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Optically-pumped color centers in semiconductor powders can potentially induce high levels of nuclear spin polarization in surrounding solids or fluids at or near ambient conditions, but complications stemming from the random orientation of…

We present an enhanced diffusion of nuclear spin polarization in fractional quantum Hall domain phases at $\nu = 2/3$. Resistively-detected NMR mediated by electrically driven domain-wall motion is used as a probe of local nuclear…

Mesoscale and Nanoscale Physics · Physics 2016-05-24 S. Miyamoto , T. Hatano , S. Watanabe , Y. Hirayama

We study repeated (noncontinuous) measurements on the electron spin in a quantum dot and find that the measurement technique may lead to a different met$ or mechanism to realize nuclear spin polarization. While it may be used in any case,…

Quantum Physics · Physics 2011-07-28 Lian-Ao Wu

High-fidelity multi-qubit initialization is vital for quantum simulation, quantum information processing (QIP), and quantum sensing. In diamond platforms, nuclear spin registers can be initialized through polarization transfer from a nearby…

Quantum Physics · Physics 2026-03-02 Soham Pal , Oliver T. Whaites , Wolfgang Knolle , Tania S. Monteiro , Helena S. Knowles

Most of dynamic nuclear polarization (DNP) has been requiring helium cryogenics and strong magnetic fields for a high degree of polarization. In this work, we instead demonstrate an optical hyperpolarization of naturally abundant $^{13}$C…

Current-induced electron spin polarization is shown to produce nuclear hyperpolarization through dynamic nuclear polarization. Saturated fields of several millitesla are generated upon the application of electric field over a timescale of a…

Mesoscale and Nanoscale Physics · Physics 2014-10-31 C. J. Trowbridge , B. M. Norman , Y. K. Kato , D. D. Awschalom , V. Sih

Dynamic nuclear polarization (DNP) enhanced nuclear magnetic resonance (NMR) offers a promising route to studying local atomic environments at the surface of both crystalline and amorphous materials. We take advantage of unpaired electrons…

Nuclear-spin diffusion in double quantum wells (QWs) is examined by using dynamic nuclear polarization (DNP) at a Landau level filling factor $\nu=2/3$ spin phase transition (SPT). The longitudinal resistance increases during the DNP of one…

Mesoscale and Nanoscale Physics · Physics 2015-04-01 T. Hatano , W. Kume , S. Watanabe , K. Akiba , K. Nagase , Y. Hirayama

Understanding the joint dynamics of electron and nuclear spins is central to core concepts in solid-state magnetic resonance - such as spin-lattice relaxation and dynamic nuclear polarization - but a generalization that capitalizes on…

Quantum Physics · Physics 2021-06-16 Santiago Bussandri , Pablo R. Zangara , Rodolfo H. Acosta , Carlos A. Meriles

Understanding fully the dynamics of coupled electron-nuclear spin systems, which are important for the development of long-lived qubits based on solid-state systems, remains a challenge. We show that in a singly charged semiconductor…

Mesoscale and Nanoscale Physics · Physics 2010-07-26 Wenxian Zhang , Jian-Liang Hu , Jun Zhuang , J. Q. You , Ren-Bao Liu

The polarisation dynamics of nuclear spins weakly coupled to an NV center is highly sensitive to the parameters of the microwave control and the nuclear Larmor frequency. What is commonly regarded as a challenge, we propose here as a…

Quantum Physics · Physics 2018-10-24 Q. Chen , Z. -Y. Wang , B. Tratzmiller , I. Schwartz , M. B. Plenio

Direct dynamic nuclear polarization of 1H nuclei in frozen water and water-ethanol mixtures is demonstrated using silicon nanoparticles as the polarizing agent. Electron spins at dangling-bond sites near the silicon surface are identified…

Mesoscale and Nanoscale Physics · Physics 2014-01-14 M. C. Cassidy , C. Ramanathan , D. G. Cory , J. W. Ager , C. M. Marcus

We investigate the dynamic nuclear polarization from the hyperfine interaction between nonequilibrium electronic spins and nuclear spins coupled to them in semiconductor nanostructures. We derive the time and position dependence of the…

Materials Science · Physics 2007-05-23 Ionel Tifrea , Michael E. Flatte

We theoretically investigate the dynamical nuclear spin polarization in a quantum point contact (QPC) at finite magnetic field. We find that when the QPC is tuned to be spin selective, at the conductance of e^2/h, a finite bias induces a…

Mesoscale and Nanoscale Physics · Physics 2018-03-20 Peter Stano , Tomosuke Aono , Minoru Kawamura

We consider the problem of determining the spectrum of an electronic spin via polarization transfer to coupled nuclear spins and their subsequent readout. This suggests applications for employing dynamic nuclear polarization (DNP) for…

Quantum Physics · Physics 2021-10-19 Moniish Elanchezhian , Arjun Pillai , Teemu Virtanen , Ashok Ajoy

Low thermal polarization of nuclear spins is a primary sensitivity limitation for nuclear magnetic resonance. Here we demonstrate optically pumped (microwave-free) nuclear spin polarization of $^{13}\mathrm{C}$ and $^{15}\mathrm{N}$ in…

Mesoscale and Nanoscale Physics · Physics 2017-08-09 Ben L. Green , Ben G. Breeze , Gregory J. Rees , John V. Hanna , Jyh-Pin Chou , Viktor Ivády , Adam Gali , Mark E. Newton

Dynamical magnetic and nuclear polarization in complex spin systems is discussed on the example of transfer of spin from exciton to the central spin of magnetic impurity in a quantum dot in the presence of a finite number of nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Ramin M. Abolfath , Anna Trojnar , Bahman Roostaei , Thomas Brabec , Pawel Hawrylak

We implement several non-binary logic systems using the spin dynamics of nuclear spins in nuclear magnetic resonance (NMR). The NMR system is a suitable test system because of its high degree of experimental control; findings from NMR…

Emerging Technologies · Computer Science 2015-12-03 Pedro M. Aguiar , Robert Hornby , Cameron McGarry , Simon O'Keefe , Angelika Sebald

Nuclear spin hyperpolarization provides a promising route to overcome the challenges imposed by the limited sensitivity of nuclear magnetic resonance. Here we demonstrate that dissolution of spin-polarized pentacene-doped naphthalene…

By applying a new technique for dynamic nuclear polarization involving simultaneous excitation of electronic and nuclear transitions, we have enhanced the nuclear polarization of the nitrogen nuclei in 15N@C60 by a factor of 1000 at a fixed…

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