Related papers: Strongly aligned gas-phase molecules at Free-Elect…
Experiments were performed to study electron acceleration by intense sub-picosecond laser pulses propagating in sub-mm long plasmas of near critical electron density (NCD). Low density foam layers of 300-500 um thickness were used as…
We describe an instrument which can be used to analyze complex chemical mixtures at high resolution and high sensitivity. Molecules are collisionally cooled with helium gas at cryogenic temperatures (~ 4-7 K), and subsequently detected…
It is demonstrated that strong laser pulses can introduce torsional motion in the axially chiral molecule 3,5-diflouro-3',5'-dibromo-biphenyl (DFDBrBPh). A nanosecond laser pulse spatially aligns the stereogenic carbon-carbon (C-C) bond…
Experimental measurements using the OMEGA EP laser facility demonstrated direct laser acceleration (DLA) of electron beams to (505 $\pm$ 75) MeV with (140 $\pm$ 30)~nC of charge from a low-density plasma target using a 400 J, picosecond…
Recently, the self-modulation scheme of a weakly pre-bunched electron beam has been proposed [Yan et al., Physical Review Letters 126, 084801 (2021)], which is of great promise for high-repetition-rate seeded free-electron lasers (FELs),…
We report experiments on field-free molecular alignment performed at FLASH, the free electron laser (FEL) in Hamburg. The impulsive alignment induced by a 100 fs near-infrared laser pulse in a rotationally cold CO_2 sample is characterized…
Quantum coherent control of ultrafast bond making and the subsequent molecular dynamics is crucial for the realization of a new photochemistry, where a shaped laser field is actively driving the chemical system in a coherent way from the…
This paper describes a 561 nm laser heterodyne interferometer that provides time-resolved measurements of line-integrated plasma electron density within the range of 10^15-10^18 cm^(-2). Such plasmas are produced by railguns on the Plasma…
We propose a novel technique for the creation of maximally entangled symmetric Dicke states in an ion trap using adiabatic passage, which requires only a pair of chirped pulses from a single laser and is applicable to any number of ions and…
The development of a directional, small-divergence, and short-duration picosecond x-ray probe beam with an energy greater than 50 keV is desirable for high energy density science experiments. We therefore explore through particle-in-cell…
We theoretically and numerically analyze x-ray scattering from asymmetric-top molecules three-dimensionally aligned using elliptically polarized laser light. A rigid-rotor model is assumed. The principal axes of the polarizability tensor…
We present a theoretical investigation of coherent control over the orientation of an individual molecule strongly coupled with a cavity using chirped-pulse driving. Specifically, we explore the dynamics of carbonyl sulfide (OCS) molecules…
Typically, in Self-Amplified Spontaneous Emission Free Electron Laser (SASE FEL) based short-pulse schemes, pulse duration is limited by FEL coherence time. For hard X-ray FELs, coherence time is in a few hundred attosecond range while for…
The propensity of molecules to spatially align along the polarization vector of intense, pulsed light fields is related to readily-accessible parameters (molecular polarizabilities, moment of inertia, peak intensity of the light and its…
We report on the nonlinear temporal compression of mJ energy pulses from a Ti:Sa chirped pulse amplifier system in a multipass cell filled with argon. The pulses are compressed from 30 fs down to 5.3 fs, corresponding to two optical cycles.…
A series of simple and low-cost devices for switching, amplifying, and chirping diode lasers based on current modulation are presented. Direct modulation of diode laser currents is rarely sufficient to establish precise amplitude and phase…
We demonstrate the experimental realization of impulsive alignment of carbonyl sulfide (OCS) molecules at the Low Density Matter Beamline (LDM) at the free-electron laser FERMI. OCS molecules in a molecular beam were impulsively aligned…
Laser plasma acceleration at kilohertz repetition rate has recently been shown to work in two different regimes, with pulse lengths of either 30 fs or 3.5 fs. We now report on a systematic study in which a large range of pulse durations and…
An ultrafast fiber chirped-pulse amplifier comprising 8 coherently combined amplifier channels is presented. The laser delivers 1 kW average power at 1 mJ pulse energy and 260 fs pulse duration. Excellent beam quality and low noise…
A two-phase model, where the plasma expansion is an isothermal one when laser irradiates and a following adiabatic one after laser ends, has been proposed to predict the maximum energy of the proton beams induced in the ultra-intense…