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Time-resolved near-infrared absorption spectroscopy of single non-repeatable transient events is performed at high spectral resolution with a dual-comb interferometer using a continuous-wave laser followed by a single electro-optic…

Ultrafast electron diffraction (UED) is a technique in which short-pulse electron beams can probe the femtosecond-scale evolution of atomic structure in matter driven far from equilibrium. As an accelerator physics challenge, UED imposes…

The precise temporal characterization of laser pulses is crucial for ultrashort applications in biology, chemistry, and physics. Especially in femto- and attosecond science, diverse laser pulse sources in different spectral regimes from the…

Single molecule spectroscopy aims at unveiling often hidden but potentially very important contributions of single entities to a system's ensemble response. Albeit contributing tremendously to our ever growing understanding of molecular…

Chemical Physics · Physics 2017-12-19 Matz Liebel , Costanza Toninelli , Niek F. van Hulst

We propose a simple laser-driven electron acceleration scheme based on tightly focused radially polarized laser pulses for the production of femtosecond electron bunches with energies in the few-hundreds-of-keV range. In this method, the…

Accelerator Physics · Physics 2013-12-10 Vincent Marceau , Charles Varin , Thomas Brabec , Michel Piché

Recently, the delayed-choice quantum eraser has been applied for coherently excited superresolution using phase-controlled projection measurements of laser light to overcome the diffraction limit in classical physics as well as to solve the…

Quantum Physics · Physics 2024-02-27 Byoung S. Ham

Imaging the structure of molecules in transient excited states remains a challenge due to the extreme requirements for spatial and temporal resolution. Ultrafast electron diffraction from aligned molecules (UEDAM) provides atomic resolution…

Atomic Physics · Physics 2015-10-23 Jie Yang , Joshua Beck , Cornelis J. Uiterwaal , Martin Centurion

Free electrons provide a powerful tool to probe material properties at atomic-scale spatial resolution. Recent advances in ultrafast electron microscopy enable the manipulation of free electron wavefunctions using laser pulses. It would be…

Quantum Physics · Physics 2021-06-16 Ron Ruimy , Alexey Gorlach , Chen Mechel , Nicholas Rivera , Ido Kaminer

We demonstrate phase super-resolution in the absence of entangled states. The key insight is to use the inherent time-reversal symmetry of quantum mechanics: our theory shows that it is possible to \emph{measure}, as opposed to prepare,…

Quantum Physics · Physics 2008-11-26 K. J. Resch , K. L. Pregnell , R. Prevedel , A. Gilchrist , G. J. Pryde , J. L. O'Brien , A. G. White

We present the development of a time- and angle-resolved photoemission spectroscopy based on a Yb-based femtosecond laser and a hemispherical electron analyzer. The energy of the pump photon is tunable between 1.4 and 1.9 eV, and the pulse…

Strongly Correlated Electrons · Physics 2020-03-03 Yuanyuan Yang , Tianwei Tang , Shaofeng Duan , Chaocheng Zhou , Duxing Hao , Wentao Zhang

In this paper we present proof of principle experiments of an optical gating concept for free electrons. We demonstrate a temporal resolution of 1.2+-0.3 fs via energy and transverse momentum modulation as a function of time. The scheme is…

Recent advancements in ultrafast laser systems and high harmonic generation (HHG) techniques have enabled time-resolved photoemission spectroscopy on femtosecond timescales, opening up unprecedented opportunities to explore quantum…

Strongly Correlated Electrons · Physics 2025-11-03 Takeshi Suzuki , Kozo Okazaki

The investigation of ultrafast electronic and structural dynamics in low-dimensional systems like nanowires and two-dimensional materials requires femtosecond probes providing high spatial resolution and strong interaction with small volume…

Mesoscale and Nanoscale Physics · Physics 2014-11-18 Melanie Müller , Alexander Paarmann , Ralph Ernstorfer

The paper describes a time- and angle-resolved photoemission apparatus consisting of a hemispherical analyzer and a pulsed laser source. We demonstrate 1.48-eV pump and 5.90-eV probe measurements at the >10.5-meV and >240-fs resolutions by…

Materials Science · Physics 2016-12-16 Y. Ishida , T. Togashi , K. Yamamoto , M. Tanaka , T. Kiss , T. Otsu , Y. Kobayashi , S. Shin

The generation of a flat electron beam directly from a photoinjector is an attractive alternative to the electron damping ring as envisioned for linear colliders. It also has potential applications to light sources such as the generation of…

Accelerator Physics · Physics 2009-11-11 P. Piot , Y. -E Sun , K. -J. Kim

We propose a method for a straightforward characterization of the temporal shape of femtosecond pulses in the extreme-ultraviolet/soft X-ray spectral region. The approach is based on the presence of a significant linear frequency chirp in…

Optics · Physics 2015-06-15 David Gauthier , Benoît Mahieu , Giovanni De Ninno

Photoinjectors are the main high brightness electron sources for X-ray free electron lasers (XFEL). Photoinjector emittance reduction is one of the key knobs for improving XFEL lasing, so precise emittance measurement is critical. It's well…

The emission times of laser-triggered electrons from a sharp tungsten tip are directly characterized under ultrafast, near-infrared laser excitation at Keldysh parameters $6.6< \gamma < 19.1$. Emission delays up to 10 fs are observed, which…

Paradoxically, imaging with resolution much below the wavelength $\lambda$ - now common place in the visible spectrum - remains challenging at lower frequencies, where arguably it is needed most due to the large wavelengths used. Techniques…

Optics · Physics 2023-12-12 Alessandro Tuniz , Boris T. Kuhlmey

Non-line-of-sight (NLOS) imaging enables monitoring around corners and is promising for diverse applications. The resolution of transient NLOS imaging is limited to a centimeter scale, mainly by the temporal resolution of the detectors.…

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