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X-ray free electron lasers (XFELs) generate sequences of ultra-short, spatially coherent pulses of x-ray radiation. We propose the diffraction focusing spectrometer (DFS), which is able to measure the whole energy spectrum of the radiation…

Optics · Physics 2013-02-22 V. G. Kohn , O. Y. Gorobtsov , I. A. Vartanyants

Streaking of photoelectrons with optical lasers has been widely used for temporal characterization of attosecond extreme ultraviolet pulses. Recently, this technique has been adapted to characterize femtosecond x-ray pulses in free-electron…

Diffraction-before-destruction imaging with single ultrashort X-ray pulses has the potential to visualise non-equilibrium processes, such as chemical reactions, at the nanoscale with sub-femtosecond resolution in the native environment…

Diffraction imaging of non-equilibrium dynamics at atomic resolution is becoming possible with X-ray free-electron lasers. However, there are unresolved problems with applying this method to objects that are confined in only one dimension.…

Strongly Correlated Electrons · Physics 2018-02-19 Kenneth R. Beyerlein

A new approach for few-femtosecond time-resolved photoelectron spectroscopy in condensed matter that balances the combined needs for both temporal and energy resolution is demonstrated. Here, the method is designed to investigate a…

The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectroscopy and diffraction imaging is a powerful approach to…

The time-resolved electron beam envelope parameters including sectional distribution and position are important and necessary for the study of beam transmission characteristics in the magnetic field and verifying the magnetic field setup…

Accelerator Physics · Physics 2015-02-10 Jiang Xiaoguo , Wang Yuan , Yang Zhiyong , Zhang Huang , Wang Yi , Wei Tao

The wavefront measurement of a light beam is a complex task, which often requires a series of spatially resolved intensity measurements. For instance, a detector array may be used to measure the local phase gradient in the transverse plane…

One of the frontiers in electron scattering is to couple ultrafast temporal resolution with highly localized probes to investigate the role of microstructure on material properties. Here, taking advantage of the unprecedented average…

Applied Physics · Physics 2019-06-07 Fu-Hao Ji , Daniel Durham , Andrew Minor , Pietro Musumeci , Jorge Navarro , Daniele Filippetto

Ultrashort, low-emittance electron pulses can be created at a high repetition rate by using a TM$_{110}$ deflection cavity to sweep a continuous beam across an aperture. These pulses can be used for time-resolved electron microscopy with…

Applied Physics · Physics 2018-04-24 W. Verhoeven , J. F. M. van Rens , E. R. Kieft , P. H. A. Mutsaers , O. J. Luiten

This paper describes a new radio frequency timer of keV energy electrons. It is based on a helical deflector, which performs circular or elliptical sweeps of keV electrons, by means of 500 MHz radio frequency field. By converting a time…

Temporally-shaped electron bunches at ultrafast time scales are foreseen to support an array of applications including the development of small-footprint accelerator-based coherent light sources or as probes for, e.g., ultrafast…

Accelerator Physics · Physics 2019-11-13 A. Halavanau , Q. Gao , M. Conde , G. Ha , P. Piot , J. G. Power , E. Wisniewski

The undulator is a critical component to produce synchrotron radiation and free electron laser. When a Bessel light beam carrying the orbit angular momentum co-propagates with an electron beam, a net transverse deflection force will be…

Accelerator Physics · Physics 2017-09-13 Bocheng Jiang , Qinglei Zhang , Zhentang Zhao

Pushing the limits in temporal resolution for transmission electron microscopy (TEM) requires a revolutionary change in the electron source technology. In this paper we study the possibility of employing a radiofrequency photoinjector as…

Accelerator Physics · Physics 2014-05-26 R. K. Li , P. Musumeci

The temporal resolution of sub-relativistic ultrafast electron diffraction (UED) is generally limited by radio frequency (RF) phase and amplitude jitter of the RF lenses that are used to compress the electron pulses. We theoretically show…

Accelerator Physics · Physics 2017-05-29 J. G. H. Franssen , O. J. Luiten

We present time-resolved X-ray diffraction measurements using advanced timing schemes that provide high temporal resolution while also maintaining a high flux in the X-ray probe beam. The method employs patterned probe pulse sequences that…

We report the design and performance of a time-resolved electron diffraction apparatus capable of producing intense bunches with simultaneously single digit micron probe size, long coherence length, and $200$ fs rms time resolution. We…

Electrical pulse stimulation drives many important physical phenomena in condensed matter as well as in electronic systems and devices. Often, nanoscopic and mesoscopic mechanisms are hypothesized, but methods to image electrically driven…

Mesoscale and Nanoscale Physics · Physics 2023-06-05 Thomas E Gage , Daniel B Durham , Haihua Liu , Supratik Guha , Ilke Arslan , Charudatta Phatak

Angle-resolved photoemission spectroscopy (ARPES) provides a direct access to the electronic band structure of solid and molecular systems. The momentum range accessible by this technique depends directly on the photon energy used, and…