English
Related papers

Related papers: Dynamic nuclear polarization as kinetically constr…

200 papers

By using highly time-resolved spectroscopy with an alternative {\sigma}+/{\sigma} - laser pulse modulation technique, we are able to measure the fast buildup and decay times of the dynamical nuclear spin polarization (DNSP) at 5 K for a…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 X. M. Dou , B. Q. Sun , D. S. Jiang , H. Q. Ni , Z. C. Niu

Nuclear spin polarization can be pumped into spin-blocked quantum dots by multiple Landau- Zener passages through singlet-triplet anticrossings. By numerical simulations of realistic systems including approximately $10^7$ nuclear spins…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Arne Brataas , Emmanuel I. Rashba

We introduce a novel NMR approach that extends the capabilities of indirect dynamic nuclear polarization (DNP) under magic-angle spinning to probe the local environment of half-integer spin quadrupolar nuclei. Compared to…

We observe multiple stable states of nuclear polarization in a double quantum dot under conditions of electron spin resonance. The stable states can be understood within an elaborated theoretical rate equation model for the polarization in…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 J. Danon , I. T. Vink , F. H. L. Koppens , K. C. Nowack , L. M. K. Vandersypen , Yu. V. Nazarov

We propose a nuclear-spin-polarization protocol in a general evolution-and-measurement framework. The protocol works in a spin-star configuration, where the central spin is coupled to the surrounding bath (nuclear) spins by flip-flop…

Quantum Physics · Physics 2022-12-07 Zhu-yao Jin , Jia-shun Yan , Jun Jing

Hyperpolarized nanoparticles (NPs) offer high polarization levels with room temperature relaxation times exceeding half an hour. In this work, we demonstrate that the achievable hyperpolarization enhancement and relaxation (decay) time at…

The interplay of dynamical nuclear polarization (DNP) and leakage current through a double quantum dot in the spin-blockade regime is analyzed. A finite DNP is built up due to a competition between hyperfine (HF) spin-flip transitions and…

Mesoscale and Nanoscale Physics · Physics 2013-07-30 Anders Mathias Lunde , Carlos López-Monís , Ioanna A. Vasiliadou , Luis L. Bonilla , Gloria Platero

Dynamic polarization protocols aim to hyperpolarize a spin bath by transferring spin polarization from a well-controlled qubit such as a quantum dot or a color defect. Building on techniques from shortcuts to adiabaticity, we design fast…

Quantum Physics · Physics 2021-02-17 Tamiro Villazon , Pieter W. Claeys , Anatoli Polkovnikov , Anushya Chandran

We report record high Si-29 spin polarization obtained using dynamic nuclear polarization in microcrystalline silicon powder. Unpaired electrons in this silicon powder are due to dangling bonds in the amorphous region of this intrinsically…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 A. E. Dementyev , D. G. Cory , C. Ramanathan

The inhomogeneous distribution of P1 centers in type 1b HPHT diamond samples allows multiple DNP mechanisms to occur within the same crystal, resulting in complex DNP spectra. At some crystal orientations, different DNP mechanisms can…

Chemical Physics · Physics 2025-12-19 Brendan C. Sheehan , Margaret Hubble , Daphna Shimon , Chandrasekhar Ramanathan

A highly asymmetric dynamic nuclear spin pumping is observed in a single self assembled InGaAs quantum dot subject to resonant optical pumping of the neutral exciton transition leading to a large maximum polarization of 54%. This dynamic…

Mesoscale and Nanoscale Physics · Physics 2010-09-30 F. Klotz , V. Jovanov , J. Kierig , E. C. Clark , M. Bichler , G. Abstreiter , M. S. Brandt , J. J. Finley , H. Schwager , G. Giedke

Dynamic nuclear polarization enables the hyperpolarization of nuclear spins beyond the thermal-equilibrium Boltzmann distribution. However, it is often unclear why the experimentally measured hyperpolarization is below the theoretical…

Chemical Physics · Physics 2023-12-13 Gevin von Witte , Aaron Himmler , Sebastian Kozerke , Matthias Ernst

The influence of the core polarization on the effective nuclear interaction of asymmetric nuclear matter is calculated in the framework of the induced interaction theory. The strong isospin dependence of the density and spin density…

Nuclear Theory · Physics 2016-05-25 S. S. Zhang , L. G. Cao , U. Lombardo , P. Schuck

We analyze electron spin relaxation in electronic transport through coherently coupled double quantum dots in the spin blockade regime. In particular, we focus on hyperfine interaction as the spin relaxation mechanism. We pay special…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 Carlos López-Monís , Jesús Iñarrea , Gloria Platero

We study dynamic polarization and resistive detection of nuclear spins in a semiconductor quantum dot (QD) under the Kondo effect regime. We find that the differential conductance spectra of the QD exhibit hysteresis under the Kondo effect…

Mesoscale and Nanoscale Physics · Physics 2013-02-19 Minoru Kawamura , Daniel Gottwald , Keiji Ono , Tomoki Machida , Kimitoshi Kono

The nuclear spin fluctuations (NSF) as well as the dynamic nuclear polarization (DNP) and their effects on the electron spins in negatively charged (In,Ga)As/GaAs quantum dots have been studied by polarized pump-probe and photoluminescence…

Nuclear ground state and collective excitation properties provide a means to probe the nuclear matter equation of state and establish connections between observables in finite nuclei and neutron stars. Specifically, the electric dipole…

Nuclear Theory · Physics 2026-01-07 P. S. Koliogiannis , E. Yuksel , T. Ghosh , N. Paar

The interaction of condensed phase systems with external electric fields is crucial in myriad processes in nature and technology ranging from the field-directed motion of cells (galvanotaxis), to energy storage and conversion systems…

Chemical Physics · Physics 2024-09-25 Kit Joll , Philipp Schienbein , Kevin M. Rosso , Jochen Blumberger

We theoretically study the nuclear spin dynamics driven by electron transport and hyperfine interaction in an electrically-defined double quantum dot (DQD) in the Pauli-blockade regime. We derive a master-equation-based framework and show…

Mesoscale and Nanoscale Physics · Physics 2014-06-03 Martin J. A. Schuetz , Eric M. Kessler , Lieven M. K. Vandersypen , J. Ignacio Cirac , Geza Giedke

After initial proof-of-principle demonstrations, optically pumped nitrogen-vacancy (NV) centres in diamond have been proposed as a non-invasive platform to achieve hyperpolarisation of nuclear spins in molecular samples over macroscopic…

Mesoscale and Nanoscale Physics · Physics 2021-01-27 J. -P. Tetienne , L. T. Hall , A. J. Healey , G. A. L. White , M. -A. Sani , F. Separovic , L. C. L. Hollenberg