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Related papers: Anomalous valley polarization in monolayer MoSe2

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Single layers of MoS2 and MoSe2 were optically pumped with circularly polarized light and an appreciable polarization was initialized as the pump energy was varied. The circular polarization of the emitted photoluminescence was monitored as…

Materials Science · Physics 2016-02-02 George Kioseoglou , Aubrey T. Hanbicki , Marc Currie , Adam L. Friedman , Berend T. Jonker

We report on the influence of a photochemical doping method on the spin-valley polarization degree ($P_{c}$) of excitons in WSe$_2$ monolayers. By varying the carrier density and transitioning from an excess of electrons (n-type) to an…

Chiral interaction between light and two-dimensional transition metal dichalcogenides (2D-TMDs) has recently drawn enormous scientific attention. The optical selection rules of these atomically thin semiconductors allow the attribution of a…

Optics · Physics 2021-06-08 Irina Komen , Sabrya E. van Heijst , Sonia Conesa-Boj , L. Kuipers

For a long time, two-dimensional (2D) hexagonal MoS2 was proposed as a promising material for valleytronic system. However, the limited size of growth and low carrier motilities in MoS2 restrict its further application. Very recently, a new…

Materials Science · Physics 2021-01-27 Chen Yang , Zhigang Song , Xiaotian Sun , Jing Lu

The optical selection rules obeyed by two-dimensional materials with spin-valley coupling enable the selective excitation of carriers. We show that six members of the monolayer MA2Z4 (M = Mo and W; A = C, Si, and Ge; Z = N, P, and As)…

Materials Science · Physics 2022-06-15 Jiaren Yuan , Qingyuan Wei , Minglei Sun , Xiaohong Yan , Yongqing Cai , Lei Shen , Udo Schwingenschlögl

Semiconducting transition metal dichalcogenide monolayers have emerged as promising candidates for future valleytronics-based quantum information technologies. Two distinct momentum-states of tightly-bound electron-hole pairs in these…

Mesoscale and Nanoscale Physics · Physics 2017-03-16 Gerd Plechinger , Tobias Korn , John M. Lupton

Recently, altermagnets demonstrate numerous newfangle physical phenomena due to their inherent antiferromagnetic coupling and spontaneous spin splitting, that are anticipated to enable innovative spintronic devices. However, the rare…

Materials Science · Physics 2025-04-28 Xin Hu , Weihang Zhao , Wenjun Xia , Hanbo Sun , Chao Wu , Yin-Zhong Wu , Ping Li

We report an experimental study of the magnetic-field dependence of the optically pumped valley polarization in an epitaxial tungsten diselenide (WSe$_2$) monolayer grown by molecular-beam epitaxy (MBE) on a hexagonal boron nitride (hBN)…

Monolayers of transition metal dichalcogenides (TMDCs) are atomically thin direct-gap semiconductors with potential applications in nanoelectronics, optoelectronics, and electrochemical sensing. Recent theoretical and experimental efforts…

Mesoscale and Nanoscale Physics · Physics 2013-02-26 Sanfeng Wu , Chunming Huang , Grant Aivazian , Jason S Ross , David H Cobden , Xiaodong Xu

The direct gap interband transitions in transition metal dichalcogenides monolayers are governed by chiral optical selection rules. Determined by laser helicity, optical transitions in either the $K^+$ or $K^-$ valley in momentum space are…

Mesoscale and Nanoscale Physics · Physics 2016-10-26 G. Wang , X. Marie , B. L. Liu , T. Amand , C. Robert , F. Cadiz , P. Renucci , B. Urbaszek

The valley degree of freedom of electrons in materials promises routes toward energy-efficient information storage with enticing prospects towards quantum information processing. Current challenges in utilizing valley polarization are…

We calculate linear and nonlinear optical susceptibilities arising from the excitonic states of mono- layer MoS2 for in-plane light polarizations, using second-quantized bound and unbound exciton operators. Optical selection rules are…

Mesoscale and Nanoscale Physics · Physics 2018-04-11 Daniel B. S. Soh , Christopher Rogers , Dodd J. Gray , Eric Chatterjee , Hideo Mabuchi

The modulation of the valley structure in two-dimensional valley materials is vital in the field of valleytronics. The multiferroicity provides possibility for multiple modulations of the valley, including the magnetic and electric means.…

Materials Science · Physics 2023-07-10 Huiqian Wang , Li Liang , Xiaohui Wang , Xiaoyu Wang , Xiao Li

We report circularly-polarized optical reflection spectroscopy of monolayer WS$_2$ and MoS$_2$ at low temperatures (4~K) and in high magnetic fields to 65~T. Both the A and the B exciton transitions exhibit a clear and very similar Zeeman…

Mesoscale and Nanoscale Physics · Physics 2016-02-11 Andreas V. Stier , Kathleen M. McCreary , Berend T. Jonker , Junichiro Kono , Scott A. Crooker

We investigate the valley related carrier dynamics in monolayer MoS2 using helicity resolved non-degenerate ultrafast pump-probe spectroscopy at the vicinity of the high-symmetry K point under the temperature down to 78 K. Monolayer MoS2…

Optics · Physics 2014-05-08 Qinsheng Wang , Shaofeng Ge , Xiao Li , Jun Qiu , Yanxin Ji , Ji Feng , Dong Sun

We have investigated the valley degeneracy of MoS2 multilayers and its effect on thermoelectric properties. By modulating the layer thickness and external electric field, the hole valleys at {\Gamma} and K points in the highest energy…

Materials Science · Physics 2016-02-03 Jisook Hong , Changhoon Lee , Jin-Seong Park , Ji Hoon Shim

Valley polarization is amongst the most critical attributes of atomically thin materials. However, achieving a high contrast from monolayer transition metal dichalcogenides (TMDs) has so far been challenging. In this work, a giant valley…

Monolayer 2D semiconductors provide an attractive option for valleytronics due to the valley-addressability by helicity-specific light beam. But the short valley lifetime for excitons have hindered potential valleytronic applications. In…

Mesoscale and Nanoscale Physics · Physics 2022-08-17 Qiyao Zhang , Hao Sun , Jiacheng Tang , Xingcan Dai , Zhen Wang , Cun-Zheng Ning

In van der Waals heterostructures (HS) consisting of stacked MoSe$_2$ and WSe$_2$ monolayers, optically bright interlayer excitons (ILE) can be observed when the constituent layers are crystallographically aligned. The symmetry of the…

Valley pseudospin in two-dimensional (2D) transition-metal dichalcogenides (TMDs) allows optical control of spin-valley polarization and intervalley quantum coherence. Defect states in TMDs give rise to new exciton features and…

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