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The ability to initialise nuclear spins, which are typically in a mixed state even at low temperature, is a key requirement of many protocols used in quantum computing and simulations as well as in magnetic resonance spectroscopy and…

Quantum Physics · Physics 2018-10-02 J. E. Lang , J. -P. Tetienne , T. S. Monteiro

We demonstrate a way to polarize and detect nuclear spin in a gate-defined quantum point contact operating at high Landau levels. Resistively-detected Nuclear Magnetic Resonance (RDNMR) can be achieved up to the $5$th Landau level and at a…

Mesoscale and Nanoscale Physics · Physics 2018-06-06 M. H. Fauzi , A. Noorhidayati , M. F. Sahdan , K. Sato , K. Nagase , Y. Hirayama

Resonant optical excitation of lowest-energy excitonic transitions in self-assembled quantum dots lead to nuclear spin polarization that is qualitatively different from the well known optical orientation phenomena. By carrying out a…

Mesoscale and Nanoscale Physics · Physics 2014-10-03 A. Högele , M. Kroner , C. Latta , M. Claassen , I. Carusotto , C. Bulutay , A. Imamoglu

We theoretically investigate dynamic nuclear spin polarization in a self-assembled quantum dot pumped optically by two laser beams. With the assumption that a noncollinear interaction between the hole spin and nuclear spins leads to nuclear…

Mesoscale and Nanoscale Physics · Physics 2013-06-07 Xiao-Feng Shi

This study explores, both theoretically and experimentally, the photochemically induced dynamic nuclear polarization (photo-CIDNP) of 19F nuclei, the associated spin relaxation, cross-relaxation and cross-correlation effects, as well as…

Chemical Physics · Physics 2011-04-28 Ilya Kuprov

Distant dipolar field (DDF)-based nuclear magnetic resonance is an active research area with many fundamental properties still not well understood. Already several intriguing applications have developed, like HOMOGENIZED and IDEAL…

Medical Physics · Physics 2009-09-29 Curtis Andrew Corum

A novel mathematical treatment is proposed for computing the time evolution of dynamic nuclear polarization processes in the low temperature thermal mixing regime. Without assuming any a priori analytical form for the electron polarization,…

Statistical Mechanics · Physics 2017-08-23 Sonia Colombo Serra , Alberto Rosso , Fabio Tedoldi

The integration on a single chip of the sensitivity-relevant electronics of nuclear magnetic resonance (NMR) and electron spin resonance (ESR) spectrometers is a promising approach to improve the limit of detection, especially for samples…

Instrumentation and Detectors · Physics 2020-03-09 Nergiz Sahin Solmaz , Marco Grisi , Alessandro Valentino Matheoud , Gabriele Gualco , Giovanni Boero

$^1$H nuclear spin-lattice relaxation and Dynamic Nuclear Polarization (DNP) have been studied in amorphous samples of trehalose sugar doped with TEMPO radicals by means of mechanical milling, in the 1.6 K $\div$ 4.2 K temperature range.…

We report on a polarized-neutron Laue diffraction experiment on a single crystal of neodynium doped lanthanum magnesium nitrate hydrate containing polarized proton spins. By using dynamic nuclear polarization to polarize the proton spins,…

We investigate analytically and numerically the Multiple Quantum (MQ) NMR dynamics in systems of nuclear spins 1/2 coupled by the dipole-dipole interactions in the case of the dipolar ordered initial state. We suggest two different methods…

Other Condensed Matter · Physics 2009-11-13 S. I. Doronin , E. B. Fel'dman , E. I. Kuznetsova , G. B. Furman , S. D. Goren

Nuclear spins and paramagnetic centers in a solid randomly group to form clusters featuring nearly-degenerate, hybrid states whose dynamics are central to processes involving nuclear spin-lattice relaxation and diffusion. Their…

Dynamic nuclear polarisation, which transfers the spin polarisation of electrons to nuclei, is routinely applied to enhance the sensitivity of nuclear magnetic resonance; it is also critical in spintronics, particularly when spin…

We demonstrate that the dynamic nuclear polarization (DNP) of phosphorus donors in silicon can be very effective in a magnetic field of 4.6 T and at temperatures below 1 K. The DNP occurs due to the Overhauser effect following a cross…

Spin engineering of advanced pulse sequences has had a transformative impact on the development of nuclear magnetic resonance (NMR) spectroscopy, to an extending degree also electron paramagnetic resonance (EPR), and the hybrid between the…

Chemical Physics · Physics 2025-01-31 Jose P. Carvalho , Anders Bodholt Nielsen , Eniko Baligacs , Nino Wili , Niels Chr. Nielsen

We report on a study of Dynamic Nuclear Polarization and electron and nuclear spin relaxation of atomic hydrogen and deuterium in solid molecular matrices of H$_{2}$, D$_{2}$, and HD mixtures. The electron and nuclear spin relaxation times…

Atomic and Molecular Clusters · Physics 2017-02-08 S. Sheludiakov , J. Ahokas , J. Järvinen , O. Vainio , L. Lehtonen , S. Vasiliev , D. M. Lee , V. V. Khmelenko

In a dynamic nuclear polarization experiment on a 40 mM solution of 4-amino-TEMPO in a 40:60 water/glycerol mixture, we have observed that the bulk dipolar reservoir is cooled to a spin temperature of 15.5 micro-K, following microwave…

Other Condensed Matter · Physics 2009-04-01 Anatoly E. Dementyev , David G. Cory , Chandrasekhar Ramanathan

At the magnetic fields of common NMR instruments, electron Zeeman frequencies are too high for efficient electron-nuclear dipolar cross-relaxation to occur in solution. The rate of that process fades with the electron Zeeman frequency as…

Quantum Physics · Physics 2021-04-22 Maria Grazia Concilio , Murari Soundararajan , Lucio Frydman , Ilya Kuprov

We analyze the polarization of nuclear spins in a quantum dot induced by a single-electron spin that is electrically driven to perform coherent Rabi oscillations. We derive the associated nuclear-spin polarization rate and analyze its…

Mesoscale and Nanoscale Physics · Physics 2023-10-25 Peter Stano , Takashi Nakajima , Akito Noiri , Seigo Tarucha , Daniel Loss

Amplification of a single spin state using nuclear magnetic resonance (NMR) techniques in a rotating frame is considered. The main aim is to investigate the efficient of various schemes for quantum detection. Results of numerical simulation…

Quantum Physics · Physics 2007-08-31 Gregory B. Furman , Victor M. Meerovich , Vladimir L. Sokolovsky
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