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We study spatial photoluminescence characteristics of neutral and charged excitons across extended monolayer MoS$_2$ synthesized by chemical vapor deposition. Using two-dimensional hyperspectral photoluminescence mapping at cryogenic…

Mesoscale and Nanoscale Physics · Physics 2019-02-20 Andre Neumann , Jessica Lindlau , Manuel Nutz , Aditya D. Mohite , Hisato Yamaguchi , Alexander Högele

Monolayers of transition metal dichalcogenides (TMDs) have been established in the last years as promising materials for novel optoelectronic devices. However, the performance of such devices is often limited by the dissociation of tightly…

Mesoscale and Nanoscale Physics · Physics 2024-02-13 Raul Perea-Causin , Samuel Brem , Ermin Malic

We have investigated the exciton dynamics in transition metal dichalcogenide mono-layers using time-resolved photoluminescence experiments performed with optimized time-resolution. For MoSe2 monolayers, we measure $\tau_{rad}=1.8\pm0.2$ ps…

Materials Science · Physics 2016-05-18 C. Robert , D. Lagarde , F. Cadiz , G. Wang , B. Lassagne , T. Amand , A. Balocchi , P. Renucci , S. Tongay , B. Urbaszek , X. Marie

Monolayers of transition metal dichalcogenides present an intriguing platform to investigate the interplay of excitonic complexes in two dimensional semiconductors. Here, we use optical spectroscopy to study light-matter coupling and…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 Jonas Zipfel , Koloman Wagner , Jonas D. Ziegler , Takashi Taniguchi , Kenji Watanabe , Marina A. Semina , Alexey Chernikov

We investigate how many-electron excited states emerge in twisted MoSe2 homobilayers when the lattice reconstructions evolve. Notably, we identify a new trion resonance that arises in the transition regime of lattice reconstruction, where…

Charged optical excitations (trions) generated by charge carrier injection are crucial for emerging optoelectronic technologies as they can be produced and manipulated by electric fields. Trions and neutral excitons can be efficiently…

Atomic and Molecular Clusters · Physics 2021-12-23 Jiří Doležal , Sofia Canola , Pablo Merino , Martin Švec

We perform photoluminescence experiments at 4K on two different transition metal diselenide monolayers, namely MoSe2 and WSe2 in magnetic fields $B_z$ up to 9T applied perpendicular to the sample plane. In MoSe2 monolayers the valley…

Materials Science · Physics 2015-06-12 G. Wang , L. Bouet , M. M. Glazov , T. Amand , E. L. Ivchenko , E. Palleau , X. Marie , B. Urbaszek

We investigate the diffusion process of negatively charged excitons (trions) in WSe2 transition metal dichalcogenide monolayer. We measure time-resolved photoluminescence spatial profiles of these excitonic complexes which exhibit a…

Transition metal dichalcogenide (TMDC) heterostructures have unique properties that depend on the twisting angle and stacking order of two or more monolayers. However, their practical applications are limited by the low photoluminescence…

We present a microscopic many-body calculation of the nonlinear two-dimensional coherent spectroscopy (2DCS) of trion-polaritons and exciton-polaritons in charge-tunable transition-metal-dichalcogenides monolayers placed in an optical…

Quantum Gases · Physics 2025-04-22 Hui Hu , Jia Wang , Riley Lalor , Xia-Ji Liu

Monolayer transition metal dichalcogenides (TMDs) are direct gap semiconductors that hold great promise for advanced applications in photonics and optoelectronics. Understanding the interplay between their radiative and non-radiative…

Charge doping in transition metal dichalcogenide is currently a subject of high importance for future electronic and optoelectronic applications. Here we demonstrate chemical doping in CVD grown monolayer (1L) of WS2 by a few commonly used…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Anand P. S. Gaur , Adriana M. Rivera , Saroj P. Dash , Sandwip Dey , Ram S. Katiyar , Satyaprakash Sahoo

Excitons in monolayer transition metal dichalcogenide (TMD) provide a paradigm of composite Boson in 2D system. This letter reports a photoluminescence and reflectance study of excitons in monolayer molybdenum diselenide (MoSe2) with…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 Ke Xiao , Tengfei Yan , Qiye Liu , Siyuan Yang , Chiming Kan , Ruihuan Duan , Zheng Liu , Xiaodong Cui

We study a doped transition metal dichalcogenide (TMDC) monolayer in an optical microcavity. Using the microscopic theory, we simulate spectra of quasiparticles emerging due to the interaction of material excitations and a high-finesse…

Materials Science · Physics 2024-07-23 Y. V. Zhumagulov , S. Chiavazzo , D. R. Gulevich , V. Perebeinos , I. A. Shelykh , O. Kyriienko

Trions are a three-particle bound state of electrons and holes. Experimental realization of a trion liquid in the degenerate quantum limit would open a wide range of phenomena in quantum many-body physics. However, trions have been observed…

Mesoscale and Nanoscale Physics · Physics 2023-12-21 Phuong X. Nguyen , Raghav Chaturvedi , Liguo Ma , Patrick Knuppel , Kenji Watanabe , Takashi Taniguchi , Kin Fai Mak , Jie Shan

Vertical heterostructures (HS) of transition metal dichalcogenides (TMDs) host interlayer excitons (ILX), with electrons and holes residing in different layers. With respect to their intralayer counterparts, ILX feature much longer…

Monolayer phosphorene provides a unique two-dimensional (2D) platform to investigate the fundamental dynamics of excitons and trions (charged excitons) in reduced dimensions. However, owing to its high instability, unambiguous…

Materials Science · Physics 2015-04-30 Jiong Yang , Renjing Xu , Jiajie Pei , Ye Win Myint , Fan Wang , Zhu Wang , Shuang Zhang , Zongfu Yu , Yuerui Lu

Strong Coulomb interactions in single-layer transition metal dichalcogenides (TMDs) result in the emergence of strongly bound excitons, trions and biexcitons. These excitonic complexes possess the valley degree of freedom, which can be…

We report a photoluminescence (PL) and transient reflection spectroscopy study of exciton dynamics in monolayer transition transition-metal dichalcogenides (TMDs). PL saturation in monolayer MoSe2 occurs an excitation intensity more than…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Min Ju Shin , Dong Hak Kim , D. Lim

Monolayer transition metal dichalcogenides (TMDs) have been in focus of current research, among others due to their remarkable exciton landscape consisting of bright and dark excitonic states. Although dark excitons are not directly visible…

Materials Science · Physics 2020-12-21 Maja Feierabend , Samuel Brem , August Ekman , Ermin Malic