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We present a detailed investigation of the exciton and trion dynamics in naturally doped MoSe2 and WSe2 single atomic layers as a function of temperature in the range 10-300K under above band-gap laser excitation. By combining…

Monolayer transition metal dichalcogenides (1L-TMDs) have tremendous potential as atomically thin, direct bandgap semiconductors that can be used as convenient building blocks for quantum photonic devices. However, the short exciton…

We study the dynamic equilibrium between trions and excitons in monolayers of transition metal dichalcogenides in the presence of resident charge carriers and continuous photogeneration of excitons. We show that heating of the system via…

Mesoscale and Nanoscale Physics · Physics 2026-03-25 A. M. Shentsev

Transition metal dichalcogenide (TMD) heterobilayers provide a versatile platform to explore unique excitonic physics via properties of the constituent TMDs and external stimuli. Interlayer excitons (IXs) can form in TMD heterobilayers as…

Mesoscale and Nanoscale Physics · Physics 2023-11-02 Hanlin Fang , Qiaoling Lin , Yi Zhang , Joshua Thompson , Sanshui Xiao , Zhipei Sun , Ermin Malic , Saroj Dash , Witlef Wieczorek

Hyperspectral imaging at cryogenic temperatures is used to investigate exciton and trion propagation in MoSe$_2$ monolayers encapsulated with hexagonal boron nitride (hBN). Under a tightly focused, continuous-wave laser excitation, the…

Two-dimensional (2D) transition metal dichalcogenides (TMDC) and their moir\'e interfaces have been demonstrated for correlated electron states, including Mott insulators and electron/hole crystals commensurate with moir\'e superlattices.…

Mesoscale and Nanoscale Physics · Physics 2024-01-08 Yusong Bai , Yiliu Li , Song Liu , Yinjie Guo , Jordan Pack , Jue Wang , Cory R. Dean , James Hone , X. -Y. Zhu

The optical properties of atomically thin transition metal dichalcogenide (TMDC) semiconductors are shaped by the emergence of correlated many-body complexes due to strong Coulomb interaction. Exceptional electron-hole exchange predestines…

We analyze the dielectric-function spectra of low dimensional transition metal dichalcogenides (TMDCs) using a fully analytical model of the complex dielectric function that is applicable in fractional dimensional space. We extract the…

Materials Science · Physics 2018-12-04 A. Thilagam

Recent synthetic progress has enabled the controlled fusion of colloidal CdSe/CdS quantum dots in order to form dimers manifesting electronic coupling in their optical response. While this ``artificial H2 molecule'' constitutes a milestone…

Mesoscale and Nanoscale Physics · Physics 2024-11-27 Jordi Llusar , Juan I. Climente

Spin-forbidden intravalley dark exciton in tungsten-based transition metal dichalcogenides (TMDCs), owing to its unique spin texture and long lifetime, has attracted intense research interest. Here, we show that we can control the dark…

Developments in optoelectronics and spin-optronics based on transition metal dichalcogenide monolayers (MLs) need materials with efficient optical emission and well-defined transition energies. In as-exfoliated MoS2 MLs the…

Strong Coulomb interaction in atomically-thin transition metal dichalcogenides makes these systems particularly promising for studies of excitonic physics. Of special interest are the manifestations of the charged excitons, also known as…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 M. M. Glazov

The possibility of almost linear tuning of the band gap and of the electrical and optical properties in monolayers (MLs) of semiconducting transition metal dichalcogenide (S-TMD) alloys opens up the way to fabricate materials with on-demand…

We theoretically investigate the corrections of exciton binding energy in monolayer transition metal dichalcogenides (TMDs) due to the exciton-optical phonon coupling in the Fr$\ddot{o}$hlich interaction model by using the linear operator…

Mesoscale and Nanoscale Physics · Physics 2017-01-04 Zi-Wu Wang , Yao Xiao , Wei-Ping Li , Run-Ze Li , Zhi-Qing Li

We study possible optically excited bound states in monolayer MoS2: excitons and trions. For this purpose we formulate and apply a generalized time-dependent density-matrix functional approach for bound states of multiple excitations. The…

Mesoscale and Nanoscale Physics · Physics 2014-02-18 Alfredo Ramirez-Torres , Volodymyr Turkowski , Talat S. Rahman

Heterostructures of two-dimensional transition metal dichalcogenides (TMDs) are emerging as a promising platform for investigating exotic correlated states of matter. Here, we propose to engineer Bose-Fermi mixtures in these systems by…

Mesoscale and Nanoscale Physics · Physics 2024-08-01 Caterina Zerba , Clemens Kuhlenkamp , Ataç Imamoğlu , Michael Knap

Exciton binding energies of hundreds of meV and strong light absorption in the optical frequency range make transition metal dichalcogenides (TMDs) promising for novel optoelectronic nanodevices. In particular, atomically thin TMDs can be…

Mesoscale and Nanoscale Physics · Physics 2018-04-24 Simon Ovesen , Samuel Brem , Christopher Linderälv , Mikael Kuisma , Paul Erhart , Malte Selig , Ermin Malic

Strong light-matter interactions in layered transition metal dichalcogenides (TMDs) open up vivid possibilities for novel exciton-based devices. The optical properties of TMDs are dominated mostly by the tightly bound excitons and more…

Transition-metal dichalcogenides can be easily produced as atomically thin sheets, exhibiting the possibility to optically polarize and read out the valley pseudospin of extremely stable excitonic quasiparticles present in these 2D…

We examine a mechanism by which excitons undergo ultrafast relaxation in common monolayer transition metal dichalcogenides. It is shown that at densities $\approx$ 1$\times$ 10$^{11}$ cm$^{-2}$ and temperatures $ \le 60$ K, excitons in well…

Mesoscale and Nanoscale Physics · Physics 2016-06-29 A. Thilagam
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