Related papers: Strongly aligned gas-phase molecules at Free-Elect…
We demonstrate for the first time coherent control of bond making, a milestone on the way to coherent control of photo-induced bimolecular chemical reactions. In strong-field multiphoton femtosecond photoassociation experiments, we find the…
Laser-produced plasma (LPP) induced during irradiation of a liquid tin droplet with diameter of 150 um and 180 um by CO2 laser pulse with various pulse durations and energies is considered. The two-dimensional radiative magnetohydrodynamic…
XUV and X-ray Free Electron Lasers (FELs) produce short wavelength pulses with high intensity, ultrashort duration, well-defined polarization and transverse coherence, and have been utilised for many experiments previously possible at long…
Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…
We demonstrate strong laser-field-free orientation of absolute-ground-state carbonyl sulfide molecules. The molecules are oriented by the combination of a 485-ps-long non-resonant laser pulse and a weak static electric field. The edges of…
Two dimensional particle-in-cell simulations characterizing the interaction of ultraintense short pulse lasers in the range 10^{18} \leq I \leq 10^{20} W/cm^{2} with converging target geometries are presented. Seeking to examine intensity…
Active energy compression scheme is presently being investigated for future laser-plasma accelerators. This method enables generating laser-plasma accelerator electron beams with a small, $\sim 10^{-5}$, relative slice energy spread. When…
Using frequency-chirped radiation pressure slowing, we precisely control the velocity of a pulsed CaF molecular beam down to a few m/s, compressing its velocity spread by a factor of 10 while retaining high intensity: at a velocity of…
Dalian Coherent Light Source will use a 300MeV LINAC to produce fully coherent photon pulses in the wavelength range between 150-50nm by high gain harmonic generation free electron laser (FEL) scheme. To generate stable FEL pulses,…
Advances in ultra-intense laser technology are enabling, for the first time, relativistic intensities at mid-infrared (mid-IR) wavelengths. Anticipating further experimental research in this domain, we present high-resolution two…
We investigate a single-laser scheme for reaching the strong-field QED regime based on direct laser acceleration (DLA) of electrons followed by their head-on collision with the same laser pulse reflected from an overdense foil. In this…
A time-dependent bond-hardening process is discovered in a polyatomic molecule (tetramethyl silane, TMS) using few-cycle pulses of intense 800 nm light. In conventional mass spectrometry, symmetrical molecules like TMS do not exhibit a…
We propose a technique, to be used for time-resolved pump-probe experiments, for timing an x-ray free electron laser (XFEL) to a high-power conventional laser with femtosecond accuracy. Our method takes advantage of the same electron bunch…
We show that a laser pulse designed as an adiabatic ramp followed by a kick allows one to reach a perfect postpulse molecular alignment, free of saturation. The mechanism is based on an optimized distribution of the energy between a weakly…
Converting light into matter has been a longstanding goal in physics, particularly the creation of electron-positron pairs through quantum electrodynamic (QED) processes. While current approaches using multiple colliding laser pulses can…
We theoretically analyze the effectiveness of multiple-pulse laser alignment methods for asymmetric-top molecules. As an example, we choose SO_2 and investigate the alignment dynamics induced by two different sequences, each consisting of…
We present experimental results of vacuum laser acceleration (VLA) of electrons using radially polarized laser pulses interacting with a plasma mirror. Tightly focused radially polarized laser pulses have been proposed for electron…
While many-particle entanglement can be found in natural solids and strongly interacting atomic and molecular gases, generating highly entangled states between weakly interacting particles in a controlled and scalable way presents a…
We explore long lived electronic coherences in molecules using shaped ultrafast laser pulses to launch and probe entangled nuclear-electronic wave packets. We find that under certain conditions, the electronic phase remains well defined…
X-ray free-electron lasers (XFELs) are the only sources currently able to produce bright few-fs pulses with tunable photon energies from 100 eV to more than 10 keV. Due to the stochastic SASE operating principles and other technical issues…