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We report detailed temperature-dependent inelastic neutron scattering and ab-initio lattice dynamics investigation of magnetic perovskites YCrO3 and LaCrO3. The magnetic neutron scattering from the Cr ions exhibits significant changes with…

Sodium niobate (NaNbO3) exhibits most complex sequence of structural phase transitions in perovskite family and therefore provides as excellent model system for understanding the mechanism of structural phase transitions. We report…

Materials Science · Physics 2014-06-13 S. K. Mishra , M. K. Gupta , R. Mittal , M. Zbiri , S. Rols , H. Schober , S. L. Chaplot

Local structural measurements have been performed on hexagonal HoMnO3 in order to ascertain the specific changes in bond distances which accompany magnetic ordering transitions. The transition from paramagnetic to the antiferromagetic…

Strongly Correlated Electrons · Physics 2015-05-14 T. A. Tyson , T. Wu , K. H. Ahn , S. Kim , S. -W. Cheong

Hexagonal YMnO$_3$ is well known for the co-occurrence of ferroelectricity and antiferromagnetism at low temperatures. Using temperature-dependent spectroscopic ellipsometry at an $a$-plane oriented single crystal, we show how the…

Materials Science · Physics 2015-03-16 Steffen Richter , Stefan G. Ebbinghaus , Marius Grundmann , Rüdiger Schmidt-Grund

We report on the structural evolution, spin phonon interactions, and magnetoelastic effects in bulk LaFeO3 perovskite across its antiferromagnetic transition. We found that while the lattice constants exhibit slight deviations at the Neel…

We measured phonon dispersion in single crystal EuTiO$_3$ using inelastic x-ray scattering. A structural transition to an antiferrodistortive phase was found at a critical temperature $T_0$=287$\pm$1 K using powder and single-crystal x-ray…

Strongly Correlated Electrons · Physics 2015-06-11 David S. Ellis , Hiroshi Uchiyama , Satoshi Tsutsui , Kunihisa Sugimoto , Kenichi Kato , Daisuke Ishikawa , Alfred Q. R. Baron

We report inelastic neutron scattering measurements of phonon spectra in the parent superconductor iron-tuned chalcogenide Fe$_{1+x}$Te, for two different x contents (x $\leq$ 0.11), using neutron time-of-flight technique. Thermal neutron…

Materials Science · Physics 2017-10-18 Mohamed Zbiri , Romain Viennois

The present work reports the preparation of polycrystalline multiferroic $GdFeO_3$ (GdFO) and characterization with x-ray diffraction (XRD), magnetization, temperature dependent Raman spectroscopy, temperature and magnetic field dependent…

Materials Science · Physics 2021-12-06 Anjali Panchwanee , V. Raghavendra Reddy , Ajay Gupta , V. G. Sathe

Temperature-dependent Raman spectra of TbMnO$_3$ from 5 K to 300 K in the spectral range of 200 to 1525 cm$^{-1}$ show five first-order Raman allowed modes and two high frequency modes. The intensity ratio of the high frequency Raman band…

Strongly Correlated Electrons · Physics 2010-04-12 Pradeep Kumar , Surajit Saha , D. V. S. Muthu , J. R. Sahu , A. K. Sood , C. N. R. Rao

The idea of embedding and transmitting information within the fluctuations of the magnetic moments of spins (spin waves) has been recently proposed and experimentally tested. The coherence of spin waves, which describes how well defined…

The novel ferroelectric-like structural transition observed in metallic LiOsO$_3$ [Y. Shi et al., Nat. Mater. 12, 1024 (2013)], has invoked many theoretical and experimental interests. In this work, we have performed polarized and…

Materials Science · Physics 2017-03-09 Feng Jin , Anmin Zhang , Jianting Ji , Kai Liu , Le Wang , Youguo Shi , Yong Tian , Xiaoli Ma , Qingming Zhang

The coupling between localized spins and phonons can lead to shifts in the dielectric constant of insulating materials at magnetic ordering transitions. Studies on isostructural SeCuO3 (ferromagnetic) and TeCuO3 (antiferromagnetic)…

Materials Science · Physics 2009-04-14 G. Lawes , T. Kimura , C. M. Varma , M. A. Subramanian , R. J. Cava , A. P. Ramirez

We present neutron inelastic scattering measurements of the low-energy phonons in single crystal BiFeO3. The dispersions of the three acoustic phonon modes (LA along [100], TA1 along [010] and TA2 along [110]) and two low energy optic…

Layered antiferromagnetic materials have emerged as a novel subset of the two-dimensional family providing a highly accessible regime with prospects for layer-number-dependent magnetism. Furthermore, transition metal phosphorous…

Materials Science · Physics 2024-01-09 Daniel J. Gillard , Daniel Wolverson , Oscar M. Hutchings , Alexander I. Tartakovskii

Temperature dependence of longitudinal optical phonons with oxygen character was measured in La1-xSrxMnO3 (x=0.2, 0.3) by inelastic neutron scattering in the (1 0 0) cubic direction. The zone center mode intensity is consistent with the…

Strongly Correlated Electrons · Physics 2007-05-23 D. Reznik , W. Reichardt

We have measured the optical conductivity of single crystal LuMnO3 from 10 to 45000 cm-1 at temperatures between 4 and 300 K. A symmetry allowed on-site Mn $d$-$d$ transition near 1.7 eV is observed to blue shift (~0.1 eV) in the…

Strongly Correlated Electrons · Physics 2009-11-07 A. B. Souchkov , J. R. Simpson , H. D. Drew , M. Quijada , H. Ishibashi , N. Hur , J. S. Ahn , S. W. Cheong , A. J. Millis

We perform thermodynamic and inelastic neutron scattering (INS) measurements to study the lattice dynamics (phonons) of a cubic collinear antiferromagnet Cu$_3$TeO$_6$ which hosts topological spin excitations (magnons). While the specific…

We present a systematic study of the structure and lattice dynamics at room temperature, and the phonon behavior at low temperatures in orthorhombic Gd$_{1-x}$Y$_{x}$MnO$_{3}$ manganites, with 0 $\leq$ x $\leq$ 0.4, using powder x-ray…

Strongly Correlated Electrons · Physics 2014-12-31 R. Vilarinho , E. C. Queirós , A. Almeida , P. B. Tavares , J. Agostinho Moreira

Raman scattering experiments have been carried out on single crystals of Nd$_{0.5}$Sr$_{0.5}$MnO$_3$ as a function of temperature in the range of 320-50 K, covering the paramagnetic insulator-ferromagnetc metal transition at 250 K and the…

Materials Science · Physics 2007-05-23 Md. Motin Seikh , A. K. Sood , Chandrabhas Narayana

To understand spin interactions in materials of the Cu$_2$Sb structure type, inelastic neutron scattering of Fe$_2$As single crystals was examined at different temperatures and incident neutron energies. The experimental phonon spectra…