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Cd(Se,Te) Quantum Dots (QD) in ZnSe barrier typically exhibit a very high spectral density, which precludes investigation of single dot photoluminescence. We design, grow and study individual Cd(Se,Te)/ZnSe QDs of low spectral density of…

Atomically flat semiconductor nanostructures have sharp photoluminescence emission, short radiative lifetimes and a well-defined planar structure. However, these nanostructures lack the optical and electronic fine-tuning that justify…

Materials Science · Physics 2015-09-29 Sébastien Lamarre , Étienne Rochette , Samuel Tremblay , Claudine Nì. Allen

Colloidal Cadmium Selenide (CdSe) nanoplatelets (NPLs) are a recently developed class of efficient luminescent nanomaterial suitable for optoelectronic device applications. A change in temperature greatly affects their electronic…

Mesoscale and Nanoscale Physics · Physics 2017-10-26 Sumanta Bose , Sushant Shendre , Zhigang Song , Vijay Kumar Sharma , Dao Hua Zhang , Cuong Dang , Weijun Fan , Hilmi Volkan Demir

The Si/SiGe heterosystem would be ideally suited for the realization of complementary metal-oxide-semiconductor (CMOS)-compatible integrated light sources, but the indirect band gap, exacerbated by a type-II band offset, makes it…

We demonstrate experimental results based on time-resolved photoluminescence spectroscopy to determine the oscillator strength (OS) and the internal quantum efficiency (IQE) of InGaAs quantum dots (QDs). Using a strain-reducing layer (SRL)…

Applied Physics · Physics 2021-08-24 Jan Große , Pawel Mwrowinski , Nicole Srocka , Stephan Reitzenstein

Colloidal quantum dots (QDs) are an attractive medium for nonlinear optics and deterministic heterogeneous integration with photonic devices. Their intrinsic nonlinearities can be strengthened further by coupling QDs to low mode-volume…

A first-principles study of small CdnSen Quantum Dots (QD) ('n' =6, 12, 13, and 33) has been performed for application to QD solar cell development. We separately assess the effects of the particle size and the passivating ligands upon the…

Mesoscale and Nanoscale Physics · Physics 2013-08-22 Shanshan Wu , Michael McGuigan , Amanda L. Tiano , Stanislaus S. Wong , James G. Glimm

Optical properties of multilayer semi-conductor nano-emitters are crucially dependent on the relative energy levelsof their different components. For core/shell quantum dots, the relative energy difference between conduction bandedge of…

Quantum confinement profoundly affects the properties and interactions of electrons, holes, and excitons in nanomaterials. We apply first-principles calculations to study the effects of extreme quantum confinement on the electronic,…

Materials Science · Physics 2019-10-07 Dylan Bayerl , Emmanouil Kioupakis

Due to their band-structure and optical properties, InAs/InP quantum dots (QDs) constitute a promising system for single-photon generation at third telecom window of silica fibers and for applications in quantum communication networks.…

Mesoscale and Nanoscale Physics · Physics 2020-05-20 P. Holewa , M. Gawełczyk , C. Ciostek , P. Wyborski , S. Kadkhodazadeh , E. Semenova , M. Syperek

We show that molecular aggregation can strongly influence the nonradiative decay (NRD) lifetime of an electronic excitation. As a demonstrative example, we consider a transition-dipole-dipole-interacting dimer whose monomers have harmonic…

Chemical Physics · Physics 2017-11-01 A. Celestino , A. Eisfeld

This study presents a comprehensive investigation of chemical, structural, and magnetic properties of Ti/Ni multilayer systems with period thicknesses of 4 nm and 10 nm. Particular attention was paid to the characterization of the…

Semiconductor quantum dots (QDs) provide an essential link between light and matter in emerging fields such as light-harvesting, all-solid-state quantum communication, and quantum computing. QDs are excellent single-photon sources and can…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 Mads Lykke Andersen , Søren Stobbe , Anders Søndberg Sørensen , Peter Lodahl

Transition metal dichalcogenide (TMD) nanoscrolls (NS) exhibit significant photoluminescence (PL) signals despite their multilayer structure, which cannot be explained by the strained multilayer description of NS. Here, we investigate the…

Layered transition metal dichalcogenides (TMDs) provide an ideal platform for exploring the effects of dimensionality on correlated electronic phases such as charge density wave (CDW) order. When TMDs are reduced in thickness to the 2-D…

Mesoscale and Nanoscale Physics · Physics 2016-11-03 Linjun Li , WeiJie Zhao , Bo Liu , Tianhua Ren , Goki Eda , Kianping Loh

We report the ultrafast and large third-order nonlinear optical properties of CdS nanocrystals (NCs) embedded in a polymeric film. The CdS NCs of 2-nm radius are synthesized by an ion exchange method and highly concentrated in the two…

Materials Science · Physics 2007-05-23 J. He , W. Ji , G. H. Ma , S. H. Tang , E. S. W. Kong , S. Y. Chow , X. H. Zhang , Z. L. Hua , J. L. Shi

We report on the optical characterization of non-polar a-plane InGaN quantum dots (QDs) grown by metal-organic vapor phase epitaxy using a short nitrogen anneal treatment at the growth temperature. Spatial and spectral mapping of…

We report a systematic empirical study of nanoparticle internalization into cells via non-specific pathways. The nanoparticles were comprised of commercial quantum dots (QDs) that were highly visible under a fluorescence confocal…

Biological Physics · Physics 2010-06-30 T A Kelf , V K A Sreenivasan , J Sun , E J Kim , E M Goldys , A V Zvyagin

In this review we discuss several fundamental processes taking place in semiconductor nanocrystals (quantum dots, QDs) when their electron subsystem interacts with electromagnetic (EM) radiation. The physical phenomena of light emission and…

Mesoscale and Nanoscale Physics · Physics 2021-01-12 Vladimir A. Burdov , Mikhail I. Vasilevskiy

Over the past two decades, epitaxial semiconductor quantum dots (QDs) have demonstrated very promising properties as sources of single photons and entangled photons on-demand. Among different growth methods, droplet etching epitaxy has…