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The surface structure of SrTiO3(001) thin films homoepitaxially grown by PLD in step-flow mode was characterized using low temperature STM. It was found that one-dimensional (1D) TiOx-based nanostructures were formed on the thin film…

Materials Science · Physics 2015-05-18 Katsuya Iwaya , Takeo Ohsawa , Ryota Shimizu , Tomihiro Hashizume , Taro Hitosugi

Epitaxial SrTiO$_3$ (STO) on Si is nowadays the benchmark initial platform for the further addition of functional oxides on Si. Starting the growth of STO on a Sr-passivated Si substrate with 1/2 monolayer (ML) Sr coverage and a (1 $\times$…

Materials Science · Physics 2022-02-14 Wen-Yi Tong , Eric Bousquet , Matjaž Spreitzer , Philippe Ghosez

Oxide electronics relies on the availability of epitaxial oxide thin films. The extreme flexibility of the chemical composition of ABO3 perovskites and the broad spectrum of properties they cover, inspire the creativity of scientists and…

Materials Science · Physics 2014-04-01 Florencio Sanchez , Carmen Ocal , Josep Fontcuberta

Using low energy Time-of-Flight Scattering and Recoil Spectroscopy (TOF-SARS) and Mass Spectroscopy of Recoiled Ions (MSRI) we analyze the surface structure of an atomically smooth BaBiO$_3$ film grown by molecular beam epitaxy. We…

Other Condensed Matter · Physics 2009-11-13 A. Gozar , G. Logvenov , V. Y. Butko , I. Bozovic

The novel electronic properties emerging at interfaces between transition metal oxides, and in particular the discovery of conductivity in heterostructures composed of LaAlO$_3$ (LAO) and SrTiO$_3$ (STO) band insulators, have generated new…

To realize a chemical diffusion experiment for simple quantitative analysis of one-dimensional diffusion profiles requires the fabrication of a planar and chemically sharp interface between two phases, one serving as the diffusion source…

We have investigated how the recently-developed water-leaching method for atomically-flat SrTiO3 (STO) substrates affects the transport properties of LaAlO3 (LAO) and STO heterointerfaces. Using pulsed laser deposition at identical growth…

Materials Science · Physics 2016-04-04 J. G. Connell , J. Nichols , J. H. Gruenewald , D. -W. Kim , S. S. A. Seo

The availability of low-index rutile TiO2 single crystal substrates with atomically flat surfaces is essential for enabling epitaxial growth of rutile transition metal oxide films. The high surface energy of the rutile (001) surface often…

Materials Science · Physics 2016-03-23 Yang Wang , Shinbuhm Lee , Paolo Vilmercati , Ho Nyung Lee , Hanno H. Weitering , Paul C. Snijders

SrTiO$_{3}$ is one of the most popular insulating single-crystal substrates for various complex-oxide thin film growths, because of its good lattice match with many complex oxide films. Here, we show that a common thin film processing…

Materials Science · Physics 2011-10-11 Heiko Gross , Namrata Bansal , Yong-Seung Kim , Seongshik Oh

We have fabricated epitaxial films of CeTiO3 (CTO) on (001)oriented SrTiO3(STO) substrates, which exhibit highly insulating and diamagnetic properties. X-ray photoelectron spectroscopy (XPS) was to establish the 3+ valence state of the Ve…

Strongly Correlated Electrons · Physics 2018-08-01 Pramod Ghising , Debarchan Das , Shubhankar Das , Z. Hossain

Atomically-abrupt interfaces in transition metal oxide (TMO) heterostructures could host a variety of exotic condensed matter phases that may not be found in the bulk materials at equilibrium. A critical step in the development of such…

A first-principles atomic orbital-based electronic structure method is used to investigate the low index surfaces of rutile Titanium Dioxide. The method is relatively cheap in computational terms, making it attractive for the study of oxide…

Materials Science · Physics 2009-10-28 O. Gulseren , R. James , D. W. Bullett

In this report, the optical properties of Ta doped SrTiO3 (STO) due to its potential in transparent conducting oxides (TCOs) is explored by a combination of theoretical studies based on density functional theory and spectroscopic…

Materials Science · Physics 2024-11-25 Shammi Kumar , Raja Sen , Mamta Arya , Sankar Dhar , Priya Johari

SrTiO$_3$ thin films were used as a model system to study the effects of strain and epitaxial constraint on structural phase transitions of perovskite films. The basic phenomena revealed will apply to a variety of important structural…

Other Condensed Matter · Physics 2007-05-23 Feizhou He , B. O. Wells , S. M. Shapiro

Atomically resolved scanning tunneling microscopy (STM) and x-ray photoelectron spectroscopy (XPS) are used to gain atomic-scale insights into the heteroepitaxy of lanthanum-strontium manganite (LSMO, La$_{1-x}$Sr$_x$MnO$_{3-{\delta}}$, $x$…

Mesoscale and Nanoscale Physics · Physics 2023-11-28 Giada Franceschi , Renè Heller , Michael Schmid , Ulrike Diebold , Michele Riva

We have investigated the growth of BaTiO3 thin films deposited on pure and 1% Nb-doped SrTiO3(001) single crystals using atomic oxygen assisted molecular beam epitaxy (AO-MBE) and dedicated Ba and Ti Knudsen cells. Thicknesses up to 30 nm…

Materials Science · Physics 2015-06-12 A. Barbier , C. Mocuta , D. Stanescu , P. Jegou , N. Jedrecy , H. Magnan

A comparative first principles pseudopotential study of the adsorption and migration profiles of single Pt and Au atoms on the stoichiometric and reduced TiO2 rutile (110) surfaces is presented. Pt and Au behave similarly with respect to…

Materials Science · Physics 2009-11-10 Hakim Iddir , Serdar Ogut , Nigel D. Browning , Mark M. Disco

Direct observations using scanning transmission electron microscopy unveil an intriguing interfacial bi-layer that enables epitaxial growth of a strain-free, monoclinic, bronze-phase VO2(B) thin film on a perovskite SrTiO3 (STO) substrate.…

Understanding and manipulating properties emerging at a surface or an interface require a thorough knowledge of structure-property relationships. We report a study of a prototype oxide system, La2/3Sr1/3MnO3 grown on SrTiO3(001), by…

Strongly Correlated Electrons · Physics 2019-04-11 Lina Chen , Zhen Wang , Gaomin Wang , Hangwen Guo , Mohammad Saghayezhian , Zhaoliang Liao , Yimei Zhu , E. W. Plummer , Jiandi Zhang

This study examines the application of transition metal-doped SrTiO3 in photovoltaic technologies, such as photocatalysis. The core objective is to evaluate how different dopants influence the structural and electronic characteristics of…

Materials Science · Physics 2024-10-15 Zdeněk Jansa , Lucie Prušáková , Štěpánka Jansová , Pavel Calta , Pavol Šutta , Ján Minár