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We present a new method for the generation of rotationally and vibrationally state-selected, translationally cold molecular ions in ion traps. Our technique is based on the state-selective threshold photoionization of neutral molecules…

Chemical Physics · Physics 2010-06-30 Xin Tong , Alexander H. Winney , Stefan Willitsch

The generation and evolution of entanglement in quantum many-body systems is an active area of research that spans multiple fields, from quantum information science to the simulation of quantum many-body systems encountered in condensed…

Trapped ions are among the leading platforms for quantum technologies, particularly in the field of quantum computing. Detecting states of trapped ions is essential for ensuring high-fidelity readouts of quantum states. In this work, we…

Samples of ultracold 174 Yb+ ions, confined in a linear radio-frequency Paul trap, are heated via self-induced micromotion interruption, while their temperature, density, and therefore structural phase are monitored and simulated. The…

Atomic Physics · Physics 2015-06-12 Kuang Chen , Scott T. Sullivan , Wade G. Rellergert , Eric R. Hudson

Trapped ions arranged in Coulomb crystals provide us with the elements to study the physics of a single spin coupled to a boson bath. In this work we show that optical forces allow us to realize a variety of spin-boson models, depending on…

Quantum Physics · Physics 2009-11-13 D. Porras , F. Marquardt , J. von Delft , J. I. Cirac

We investigate the photodissociation of the metastable triplet state of HeH+ as well as its formation through the inverse process, radiative association. In models of astrophysical plasmas, HeH+ is assumed to be present only in the ground…

Chemical Physics · Physics 2015-06-12 J. Loreau , S. Vranckx , M. Desouter-Lecomte , N. Vaeck , A. Dalgarno

We present a theoretical and experimental investigation of homonuclear ionizing collisions of laser-cooled metastable helium atoms, considering both the fermionic He-3 and bosonic He-4 isotope. The theoretical description combines quantum…

Other Condensed Matter · Physics 2007-05-23 R. J. W. Stas , J. M. McNamara , W. Hogervorst , W. Vassen

Trapped ion systems are a leading platform for quantum information processing, but they are currently limited to 1D and 2D arrays, which imposes restrictions on both their scalability and their range of applications. Here, we propose a path…

Coulomb crystallisation of large ensembles of ions has in the past years been intensively studied experimentally with many spectacular results of relevance to infinite systems in one-, two-, and three-dimensions.While strings of a few ions…

Atomic and Molecular Clusters · Physics 2012-02-14 Michael Drewsen , Thierry Matthey , Anders Mortensen , Jan Petter Hansen

The quadrupole linear Paul trap is one of the key instruments in building highly stable atomic clocks. However, a frequency reference based on a single trapped ion is limited in stability due to the time needed for the interrogation cycle…

Instrumentation and Detectors · Physics 2021-12-07 Martin Oral , Lukáš Slodička , Ondřej Číp

We investigate the motional resonances of dual-species Coulomb crystals comprised of $^9$Be$^+$ and $^{24}$Mg$^+$ ions held in a 4-rod linear Paul trap. Our experimental data and simulations show that the secular motion of such mixed…

Atomic Physics · Physics 2021-02-16 Byoung-moo Ann , Fabian Schmid , Jonas Krause , Theodor W. Hänsch , Thomas Udem , Akira Ozawa

We describe one-dimensional photonic crystals that support a guided mode suitable for atom trapping within a unit cell, as well as a second probe mode with strong atom-photon interactions. A new hybrid trap is analyzed that combines optical…

Optics · Physics 2013-09-17 C. -L. Hung , S. M. Meenehan , D. E. Chang , O. Painter , H. J. Kimble

We demonstrate the cooling of a two species ion crystal consisting of one $^9Be^+$ and one $^{24}Mg^+$ ion. Since the respective cooling transitions of these two species are separated by more than 30 nm, laser manipulation of one ion has…

In this article, the dynamics of an unbalanced two-ion crystal comprising the 'target' and the 'sensor' ions confined in a Penning trap has been studied. First, the low amplitude regime is addressed. In this regime, the overall potential…

We report the generation, trapping and sympathetic cooling of individual conformers of molecular ions with the example of cis- and trans-meta-aminostyrene. Following conformationally selective photoionization, the incorporation of the…

Chemical Physics · Physics 2023-08-09 Lei Xu , Jutta Toscano , Stefan Willitsch

Atomic-scale crystal defects in Si are quantum-light sources offering tantalizing integration with existing photonic technologies. Yet, the controlled creation of near-infrared color centers for long- haul quantum communication and…

We investigate theoretically the dissociative ionization of a H2+ molecule using two ultrashort laser (pump-probe) pulses. The pump pulse prepares a dissociating nuclear wave packet on an ungerade surface of H2+. Next, an UV (or XUV) probe…

Quantum Physics · Physics 2013-05-29 Szczepan Chelkowski , André D. Bandrauk

We study the Doppler-cooling of radial two-dimensional (2D) Coulomb crystals of trapped barium ions in a radiofrequency trap. Ions in radial 2D crystals experience micromotion of an amplitude that increases linearly with the distance from…

We report the realization of a BEC of metastable helium-4 atoms (4He*) in an all optical potential. Up to 10^5 spin polarized 4He* atoms are condensed in an optical dipole trap formed from a single, focused, vertically propagating far…

Quantum Gases · Physics 2010-05-31 G. B. Partridge , J. -C. Jaskula , M. Bonneau , D. Boiron , C. I. Westbrook

There is a growing interest in high-precision spectroscopy and frequency metrology for fundamental studies using sympathetically cooled highly charged ions (HCIs) embedded in Coulomb crystals of laser-cooled ions. In order to understand how…