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The use of radioactive molecules for fundamental physics research is a developing interdisciplinary field limited dominantly by their scarce availability. In this work, radioactive molecular ion beams containing actinide nuclei extracted…
Trapped atomic ions find wide applications ranging from precision measurement to quantum information science and quantum computing. Among the different atomic species employed, beryllium ions are widely used due to its light mass and…
Direct dissociative recombination and resonant ion-pair formation reactions of $\mathrm{HeH^+}$ are theoretically studied using time-dependant wave-packets methods. The wave packets are propagated on potential energy curves that are in…
While laser excitation of the nuclear isomeric transition in $^{229}$Th has been recently achieved for thorium atoms embedded in large-bandgap crystals, laser excitation and characterization of the nuclear transition in trapped…
We recently used a compact Penning trap to capture and isolate highly-charged ions extracted from an electron beam ion trap (EBIT) at the National Institute of Standards and Technology (NIST). Isolated charge states of highly-stripped argon…
We report on photo ionization of ultracold magnetically trapped Rb atoms on an atom chip. The atoms are trapped at 5 $\mu $K in a strongly anisotropic trap. Through a hole in the chip with a diameter of 150 $\mu $m two laser beams are…
Recent experimental work on the photorecombination and the photoionization of astrophysically relevant atomic ions employing the merged-beams technique at heavy-ion storage-rings and synchrotron-light sources, respectively, is summarized.…
We demonstrate a spatial-imaging thermometry technique for ions in a one-dimensional Coulomb crystal by relating their imaged spatial extent along the linear radiofrequency ion trap axis to normal modes of vibration of coupled oscillators…
High-resolution photoionization experiments were carried out using beams of Be-like C$^{2+}$, N$^{3+}$, and O$^{4+}$ ions with roughly equal populations of the $^1$S ground-state and the $^3$P$^o$ manifold of metastable components. The…
We use (1+1$'$) resonance-enhanced multiphoton photodissociation (REMPD) to detect the population in individual rovibronic states of trapped HfF$^+$ with a single-shot absolute efficiency of 18%, which is over 200 times better than that…
The mechanism of ionization of helium droplets has been investigated in numerous reports but one observation has not found a satisfactory explanation: How are $He^+$ ions formed and ejected from undoped droplets at electron energies below…
Linear strings of trapped atomic ions held in radio-frequency (rf) traps constitute one of the leading platforms for quantum simulation experiments, allowing for the investigation of interacting quantum matter. However, linear ion strings…
We describe a hybrid vacuum system in which a single ion or a well defined small number of trapped ions (in our case Ba$^+$ or Rb$^+$) can be immersed into a cloud of ultracold neutral atoms (in our case Rb). This apparatus allows for the…
We have performed laser cooling of Mg ions confined in a Penning trap. The externally produced ions were captured in flight, stored and laser cooled. Laser-induced fluorescence was observed perpendicular to the cooling laser axis. Optical…
Large, 3D trapped ion crystals offer improved sensitivity in quantum sensing protocols, and are expected to be implemented as platforms in near-future experiments. However, numerical techniques used to study the laser cooling of such…
Coulomb crystals -- ordered structures of cold ions confined in ion traps -- find applications in a variety of research fields. The number and temperature of the ions forming the Coulomb crystals are two key attributes of interest in many…
The electronic structure of the (LiYb)$^+$ molecular ion is investigated with two variants of the coupled cluster method restricted to single, double, and noniterative or linear triple excitations. Potential energy curves for the ground and…
We investigate the mechanism of damping and heating of trapped ions associated with the polarization of the residual background gas induced by the oscillating ions themselves. Reasoning by analogy with the physics of surface electrons in…
We present a detailed theoretical study of the rotational excitation of CH$^+$ due to reactive and nonreactive collisions involving C$^+(^2P)$, H$_2$, CH$^+$, H and free electrons. Specifically, the formation of CH$^+$ proceeds through the…
We present a scheme to embed molecular anions in a gas of ultracold rubidium atoms as a route towards the preparation of cold molecular ions by collisional cooling with ultracold atoms. Associative detachment as an important loss process in…