Related papers: Strongly aligned gas-phase molecules at Free-Elect…
Alignment and orientation of molecules by intense, ultrashort laser fields are crucial for a variety of applications in physics and chemistry. These include control of high harmonics generation, molecular orbitals tomography, control of…
The paper reports the results of two-dimensional particle-in-cell simulations of proton beam acceleration at the interactions of a 130 fs laser pulse of intensity from the range of 10^21-10^23 W/cm^2, predicted for the Extreme Light…
A strong inhomogeneous static electric field is used to spatially disperse a rotationally cold supersonic beam of 2,6-difluoroiodobenzene molecules according to their rotational quantum state. The molecules in the lowest lying rotational…
This dissertation explores the interaction between high-intensity lasers and plasmas to accelerate electrons and produce radiation via experimental and computational efforts. The laser pulses used in this dissertation have ultrashort…
The present work reports on the generation of short-pulse coherent extreme ultraviolet radiation of controlled polarization. The proposed strategy is based on high-order harmonics generated in pre-aligned molecules. Field-free molecular…
Highly polarized, multi-kiloampere-current electron bunches from compact laser-plasma accelerators are desired for numerous applications. Current proposals to produce these beams suffer from intrinsic limitations to the reproducibility,…
We propose and demonstrate a robust control scheme by ultrafast nonadiabatic chirped laser pulse, designed for targeting coherent superpositions of two-level systems. Robustness against power fluctuation is proved by our numerical study and…
We show that a linear molecule subjected to a short specific elliptically polarized laser field yields postpulse revivals exhibiting alignment alternatively located along the orthogonal axis and the major axis of the ellipse. The effect is…
The alignment dependence of the ionization behavior of H$_2$ exposed to intense ultrashort laser pulses is investigated on the basis of solutions of the full time-dependent Schr\"odinger equation within the fixed-nuclei and dipole…
In this paper, we studied the optimal alignment and anti-alignment of O2 molecules by femtosecond laser pulse under different input energy. The results show that there is an energy limit in molecular alignment. The optimal molecular…
Generation of high-fidelity amplified pulse bursts with a regular interpulse interval yields, in the spectral domain, an equidistant pattern of narrowband spectral modes, similar to frequency combs produced by cw mode-locked lasers, but…
The generation of intense, femtosecond-scale X-ray pulses is crucial for probing matter under extreme temporal and field conditions. Current chirped-pulse amplification (CPA) techniques in free-electron lasers (FELs), however, face…
Singly ionized nitrogen molecules in ambient air pumped by near-infrared femtosecond laser give rise to superradiant emission. Here we demonstrate coherent control of this superradiance by injecting a pair of resonant seeding pulses inside…
Quasi-phase matched direct laser acceleration (DLA) of electrons can be realized with guided, radially polarized laser pulses in density-modulated plasma waveguides. A 3-D particle-in-cell model has been developed to describe the…
The pulse-energy scaling technique electro-optically controlled divided-pulse amplification is implemented in a high-power ultrafast fiber laser system based on coherent beam combination. A fiber-integrated front end and a multi-pass cell…
An investigation of field-free molecular alignment produced by elliptically polarized laser pulses is reported. Experiments are conducted in CO$_2$ at room temperature. A non invasive all-optical technique, based on the cross defocusing of…
Ultra intense lasers are a promising source of energetic ions for various applications. An interesting approach described in Ferri et al. 2019 argues from Particle-in-Cell simulations that using two laser pulses of half energy (half…
We present a 10 mJ-class laser system for seeding petawatt-class Ti:Sa lasers based on a hybrid, femtosecond optical parametric and negatively chirped Ti:Sa-based amplification architecture. Output pulses with 13 mJ energy, 14.4 fs…
The successful operation of X-ray free-electron lasers (FELs), like the Linac Coherent Light Source or the Free-Electron Laser in Hamburg (FLASH), makes unprecedented research on matter at atomic length and ultrafast time scales possible.…
Light-phase-sensitive techniques, such as coherent multidimensional spectroscopy, are well-established in a broad spectral range, already spanning from radio-frequencies in nuclear magnetic resonance spectroscopy to visible and ultraviolet…