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Inelastic neutron scattering experiments combining time-of-flight and polarized techniques yield a comprehensive picture of the magnon dispersion in multiferroic TbMnO3 including the dynamic chirality. Taking into account only Mn3+ moments,…

Strongly Correlated Electrons · Physics 2024-02-27 S. Holbein , P. Steffens , S. Biesenkamp , J. Ollivier , A. C. Komarek , M. Baum , M. Braden

We report complex dielectric and Raman spectroscopy measurements in four samples of $\alpha$- Fe$_2$O$_3$, consisting of crystallites which are either hexagonal shaped plates or cuboids. All four samples exhibit the spin reorientation…

Strongly Correlated Electrons · Physics 2019-04-17 Namrata Pattanayak , Jitender Kumar , Partha Pratim Patra , G. V. Pavan Kumar , Ashna Bajpai

Iron manganese trioxide (Fe0.25Mn0.75)2O3 nanocrystals were synthesized by the sol-gel method. The 80 K Mossbauer spectrum was well-fitted using two doublets representing the 8b and 24d crystallographic sites of the (FexMn1-x)2O3 phase and…

Temperature dependent inelastic neutron-scattering measurements of the generalized phonon density-of-states for superconducting MgCNi_3, T_c=8 K, give evidence for a soft-mode behavior of low-frequency Ni phonon modes. Results are compared…

Superconductivity · Physics 2009-11-10 R. Heid , B. Renker , H. Schober , P. Adelmann , D. Ernst , K. -P. Bohnen

We report a comprehensive study of the low-level substitution of Mn$^{3+}$ by Fe$^{3+}$ effect on the static and dynamic magnetoelectric coupling in TbMn$_{1-x}$Fe$_x$O$_3$ ($x=0$, 0.02 and 0.04). The cationic substitution has a large…

Materials Science · Physics 2023-03-14 A. Maia , R. Vilarinho , C. Kadlec , M. Lebeda , M. Mihalik, , M. Zentková , M. Mihalik , J. Agostinho Moreira , S. Kamba

High-frequency dielectric studies of Bi_0.85Nd_0.15FeO_3 ceramics performed betweeen 100 and 900 K reveal hardening of most polar phonons on cooling below antiferroelectric phase transition, which occurs near 600 K. Moreover, a strong THz…

Materials Science · Physics 2011-10-18 V. Goian , S. Kamba , S. Greicius , D. Nuzhnyy , S. Karimi , I. M. Reaney

Spectral ellipsometry has been used to determine the dielectric function of an untwinned crystal of LaMnO_3 in the spectral range 0.5-5.6 eV at temperatures 50 K < T < 300 K. A pronounced redistribution of spectral weight is found at the…

Strongly Correlated Electrons · Physics 2009-11-10 N. N. Kovaleva , A. V. Boris , C. Bernhard , A. Kulakov , A. Pimenov , A. M. Balbashov , G. Khaliullin , B. Keimer

Spin correlations in the pyrochlore antiferromagnet Y_2Ru_2O_7 with Curie-Weiss temperature $\Theta_{CW}=-1100$ K and critical temperature T_N=77 K were examined through neutron scattering. For $T_N<T<\Theta_{CW}/3$ the data show spin…

Strongly Correlated Electrons · Physics 2014-07-03 J. van Duijn , N. Hur , J. W. Taylor , Y. Qiu , Q. Z. Huang , S. -W. Cheong , C. Broholm , T. G. Perring

The wide band gap semiconductor \b{eta}-Ga2O3 shows promise for applications in high-power and high-temperature electronics. The phonons of \b{eta}-Ga2O3 play a crucial role in determining its important material characteristics for these…

Materials Science · Physics 2019-02-08 K. A. Mengle , E. Kioupakis

We show that in YVO3 new hard phonons gradually become zone center active below ~210 K verifying that a lattice phase transition takes place at about that temperature. The Debye-Waller factor found from EXAFS measurements show an additional…

K$_3$-picene is a superconducting molecular crystal with critical temperature T$_c=7$K or 18K, depending on preparation conditions. Using density functional theory we show that electron-phonon interaction accounts for T$_c ~ 3-8$ K. The…

Superconductivity · Physics 2015-05-28 Michele Casula , Matteo Calandra , Gianni Profeta , Francesco Mauri

We report new results of a 57Fe M\"ossbauer study of multiferroic 3R-AgFeO2 powder samples performed in a wide temperature range, including two points, TN1 ~ 14 K and TN2 ~ 9 K, of magnetic phase transitions. At the intermediate temperature…

We report on THz absorption spectroscopy combined with high magnetic fields of polycrystalline RCrO3 (R= Pr, Sm, Er) aiming understanding spin wave resonances at their low temperature magnetic phases. Our measurements show that the…

The infrared and Terahertz properties of GdMnO_3 have been investigated as function of temperature and magnetic field, with special emphasis on the phase boundary between the incommensurate and the canted antiferromagnetic structures. The…

Strongly Correlated Electrons · Physics 2007-05-23 A. Pimenov , T. Rudolf , F. Mayr , A. Loidl , A. A. Mukhin , A. M. Balbashov

We present a quantitative analysis of the phonon lineshapes obtained by neutron inelastic scattering methods in the relaxor ferroelectric Pb(Mg1/3Nb2/3)O3 (PMN). Differences in the shapes and apparent positions of the transverse acoustic…

Materials Science · Physics 2009-11-07 S. Wakimoto , C. Stock , Z. -G. Ye , W. Chen , P. M. Gehring , G. Shirane

We report the temperature dependent THz to mid-infrared response of hexagonal-ErMnO3 using absorption, reflectivity, and emissivity techniques from 2 K to 1700 K. At low temperatures, lowest frequency vibrational modes coexist with…

We report on infrared, Raman, magnetic susceptibility, and specific heat measurements on CdCr2O4 and ZnCr2O4 single crystals. We estimate the nearest-neighbor and next-nearest neighbor exchange constants from the magnetic susceptibility and…

Strongly Correlated Electrons · Physics 2010-02-03 Ch. Kant , J. Deisenhofer , T. Rudolf , F. Mayr , F. Schrettle , A. Loidl , V. Gnezdilov , D. Wulferding , P. Lemmens , V. Tsurkan

We present the results of pressure-dependent far-infrared reflectivity measurements on the multiferroic perovskite BiFeO3 at room temperature. The observed behavior of the infrared-active phonon modes as a funtion of pressure clearly…

Other Condensed Matter · Physics 2007-12-06 A. Pashkin , K. Rabia , S. Frank , C. A. Kuntscher , R. Haumont , R. Saint-Martin , J. Kreisel

The infrared (IR) reflectivity spectra of orthorhombic manganese perovskites PrMnO$_3$ and CaMnO$_3$ are studied in the frequency range of optical phonon modes at temperatures varying from 300 to 4 K. The IR phonon spectra of these two…

Materials Science · Physics 2015-05-13 R. Sopracase , G. Gruener , E. Olive , J. C. Soret

The equilibrium ground-state structure of LiNbO3 in the paraelectric and ferroelectric phases is fully optimized in a first-principles calculation using the full-potential linearized augmented plane wave method. The equilibrium volume, c/a…

Materials Science · Physics 2007-05-23 A. V. Postnikov , V. Caciuc , G. Borstel
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