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Monolayer molybdenum disulfide (MoS$_2$) has emerged as an excellent 2D model system because of its two inequivalent, direct-gap valleys that lead to exotic bound and excited states. Here we focus on one such bound state, the negatively…

Materials Science · Physics 2016-06-01 Jason W. Christopher , Bennett B. Goldberg , Anna K. Swan

Transition metal dichalcogenides (TMDs) are regarded as a possible materials platform for quantum information science and related device applications. In TMD monolayers, the dephasing time and inhomogeneity are crucial parameters for any…

The remarkably strong Coulomb interaction in atomically thin transition metal dichalcogenides (TMDs) results in an extraordinarily rich many-particle physics including the formation of tightly bound excitons. Besides optically accessible…

Mesoscale and Nanoscale Physics · Physics 2017-03-10 Malte Selig , Gunnar Berghäuser , Marten Richter , Rudolf Bratschitsch , Andreas Knorr , Ermin Malic

Monolayer transition metal dichalcogenides host a variety of optically excited quasiparticles species that stem from two-dimensional confinement combined with relatively large carrier effective masses and reduced dielectric screening. The…

The strong excitonic effect in monolayer transition metal dichalcogenide (TMD) semiconductors has enabled many fascinating light-matter interaction phenomena. Examples include strongly coupled exciton-polaritons and nearly perfect atomic…

Mesoscale and Nanoscale Physics · Physics 2021-04-13 Hongchao Xie , Shengwei Jiang , Daniel A. Rhodes , James C. Hone , Jie Shan , Kin Fai Mak

The direct band gap character and large spin-orbit splitting of the valence band edges (at the K and K' valleys) in monolayer transition metal dichalcogenides have put these two-dimensional materials under the spot-light of intense…

Mesoscale and Nanoscale Physics · Physics 2017-04-10 Mark Danovich , Viktor Zólyomi , Vladimir I. Fal'ko

The nature of trions and their interaction with light has remained a puzzle. The composition and dispersion of polaritons involving trions provide insights into this puzzle. Trions and excitons in doped two-dimensional (2D) materials are…

Mesoscale and Nanoscale Physics · Physics 2021-07-28 Okan Koksal , Minwoo Jung , Christina Manolatou , A. Nick Vamivakas , Gennady Shvets , Farhan Rana

The optical properties of atomically thin semiconductors are dominated by excitons, tightly bound electron-hole pairs, which give rise to particularly rich and remarkable physics. Despite their importance, the microscopic formation…

Photoluminescence (PL) of transition metal dichalcogenide (TMD) monolayers is strongly influenced by the dielectric environment. The defect states present in the substrate induces uncontrollable doping in the TMD monolayer and thereby…

There are conflicting predictions and reports on the character of the exciton Mott transition (EMT) in monolayer transition metal dichalcogenides. It could be either a discontinuous or a continuous transition from the excitonic to the…

Materials Science · Physics 2026-01-27 Subhadra Mohapatra , Samuel Palato , Nicholas Olsen , Julia Stähler , Lukas Gierster

Transition metal dichalcogenides (TMDs) are layered materials that have a semiconducting phase with many advantageous optoelectronic properties, including tightly bound excitons and spin-valley locking. In Tungsten-based TMDs, spin and…

Mesoscale and Nanoscale Physics · Physics 2022-04-27 Saroj B. Chand , John M. Woods , Enrique Mejia , Takashi Taniguchi , Kenji Watanabe , Gabriele Grosso

The interaction between off-resonant laser pulses and excitons in monolayer transition metal dichalcogenides is attracting increasing interest as a route for the valley-selective coherent control of the exciton properties. Here, we extend…

The photoluminescence (PL) spectrum of transition metal dichalcogenides (TMDs) shows a multitude of emission peaks below the bright exciton line and not all of them have been explained yet. Here, we study the emission traces of…

Transitions metal dichalcogenides (TMDs) are direct semiconductors in the atomic monolayer (ML) limit with fascinating optical and spin-valley properties. The strong optical absorption of up to 20 % for a single ML is governed by excitons,…

Mesoscale and Nanoscale Physics · Physics 2018-09-26 B. Han , C. Robert , E. Courtade , M. Manca , S. Shree , T. Amand , P. Renucci , T. Taniguchi , K. Watanabe , X. Marie , L. E. Golub , M. M. Glazov , B. Urbaszek

Since the discovery of semiconducting monolayer transition metal dichalcogenides, a variety of experimental and theoretical studies have been carried out seeking to understand the intrinsic exciton population decay and valley relaxation…

Mesoscale and Nanoscale Physics · Physics 2016-05-04 Galan Moody , John Schaibley , Xiaodong Xu

Optical excitation typically enhances electrical conduction and low-frequency radiation absorption in semiconductors. We have, however, observed a pronounced transient decrease of conductivity in doped monolayer molybdenum disulfide (MoS2),…

Mesoscale and Nanoscale Physics · Physics 2014-10-22 C. H. Lui , A. J. Frenzel , D. V. Pilon , Y. -H. Lee , X. Ling , G. M. Akselrod , J. Kong , N. Gedik

Exciton dissociation plays a crucial role in the performance of optoelectronic devices based on two-dimensional (2D) transition metal dichalcogenides (TMDs). In this work, we investigate the effect of an in-plane electric field on the…

Materials Science · Physics 2024-10-11 Tao Zhu , Chenhang Zheng , Lei Xu , Ming Yang

Monolayers of transition metal dichalcogenides (TMDs) have recently emerged as a promising optoelectronic platform. To leverage their full potential, however, it is important to understand and engineer the properties of the different…

Screening due to surrounding dielectric medium reshapes the electron-hole interaction potential and plays a pivotal role in deciding the binding energies of strongly bound exciton complexes in quantum confined monolayers of transition metal…

Mesoscale and Nanoscale Physics · Physics 2017-08-16 Garima Gupta , Sangeeth Kallatt , Kausik Majumdar

Understanding and controlling the nanoscale transport of excitonic quasiparticles in atomically thin 2D semiconductors is crucial to produce highly efficient nano-excitonic devices. Here, we present a nano-gap device to selectively confine…

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