We combine different wavelengths from an intense high-order harmonics source with variable delay at the focus of a split-mirror interferometer to conduct pump-probe experiments on gas-phase molecules. We report measurements of the time…
We study theoretically the nonlinear four wave mixing (FWM) response of an ensemble of coupled pairs of quantum dots (quantum dot molecules). We discuss the shape of the FWM echo signal depending on the parameters of the ensemble: the…
Noncollinear wave-mixing spectroscopies with attosecond extreme ultraviolet (XUV) pulses provide unprecedented insight into electronic dynamics. In infrared and visible regimes, heterodyne detection techniques utilize a reference field to…
Programmable shaping of femtosecond ultraviolet (UV) pulses is still much less flexible than at visible and near-infrared wavelengths, mainly because direct UV modulators remain limited in bandwidth, throughput and damage threshold. Here we…
The nonlinear interaction between Near-Infrared (NIR) and Terahertz pulses is principally investigated as a means for the detection of radiation in the hardly accessible THz spectral region. Most studies have targeted second-order nonlinear…
Nonlinear wave-mixing in solids with ultrafast x-rays can provide new insight into complex electronic dynamics of materials. Here, tabletop-based attosecond noncollinear four-wave mixing (FWM) spectroscopy using one extreme ultraviolet…
The recent development of ultrafast extreme ultraviolet (XUV) coherent light sources bears great potential for a better understanding of the structure and dynamics of matter. Promising routes are advanced coherent control and nonlinear…
Nonlinear Four-wave mixing processes are a powerful technique to unravel ultrafast dynamics in solid-state systems. Here, we employ attosecond four-wave mixing spectroscopy with one extreme ultraviolet (XUV) pump and two independently…
We study theoretically the time-resolved four-wave mixing (FWM) response of an ensemble of pairs of quantum dots undergoing radiative recombination. At short (picosecond) delay times, the response signal shows beats that may be dominated by…
We have analyzed a five-level $\wedge$-configuration Four-Wave Mixing (FWM) scheme for obtaining a high-efficiency FWM based on the two electromagnetically induced transparency. We find that the maximum FWM efficiency is nearly 30%, which…
Spectro-temporal shaping of high-power femtosecond ultraviolet (UV) pulses remains a key challenge in ultrafast optics. Tailoring high-energy, ultrashort UV pulses underpins applications in ultrafast dynamics, high-precision spectroscopy,…
We measure molecular vibrations with femtometer precision using time-resolved x-ray absorption spectroscopy. For a demonstration, a Raman process excites the A$_{1g}$ mode in gas-phase SF$_6$ molecules with an amplitude of $\approx50$ fm,…